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Communications in Theoretical Physics

Influence of pump brightness, self-Kerr and cross-Kerr effects on the entanglement of partially degenerate triple-photon state

Da Zhang, Zhihong Ren

Published Aug 22, 2023• 4 citations
Publisher

Abstract

Abstract Recently, partially degenerate triple-photon states (TPS) generated by the third-order spontaneous parametric down-conversion have been observed in a superconducting cavity (2020, Phys. Rev. X 10, 011011). Their non-Gaussian entanglement properties, characterized by a series of high-order covariance matrices, have also been theoretically revealed. Here, we use the non-Gaussian entanglement criterion proposed in (2021, Phy. Rev. Lett. 127, 150502) and the logarithmic negativity to study the effect of pump brightness, self-Kerr and cross-Kerr interactions on the entanglement of partially degenerate TPS (PDTPS). We find that the brighter the pump, the easier the entanglement of PDTPS leap to higher-order covariance matrices. Although both self-Kerr and cross-Kerr interactions induce nonlinear phase shifts and weaken the entanglement of PDTPS, cross-Kerr interactions can effectively raise the threshold of entanglement loaded on the third-order covariance matrix. These results can contribute to our understanding of the mechanism of the generation of unconditional non-Gaussian entanglement.

DOI
10.1088/1572-9494/acf27e

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•Aug 16, 2019•3 citations
Abstract Recently, partially degenerate triple-photon states (TPS) generated by the third-order spontaneous parametric down-conversion have been observed in a superconducting cavity (2020, Phys. Rev. X 10, 011011). Their non-Gaussian entanglement properties, characterized by a series of high-order covariance matrices, have also been theoretically revealed. Here, we use the non-Gaussian entanglement criterion proposed in (2021, Phy. Rev. Lett. 127, 150502) and the logarithmic negativity to study the effect of pump brightness, self-Kerr and cross-Kerr interactions on the entanglement of partially degenerate TPS (PDTPS). We find that the brighter the pump, the easier the entanglement of PDTPS leap to higher-order covariance matrices. Although both self-Kerr and cross-Kerr interactions induce nonlinear phase shifts and weaken the entanglement of PDTPS, cross-Kerr interactions can effectively raise the threshold of entanglement loaded on the third-order covariance matrix. These results can contribute to our understanding of the mechanism of the generation of unconditional non-Gaussian entanglement.
Nondegenerate triple-photon parametric down-conversion (NTPD) is a potential source for unconditional tripartite non-Gaussian entangled states of continuous variables. Recent experiment has demonstrated strong third-order correlations among bright photon triplets via microwave NTPD in a superconducting cavity [C. W. Sandbo Cheng et al., Phys. Rev. X 10, 011011 (2020)]. Previous theoretic works have revealed that only short-time genuine tripartite non-Gaussian entanglement can be generated in NTPD even in the absence of dissipation. In this paper, we investigate the properties of tripartite non-Gaussian entanglement and steering in the cavity output field by taking into account the cavity dissipation. We first derive experimentally detectable criteria for fully inseparable and genuine tripartite non-Gaussian entanglement and steering. With the criteria, we then find that steady-state tripartite non-Gaussian entanglement and steering can be generated in the output field, although they merely exist in the short-time regime inside the cavity. We also find that the initial cavity-field coherent states can obviously enhance the steady-state and transient tripartite entanglement and steering, in comparison to the case of initial vacuum states. We finally show that the output tripartite non-Gaussian steerable correlations can be applied to the remote generation of negative Wigner-function quantum states by homodyne detection.
We investigate the coupling of the fully degenerate triple-photon state generated by three-mode spontaneous parametric down-conversion with the vacuum at a beam splitter via numerical modeling. By using fully degenerate triple-photon states with distinct pump phases as input states, four different squeezed states are extracted at the output, which can be referred to as zero-phase, $\ensuremath{\pi}/2$-phase, $\ensuremath{\pi}$-phase, and $3\ensuremath{\pi}/2$-phase positive Wigner squeezed states. The non-Gaussianity evolution during the coupling process is quantitatively analyzed via quantum relative entropy, and the entanglement between the two output modes is confirmed from an entropic perspective. Furthermore, the entanglement properties of the zero-phase and $\ensuremath{\pi}$-phase positive Wigner squeezed states at the third- and sixth-order moments are revealed by applying the partial transpose positive criterion based on the higher-order covariance matrix. In particular, it is found that the steerability of the two output modes at the third- and sixth-order moments can be dynamically controlled by adjusting the intensity of the input light and the transmission of the beam splitter. These results enrich the repertoire of squeezed states in quantum optics and offer a feasible approach for the deterministic preparation of non-Gaussian entanglement via coupling fully degenerate triple-photon states with vacuum.
