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Efficient frequency conversion of non-diffracting modes via four-wave mixing in rubidium vapor

Onkar N. Verma, Niti Kant

Published Jun 8, 2023• 0 citations
Publisher

Abstract

Abstract We investigate the nonlinear frequency conversion of non-diffracting optical modes via non-degenerate four-wave mixing(FWM) process in rubidium vapor. In this process, two strong control fields and a weak probe field mutually interact via afour-level double-Λ type atomic system to produce a new frequency weak Stokes field which is a phase conjugate to probe. We show that any arbitrary mode such as Airy, Bessel, Mathieu, and Weber beams encoded initially in the spatial envelope of probe field are efficiently transferred to FWM Stokes field by satisfying the phase matching condition. Interestingly, we found that the transmitted intensity profiles of Stokes beam are identical to that of probe beam while phase profile is complimentary.The phase conjugation property of output beams is revealed by interfering them with a copropagating plane wave. We further found the fidelity in terms of structural similarity between two transmitted modes of about 99%, which substantiates the high efficiency of FWM process. The efficient transfer and frequency conversion of such diffraction-free beams may have potential applications in nonlinear optical and quantum technologies.

DOI
10.21203/rs.3.rs-2936007/v1

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Abstract We investigate the nonlinear frequency conversion of non-diffracting optical modes via non-degenerate four-wave mixing(FWM) process in rubidium vapor. In this process, two strong control fields and a weak probe field mutually interact via afour-level double-Λ type atomic system to produce a new frequency weak Stokes field which is a phase conjugate to probe. We show that any arbitrary mode such as Airy, Bessel, Mathieu, and Weber beams encoded initially in the spatial envelope of probe field are efficiently transferred to FWM Stokes field by satisfying the phase matching condition. Interestingly, we found that the transmitted intensity profiles of Stokes beam are identical to that of probe beam while phase profile is complimentary.The phase conjugation property of output beams is revealed by interfering them with a copropagating plane wave. We further found the fidelity in terms of structural similarity between two transmitted modes of about 99%, which substantiates the high efficiency of FWM process. The efficient transfer and frequency conversion of such diffraction-free beams may have potential applications in nonlinear optical and quantum technologies.
We investigate the nonlinear frequency conversion of nondiffracting optical modes via a nondegenerate four-wave mixing (FWM) process in rubidium vapor. In this process, two strong control fields and a weak probe field mutually interact via a four-level double-$\mathrm{\ensuremath{\Lambda}}$ type atomic system to produce a low frequency weak Stokes field which is a phase conjugate to probe. We show that any arbitrary mode such as Airy, Bessel, Mathieu, and Weber beams encoded initially in the spatial envelope of the probe field are efficiently transferred to the FWM Stokes field by satisfying the phase-matching condition. Interestingly, we found that the transmitted intensity profiles of the Stokes beam are identical to that of the probe beam, while the phase profile is complementary. The phase conjugation property of output beams is revealed by interfering them with a copropagating plane wave. We further found the fidelity in terms of structural similarity between two transmitted modes of about 9999%99, which substantiates the high efficiency of the FWM process. The efficient transfer and frequency conversion of such diffraction-free beams may have potential applications in nonlinear optical and quantum technologies.
We propose a scheme to transfer the spatial intensity as well as phase information encoded initially in the spatial profile of a weak probe field onto a newly generated Stokes field in a nonlinear process of four-wave mixing (FWM). The FWM process is explored in a gaseous medium consisting of atoms modeled as a three-level system in the $\mathrm{\ensuremath{\Lambda}}$ configuration. We found that different orders of Hermite-Gaussian and Laguerre-Gaussian modes carried by a probe beam are effectively transferred to a Stokes beam. Interestingly, the transferred intensity of the Stokes beam is a clone of the probe beam, whereas the phase profile is conjugate to the probe. The phase distribution of the transmitted modes at the exit of the medium is explored by superimposing them on a copropagating plane wave. Moreover, the parametric amplification due to the nonlinear process of FWM prevents any information loss due to linear absorption and permits us to work at high optical depths. We found a structural similarity between transferred images of about 9999%99, which provides clear evidence for the successful transfer of information in the FWM process.
We experimentally investigate the frequency conversion of vector beams with four-wave-mixing (FWM) in rubidium vapor. The conversion of vector beams from the probe beam to the conjugate beam is realized. In FWM experiments, the pump and the probe beam have orthogonal polarizations because of the polarization sensitivity of the FWM process and detection convenience. In order to satisfy the polarization sensitive phase matching condition and realize the nonlinear frequency conversion of vector beams, a Sagnac interferometer is used to form two FWM processes in the same rubidium cell, and two generated conjugate beams are combined with a polarizing beam splitter to form a conjugate vector beam. The experimental results agree well with our theoretical simulation. Compared with nonlinear optical crystals, the atomic vapor provides another platform to control and manipulate the vector beams nonlinearly.
We report on an experimental generation of Airy beams by four-wave mixing (FWM) in atomic vapor cells. This is achieved by using a non-degenerate FWM process, which occurs with two Gaussian pump beams and one Airy signal beam in hot Rubidium vapor. After satisfying the phase matching condition, a FWM field with the profile of an Airy beam can be generated. In our experiment, the diffraction-free and self-healing behaviors of the generated FWM beam are examined. The results shown that the generated FWM beam is an Airy beam. The nonlinear generation process can be extended to other configurations in the atomic medium, which will be useful for manipulation and application of Airy beams in atomic systems.
Abstract We theoretically investigate a N-type 87Rb atomic system for efficient generation and control of a non-degenerate four wave mixing (FWM) signal in pulsed regime. The susceptibility of the atomic medium is customized as a gain profile by a weak probe pulse and two strong continuous wave control fields which allow us to generate the pulsed FWM signal. We study the propagation dynamics of the generated FWM signal inside the nonlinear medium. The FWM signal obtains the exact shape of the probe pulse and travels without changing the shape whereas, the probe pulse is absorbed inside the nonlinear medium. The conversion efficiency of this scheme without a MW field is 5.36%. However, a MW field that couples two metastable ground states enhances the conversion efficiency to 20.6%. The generation and control of such FWM signal in pulsed regime has important applications in signal processing, optical communication and information science.
Coherent frequency conversion of vector beams (VBs) without distorting their intensity profile or spatial polarization distribution is important for novel applications in quantum and classical regimes. Here, we experimentally and theoretically investigate VB transfer from near-infrared to blue light using a Sagnac interferometer, combining the parametric four-wave mixing process in atomic vapor. The vector probe beam is converted into a completely different wavelength, and the vector mode of the generated blue beam is highly similar to the incident probe beam. These results may provide a feasible solution for communication interfaces in classical and quantum science fields based on atomic ensembles.