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arXiv:2009.08910 · Physical Review X

Density Fluctuations across the Superfluid-Supersolid Phase Transition in a Dipolar Quantum Gas

Jens Hertkorn, Jan-Niklas Schmidt, Fabian Böttcher, Mingyang Guo, Matthias Schmidt, K. S. H. Ng, Sean Graham, Hans Peter Büchler, Tim Langen, Martin W. Zwierlein, Tilman Pfau

Published Feb 23, 2021• 71 citations
arXivHTMLPDF

Abstract

Phase transitions share the universal feature of enhanced fluctuations near the transition point.Here, we show that density fluctuations reveal how a Bose-Einstein condensate of dipolar atoms spontaneously breaks its translation symmetry and enters the supersolid state of matter-a phase that combines superfluidity with crystalline order.We report on the first direct in situ measurement of density fluctuations across the superfluid-supersolid phase transition.This measurement allows us to introduce a general and straightforward way to extract the static structure factor, estimate the spectrum of elementary excitations, and image the dominant fluctuation patterns.We observe a strong response in the static structure factor and infer a distinct roton minimum in the dispersion relation.Furthermore, we show that the characteristic fluctuations correspond to elementary excitations such as the roton modes, which are theoretically predicted to be dominant at the quantum critical point, and that the supersolid state supports both superfluid as well as crystal phonons.

DOI
10.1103/physrevx.11.011037

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Phase transitions share the universal feature of enhanced fluctuations near the transition point.Here, we show that density fluctuations reveal how a Bose-Einstein condensate of dipolar atoms spontaneously breaks its translation symmetry and enters the supersolid state of matter-a phase that combines superfluidity with crystalline order.We report on the first direct in situ measurement of density fluctuations across the superfluid-supersolid phase transition.This measurement allows us to introduce a general and straightforward way to extract the static structure factor, estimate the spectrum of elementary excitations, and image the dominant fluctuation patterns.We observe a strong response in the static structure factor and infer a distinct roton minimum in the dispersion relation.Furthermore, we show that the characteristic fluctuations correspond to elementary excitations such as the roton modes, which are theoretically predicted to be dominant at the quantum critical point, and that the supersolid state supports both superfluid as well as crystal phonons.
We observe signatures of radial and angular roton excitations around a droplet crystallization transition in dipolar Bose-Einstein condensates. In situ measurements are used to characterize the density fluctuations near this transition. The static structure factor is extracted and used to identify the radial and angular roton excitations by their characteristic symmetries. These fluctuations peak as a function of the interaction strength indicating the crystallization transition of the system. We compare our observations to a theoretically calculated excitation spectrum allowing us to connect the crystallization mechanism with the softening of the angular roton modes.
Motivated by a recent experiment [L. Chomaz et al., Nat. Phys. 14, 442 (2018)], we perform numerical simulations of a dipolar Bose-Einstein condensate (BEC) in a tubular, periodic confinement at T=0T=0T=0 within density functional theory, where the beyond-mean-field correction to the ground-state energy is included in the local density approximation. We study the excitation spectrum of the system by solving the corresponding Bogoliubov--de Gennes equations. The calculated spectrum shows a roton minimum, and the roton gap decreases by reducing the effective scattering length. As the roton gap disappears, the system spontaneously develops a periodic linear structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. This structure shows the hallmarks of a supersolid system, i.e., (i) a finite nonclassical translational inertia along the tube axis and (ii) the appearance of two gapless modes, i.e., a phonon mode associated with density fluctuations and resulting from the translational discrete symmetry of the system, and a Nambu-Goldstone gapless mode corresponding to phase fluctuations, resulting from the spontaneous breaking of the gauge symmetry. A further decrease in the scattering length eventually leads to the formation of a periodic linear array of self-bound droplets.
We investigate the excitation spectrum and compressibility of a dipolar Bose-Einstein condensate in an infinite tube potential in the parameter regime where the transition between superfluid and supersolid phases occurs. Our study focuses on the density range in which crystalline order develops continuously across the transition. Above the transition the superfluid shows a single gapless excitation band, phononic at small momenta and with a roton at a finite momentum. Below the transition, two gapless excitations branches (three at the transition point) emerge in the supersolid. We examine the two gapless excitation bands and their associated speeds of sound in the supersolid phase. Our results show that the speeds of sound and the compressibility are discontinuous at the transition, indicating a second-order phase transition. These results provide valuable insights into the identification of supersolid phenomena in dipolar quantum gases and the relationship to supersolidity in spin-orbit coupled gases.
In a recent experiment, it has been found that by tuning the interaction strength of a dipolar Bose-Einstein Condensate confined in a quasi-1D geometry orthogonal to the polarization direction, the roton gap vanishes, while density modulations are induced in the trapped gas. This suggests the possibility of realizing a supersolid in dipolar quantum gases. Inspired by this experiment, we simulate a dipolar BEC in a ring geometry by confining the dipoles in a ”tube” orthogonal to the polarization direction and enforcing periodic boundary conditions. Our calculations are based on a Density Functional approach where the total energy density functional includes the beyond-mean-field correction of Lee-Huang-Yang, which partially accounts for quantum fluctuations. We study the ground state properties of the system by evolving in imaginary time the EulerLagrange equation derived from the variational principle. We also study the excitation spectrum of the system by solving the corresponding Bogoliubov-de Gennes equations. We find that the calculated excitation spectrum shows indeed a roton minimum, and the roton gap can become vanishingly small by reducing the effective scattering length. As the roton gap disappears, we find that the system spontaneously develops in its ground-state a periodic structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. We find that this structure shows the hallmarks of a supersolid system, i.e. (i) a finite non-classical translational inertia and (ii) the appearance, besides the phonon mode, of the Nambu-Goldstone gapless mode corresponding to fluctuations in the phase, and related to the spontaneous breaking of the gauge symmetry.
We study the spectrum of elementary excitations of a dipolar Bose gas in a three-dimensional anisotropic trap across the superfluid-supersolid phase transition. Theoretically, we show that, when entering the supersolid phase, two distinct excitation branches appear, respectively associated with dominantly crystal and superfluid excitations. These results confirm infinite-system predictions, showing that finite-size effects play only a small qualitative role, and connect the two branches to the simultaneous occurrence of crystal and superfluid orders. Experimentally, we probe compressional excitations in an Er quantum gas across the phase diagram. While in the Bose-Einstein condensate regime the system exhibits an ordinary quadrupole oscillation, in the supersolid regime we observe a striking two-frequency response of the system, related to the two spontaneously broken symmetries.