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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Driving the Superfluid-Supersolid Phase-Transition by Heating

Juan Sánchez-Baena, Claudia Politi, Fabian Maucher, Francesca Ferlaino, Thomas Pohl

Published Jun 26, 2023• 0 citations
Publisher

Abstract

It is intuitive to think that heating any material leads to an increase in random thermal motion and, thereby, usually counteracts any ordering efforts. For example, heating ice leads to the formation of a liquid and ultimately to a gas. However, experiments with dipolar Bose-Einstein condensates suggested that this general phenomenology does not always take place [1]. In order to describe the surprising superfluid-supersolid transition upon an increase in temperature at fixed condensed particle number we employ Bogoliubov theory with local density approximation [2], [3] and, indeed, find that such behaviour can also be expected theoretically [Fig. 1(a)]. With this approach we find [3] that the scaling with respect to density of the shift in energy due to thermal fluctuations is opposite to that of quantum fluctuations and, therefore, promotes the formation of high density regions [Fig. 1(b)]. Consistent with that we find that an increase in temperature promotes roton-softening [Fig. 1(c)]. Furthermore, we find good agreement between the experimentally measured density and the theoretical prediction including thermal fluctuations, whereas not taking thermal corrections into account yields a different result [Fig. 1(d)]. These findings call for further investigation of the surprising thermodynamic behaviour of ultracold quantum ferrofluids.

DOI
10.1109/cleo/europe-eqec57999.2023.10232258

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It is intuitive to think that heating any material leads to an increase in random thermal motion and, thereby, usually counteracts any ordering efforts. For example, heating ice leads to the formation of a liquid and ultimately to a gas. However, experiments with dipolar Bose-Einstein condensates suggested that this general phenomenology does not always take place [1]. In order to describe the surprising superfluid-supersolid transition upon an increase in temperature at fixed condensed particle number we employ Bogoliubov theory with local density approximation [2], [3] and, indeed, find that such behaviour can also be expected theoretically [Fig. 1(a)]. With this approach we find [3] that the scaling with respect to density of the shift in energy due to thermal fluctuations is opposite to that of quantum fluctuations and, therefore, promotes the formation of high density regions [Fig. 1(b)]. Consistent with that we find that an increase in temperature promotes roton-softening [Fig. 1(c)]. Furthermore, we find good agreement between the experimentally measured density and the theoretical prediction including thermal fluctuations, whereas not taking thermal corrections into account yields a different result [Fig. 1(d)]. These findings call for further investigation of the surprising thermodynamic behaviour of ultracold quantum ferrofluids.
Raising the temperature of a material enhances the thermal motion of particles. Such an increase in thermal energy commonly leads to the melting of a solid into a fluid and eventually vaporises the liquid into a gaseous phase of matter. Here, we study the finite-temperature physics of dipolar quantum fluids and find surprising deviations from this general phenomenology. In particular, we describe how heating a dipolar superfluid from near-zero temperatures can induce a phase transition to a supersolid state with a broken translational symmetry. We discuss the observation of this effect in experiments on ultracold dysprosium atoms, which opens the door for exploring the unusual thermodynamics of dipolar quantum fluids.
Recent experiments have shown that raising the temperature of a dipolar gas under certain conditions leads to a transition to a supersolid state. Here, we employ the path integral Monte Carlo method, which exactly accounts for both thermal and correlation effects, to study that phenomenology in a system of ^{162}Dy atoms in the canonical ensemble. Our microscopic description allows the quantitative characterization of the emergence of spatial order and superfluidity, the two ingredients that define a supersolid state. Our calculations prove that temperature on its own can promote the formation of a supersolid in a dipolar system. Furthermore, we bridge this exotic phenomenology with the more usual melting of the supersolid at a higher temperature. Our results offer insight into the interplay between thermal excitations, the dipole-dipole interaction, quantum statistics, and supersolidity.
Phase transitions share the universal feature of enhanced fluctuations near the transition point.Here, we show that density fluctuations reveal how a Bose-Einstein condensate of dipolar atoms spontaneously breaks its translation symmetry and enters the supersolid state of matter-a phase that combines superfluidity with crystalline order.We report on the first direct in situ measurement of density fluctuations across the superfluid-supersolid phase transition.This measurement allows us to introduce a general and straightforward way to extract the static structure factor, estimate the spectrum of elementary excitations, and image the dominant fluctuation patterns.We observe a strong response in the static structure factor and infer a distinct roton minimum in the dispersion relation.Furthermore, we show that the characteristic fluctuations correspond to elementary excitations such as the roton modes, which are theoretically predicted to be dominant at the quantum critical point, and that the supersolid state supports both superfluid as well as crystal phonons.
In one dimension, quantum fluctuations prevent the appearance of long-range order in a supersolid, and only quasi-long-range order can survive. We derive this quantum critical behavior and study its influence on the superfluid response and properties of the solid. The analysis is based on an effective low-energy description accounting for the two coupled Goldstone modes. We find that the quantum phase transition from the superfluid to the supersolid is shifted by quantum fluctuations from the position where the local formation of a solid structure takes place. For current experimental parameters with dipolar atomic gases, this shift is extremely small and cannot be resolved yet, i.e., current observations in experiments are expected to be in agreement with predictions from mean-field theory based on the extended Gross-Pitaevskii formalism.
Thermal fluctuations, the microscopic fluctuations of things due to their temperature, counteract order in many-body systems. Thermal fluctuations often lead to high-temperature disordered phases and low-temperature ordered ones. In lower dimensions, thermal fluctuations are relatively stronger with two-dimensional materials being just on the brink of thermal fluctuations destroying their order. Twodimensional materials therefore display unique behaviour, for example undergoing a superfluid phase transition driven by point-like topological defects. In this work, we realise two-dimensional bosonic quantum gases of the isotope Rb-87 in precisely controlled potentials to study how quantum-tunnelling and spatially disordered potentials affect the phases of matter they form. We also present a new scheme for cooling quantum gases directly in the finely tuned radiofrequency-dressed traps confining the gases in our experiments. To study tunnel-coupled gases, this work utilises a novel method to read out information from bilayer quantum gas experiments by analysing noise patterns arising from interference effects. We find that quantum-tunnelling between the two layers in a bilayer system can cause both layers to remain superfluid at higher temperatures than without quantum tunnelling. We compare our results to predictions using renormalisation-group theory and numerical simulations. We experimentally observe the predicted double-layer superfluid phase, a novel phase where the U(1) symmetry of the relative phase is broken and relative excitations are suppressed. Separately, we investigate the topological Berezinskii-Kosterlitz-Thouless phase transition in disordered two-dimensional Bose gases. We find that such systems can be driven across this phase transition by increasing the strength of an applied disordered potential. We experimentally map out the phase diagram for a continuous 2D Bose gas in the presence of disorder, which has not previously been carried out to the best of our knowledge. We find that the presence of disorder increases the number of topological defects at a given temperature while reducing the rate at which the number of defects increases with temperature. The experimental results for 2D disordered Bose gases are in qualitative agreement with numerical simulations for the parameter regime studied.