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Photonic Indistinguishability of the Tin-Vacancy Center in Diamond

Jesús Arjona Martínez, Ryan A. Parker, Kevin C. Chen, Carola M. Purser, Linsen Li, Cathryn P. Michaels, Alexander M. Stramma, Romain Debroux, Isaac Harris, Martin Hayhurst, Eleanor C. Nichols, Matthew E. Trusheim, Dorian A. Gangloff, Dirk Englund, Mete Atatüre

Published Jan 1, 2023• 0 citations
Publisher

Abstract

Tin-vacancy centres in diamond are spin-photon interfaces with intrinsic environmental noise insensitivity. We reveal their high optical coherence in a nanostructured environment and generate single photons with a 99.7% purity and an indistinguishability of 63(9)%. [1]
DOI
10.1364/cleo_si.2023.sm1k.2

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Tin-vacancy centers in diamond are promising spin-photon interfaces owing to their high quantum efficiency, large Debye-Waller factor, and compatibility with photonic nanostructuring. Benchmarking their single-photon indistinguishability is a key challenge for future applications. Here, we report the generation of single photons with 99.7_{-2.5}^{+0.3}% purity and 63(9)% indistinguishability from a resonantly excited tin-vacancy center in a single-mode waveguide. We obtain quantum control of the optical transition with 1.71(1)-ns-long π pulses of 77.1(8)% fidelity and show it is spectrally stable over 100 ms. A modest Purcell enhancement factor of 12 would enhance the indistinguishability to 95%.
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The realization of quantum networks critically depends on establishing efficient, coherent light-matter interfaces. Optically active spins in diamond have emerged as promising quantum nodes based on their spin-selective optical transitions, long-lived spin ground states, and potential for integration with nanophotonics. Tin-vacancy (SnV -^{\,\textrm{-}}-) centers in diamond are of particular interest because they exhibit narrow-linewidth emission in nanostructures and possess long spin coherence times at temperatures above 1 K. However, a nanophotonic interface for SnV -^{\,\textrm{-}}- centers has not yet been realized. Here, we report cavity enhancement of the emission of SnV -^{\,\textrm{-}}- centers in diamond. We integrate SnV -^{\,\textrm{-}}- centers into one-dimensional photonic crystal resonators and observe a 40-fold increase in emission intensity. The Purcell factor of the coupled system is 25, resulting in channeling of the majority of photons (90%90\%90%) into the cavity mode. Our results pave the way for the creation of efficient, scalable spin-photon interfaces based on SnV -^{\,\textrm{-}}- centers in diamond.