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Laser Physics

Spatially structured optical effects in semiconductor quantum dots via biexciton coherence

Khalid Mujasam Batoo, F. Al-dolaimy, Mohd Hafiz Mohd Zaid, H Sharif, Fadhil A. Rasen, Sajjad Hussain, Karrar Shareef Mohsen, S H Kareem, Ahmed Alawadi, Ali Hashiem Alsaalamy

Published Sep 7, 2023• 2 citations
Publisher

Abstract

Abstract In this paper, we study the spatially structured optical effects that occur when weak laser lights interact with coherently prepared semiconductor quantum dots (SQDs). Initially, the SQD is prepared in a coherent superposition of the lower exciton states. By utilizing two weak optical vortex fields that couple to a biexciton state, we observe spatially dependent effects of the absorption of probe fields. Using the well-established Maxwell–Bloch equations, we analyze the generation of composite optical vortex beams within this system. Our investigation revolves around the formation of different types of spatially dependent beams, exploring their properties and characteristics. Additionally, the transfer of optical vortices through the parametric generation process is examined, for the case where only one vortex beam is present at the beginning of the medium. This study provides insights into the spatially structured optical phenomena in coherently prepared SQDs and contributes to the understanding of light–matter interactions in such systems.

DOI
10.1088/1555-6611/acf4e5

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Exciton-biexciton coherent coupling effects are examined in semiconductor quantum dots. The exciton absorption spectrum is measured with the microphotoluminescence excitation technique in a single InGaAs quantum dot. The spectrum changes from a Lorenztian-type line shape to an unusual dip-shaped line shape with increasing excitation intensities in a higher exciton state where there is a large oscillator strength between the exciton and biexciton states. The intensity dependence of the dip energy width clearly indicates that coherent Rabi oscillation occurs between the exciton and biexciton states. The absorption properties with excitation light of different polarizations show that the dip-shaped spectra only appear when there is a large biexciton state population with linear polarization. A theoretical analysis undertaken with the density matrix method agrees well with experimental results. This agreement reveals that exciton-biexciton coherent interactions lead to unusual absorption spectra and contribute crucially to the optical properties of quantum dots. The exciton-biexciton coherent effects provide a scheme for controlling four distinguishable states, which can be applied to a demonstration of quantum gate operations.
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