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Optics Letters

Trans-spectral vector beam nonlinear conversion via parametric four-wave mixing in alkali vapor

Churong Pan, Chengdong Yang, Huajie Hu, Jinwen Wang, Yingxin Zhang, Yan Qin, Dong Wei, Haixia Chen, Hong Gao, Fuli Li

Published Oct 14, 2021• 17 citations
Publisher

Abstract

Coherent frequency conversion of vector beams (VBs) without distorting their intensity profile or spatial polarization distribution is important for novel applications in quantum and classical regimes. Here, we experimentally and theoretically investigate VB transfer from near-infrared to blue light using a Sagnac interferometer, combining the parametric four-wave mixing process in atomic vapor. The vector probe beam is converted into a completely different wavelength, and the vector mode of the generated blue beam is highly similar to the incident probe beam. These results may provide a feasible solution for communication interfaces in classical and quantum science fields based on atomic ensembles.

DOI
10.1364/ol.441573

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Physical Review Research•Aug 20, 2021•11 citations
Coherent frequency conversion of vector beams (VBs) without distorting their intensity profile or spatial polarization distribution is important for novel applications in quantum and classical regimes. Here, we experimentally and theoretically investigate VB transfer from near-infrared to blue light using a Sagnac interferometer, combining the parametric four-wave mixing process in atomic vapor. The vector probe beam is converted into a completely different wavelength, and the vector mode of the generated blue beam is highly similar to the incident probe beam. These results may provide a feasible solution for communication interfaces in classical and quantum science fields based on atomic ensembles.
We experimentally investigate the frequency conversion of vector beams with four-wave-mixing (FWM) in rubidium vapor. The conversion of vector beams from the probe beam to the conjugate beam is realized. In FWM experiments, the pump and the probe beam have orthogonal polarizations because of the polarization sensitivity of the FWM process and detection convenience. In order to satisfy the polarization sensitive phase matching condition and realize the nonlinear frequency conversion of vector beams, a Sagnac interferometer is used to form two FWM processes in the same rubidium cell, and two generated conjugate beams are combined with a polarizing beam splitter to form a conjugate vector beam. The experimental results agree well with our theoretical simulation. Compared with nonlinear optical crystals, the atomic vapor provides another platform to control and manipulate the vector beams nonlinearly.
We investigate the nonlinear frequency conversion of nondiffracting optical modes via a nondegenerate four-wave mixing (FWM) process in rubidium vapor. In this process, two strong control fields and a weak probe field mutually interact via a four-level double-$\mathrm{\ensuremath{\Lambda}}$ type atomic system to produce a low frequency weak Stokes field which is a phase conjugate to probe. We show that any arbitrary mode such as Airy, Bessel, Mathieu, and Weber beams encoded initially in the spatial envelope of the probe field are efficiently transferred to the FWM Stokes field by satisfying the phase-matching condition. Interestingly, we found that the transmitted intensity profiles of the Stokes beam are identical to that of the probe beam, while the phase profile is complementary. The phase conjugation property of output beams is revealed by interfering them with a copropagating plane wave. We further found the fidelity in terms of structural similarity between two transmitted modes of about 9999%99, which substantiates the high efficiency of the FWM process. The efficient transfer and frequency conversion of such diffraction-free beams may have potential applications in nonlinear optical and quantum technologies.
Abstract We investigate the nonlinear frequency conversion of non-diffracting optical modes via non-degenerate four-wave mixing(FWM) process in rubidium vapor. In this process, two strong control fields and a weak probe field mutually interact via afour-level double-Λ type atomic system to produce a new frequency weak Stokes field which is a phase conjugate to probe. We show that any arbitrary mode such as Airy, Bessel, Mathieu, and Weber beams encoded initially in the spatial envelope of probe field are efficiently transferred to FWM Stokes field by satisfying the phase matching condition. Interestingly, we found that the transmitted intensity profiles of Stokes beam are identical to that of probe beam while phase profile is complimentary.The phase conjugation property of output beams is revealed by interfering them with a copropagating plane wave. We further found the fidelity in terms of structural similarity between two transmitted modes of about 99%, which substantiates the high efficiency of FWM process. The efficient transfer and frequency conversion of such diffraction-free beams may have potential applications in nonlinear optical and quantum technologies.
We report the transfer of phase structure and, in particular, of orbital angular momentum from near-infrared pump light to blue light generated in a four-wave-mixing process in 85Rb vapor. The intensity and phase profile of the two pump lasers at 780 and 776 nm, shaped by a spatial light modulator, influences the phase and intensity profile of light at 420 nm, which is generated in a subsequent coherent cascade. In particular, we observe that the phase profile associated with orbital angular momentum is transferred entirely from the pump light to the blue. Pumping with more complicated light profiles results in the excitation of spatial modes in the blue that depend strongly on phase matching, thus demonstrating the parametric nature of the mode transfer. These results have implications on the inscription and storage of phase information in atomic gases.
We report the transfer of phase structure, and in particular of orbital angular momentum (OAM), from near-infrared pump light to blue light generated in a four-wave-mixing process in85Rb vapour. The intensity and phase profile of the two pump lasers at 780nm and 776nm, shaped by a spatial light modulator (SLM), influences the phase and intensity profile of light at 420nm which is generated in a subsequent coherent cascade. In particular we observe that the phase profile associated with orbital angular momentum is transferred entirely from the pump light to the blue. Pumping with more complicated light profiles results in the excitation of spatial modes in the blue that depend strongly on phase matching, thus demonstrating the parametric nature of the mode transfer. These results have implications on the inscription and storage of phase information in atomic gases.
Experimental results on the phase transfer from structured beams to parametric light, generated by inducing four-wave mixing in an atomic gas, are reported. Near-infrared, Mathieu, and Gaussian pump beams yield a blue coherent Mathieu electromagnetic field and an infrared beam. Two complementary techniques enable full characterization of the up-converted modes. The unambiguous and efficient phase heritage of these complex quasipropagation invariant modes to up-converted photons is demonstrated. The presented data enable a quantitative study of dynamical variables related to Mathieu beams. These include elliptic angular momentum, a generalization of the orbital angular momentum of light, which is also up-converted through the nonlinear process.