Very recently, strongly non-Gaussian states have been observed via a direct three-mode spontaneous parametric down-conversion in a superconducting cavity [Phys. Rev. X 10, 011011 (2020)]. The created multiphoton non-Gaussian correlations are attractive and useful for various quantum information tasks. However, how to detect and classify multipartite non-Gaussian entanglement has not yet been completely understood. Here, we present an experimentally practical method to characterize continuous-variable multipartite non-Gaussian entanglement, by introducing a class of nonlinear squeezing parameters involving accessible higher-order moments of phase-space quadratures. As these parameters can depend on arbitrary operators, we consider their analytical optimization over a set of practical measurements, in order to detect different classes of multipartite non-Gaussian entanglement ranging from fully separable to fully inseparable. We demonstrate that the nonlinear squeezing parameters act as an excellent approximation to the quantum Fisher information within accessible third-order moments. The level of the nonlinear squeezing quantifies the metrological advantage provided by those entangled states. Moreover, by analyzing the above-mentioned experiment, we show that our method can be readily used to confirm fully inseparable tripartite non-Gaussian entangled states by performing a limited number of measurements without requiring full knowledge of the quantum state.
Triple-photon states generated by three-mode spontaneous parametric down-conversion are the paradigm of unconditional non-Gaussian states, essential assets for quantum advantage. How to fully characterize their non-Gaussian entanglement remains however elusive. We propose here a set of sufficient and necessary conditions for separability of the broad family of spontaneously generated three-mode non-Gaussian states. We further derive state-of-the-art conditions for genuine tripartite non-Gaussian entanglement, the strongest class of entanglement. We apply our criteria to triple-photon states revealing that they are fully inseparable and genuinely entangled in moments of order 3n. Our results establish a systematic framework for characterizing the entanglement of triple-photon states and thus fostering their application in quantum information protocols.
We theoretically demonstrate through numerical methods that the triple-photon state generated by three-photon spontaneous parametric down-conversion is a non-Gaussian Greenberger-Horne-Zeilinger state, showing super-Gaussian statistics. Interestingly, the degree of entanglement between the modes of the triple-photon state is stronger than that corresponding to the two-mode squeezed vacuum state produced by a quadratic Hamiltonian with the same parameters. Furthermore, we propose a model to prepare two-mode sub-Gaussian entangled states with a tunable negative Wigner function based on quadrature projection measurements. We find that these Gaussian projection measurements with outcomes $X\ensuremath{\ge}1$ not only improve the entanglement of the residual two modes but also introduce a Gaussian component, resulting in the coexistence of Gaussian and non-Gaussian entanglement.
The flexible engineering of superconducting circuits, together with the nonlinearity available from Josephson junctions, have made microwave quantum optics a blooming research field in the past decade. Key experiments originally performed in the optical domain have become very accessible on this microwave-frequency, such that strong atom-field interactions and optical parametric interactions in microwave. From the latter, one example is the implementation of spontaneous parametric downconversion (SPDC). This process is particularly interesting as it can act as a nonclassical radiation source which give a number of potential applications in quantum information processing. We will focus on studying SPDC in microwave throughout this thesis. \n \nIn the first half of this thesis, from designs to measurements, we will explore the well-known two-photon parametric processes, SPDC and coherent coupling, which are generated by quadratic Hamiltonians. Using three resonant modes of a SQUID-terminated parametric cavity, we proceeded to combine different two-photon processes in an effort to demonstrate a multipartite nonclassical radiation source. With detailed system gain and noise calibration of our cryogenic microwave network, we confirmed our implementation by experimentally verifying that the generated states contain genuine tripartite entanglement. This multimode entangled radiation source can be an important resource for future experiments on quantum networking. \n \nWhile two-photon parametric processes have found numerous important applications, they have also been the limit of experiments for over three decades, with higher-order parametric processes seemingly out of reach. In the second half of this thesis, we explore the potential of parametric resonators for achieving such higher-order processes. To do this, we first studied the necessary conditions for accessing cubic Hamiltonians through our SQUID-based interactions. We then fabricated a device dedicated to performing three-photon processes through these cubic Hamiltonians. For the first time, we observed a direct generation of photon triplets by a single SPDC process in microwave . The generation rate can exceed a photon flux density of 60 photon per second per Hertz at the device output, far surpassing any record to date for photon triplets. We studied various pump configurations corresponding to different three-photon SPDC processes starting from a cold vacuum state. Pumping at triple the frequency of a single mode, we observed a phase-space distribution with a non-Gaussian profile which shows strong skewness (third moment) in the quadrature amplitude distribution. We reconstruct the Wigner function of the propagating states from the directly measured moment matrix, demonstrating Wigner negativity. Pumping at the sum frequency of three modes, we observed non-zero coskewness between the quadrature amplitudes of the modes. By analysing the output signals and comparing their characteristics to the predicted theoretical signatures, we confirm our implementation of three-photon SPDC processes generated by specific cubic Hamiltonians. These types of non-Gaussian states have been suggested as a resource enabling universal quantum computation with continuous variables. Our results thus open up the realm of three-photon quantum optics, enabling a wealth of novel experimental and theoretical studies.