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Physical Review Letters

Subpicosecond Ultracold Electron Source

T. C. H. de Raadt, J. G. H. Franssen, O.J. Luiten

Published May 17, 2023• 15 citations
Publisher

Abstract

We present the first observation of subpicosecond electron bunches from an ultracold electron source. This source is based on near-threshold, two-step, femtosecond photoionization of laser-cooled rubidium gas in a grating magneto-optical trap. Bunch lengths as short as 735±7 fs (rms) have been measured in the self-compression point of the source by means of ponderomotive scattering of the electrons by a 25 fs, 800 nm laser pulse. The observed temporal structure of the electron bunch depends on the central wavelength of the ionization laser pulse, in agreement with detailed simulations of the atomic photoionization process. This shows that the bunch length limit imposed by the atomic photoionization process has been reached.

DOI
10.1103/physrevlett.130.205001

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We present the first observation of subpicosecond electron bunches from an ultracold electron source. This source is based on near-threshold, two-step, femtosecond photoionization of laser-cooled rubidium gas in a grating magneto-optical trap. Bunch lengths as short as 735±7 fs (rms) have been measured in the self-compression point of the source by means of ponderomotive scattering of the electrons by a 25 fs, 800 nm laser pulse. The observed temporal structure of the electron bunch depends on the central wavelength of the ionization laser pulse, in agreement with detailed simulations of the atomic photoionization process. This shows that the bunch length limit imposed by the atomic photoionization process has been reached.
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Electron microscopy and diffraction have long been used to study the structure of materials. A recent development is the achievement of ultrafast time resolution using high-repetition rate single electron sources and single-shot many-electron sources. Achieving large coherence lengths under these conditions is challenging due to intrinsic heating mechanisms including inter-particle Coulombic forces. Near-threshold, pulsed photoionization of atoms trapped and cooled with lasers is being investigated as a means to produce intense electron pulses with large intrinsic coherence length due to a low electron temperature. Photo-ionizaton sources are, of course, not an entirely new idea but recent implementations using trapped atoms offer new possibilities. Several properties of electron beams extracted from such ultracold sources have already been investigated, showing in particular that temperatures of a few Kelvin and emittances in the nanometer-radian range can be achieved with tens of thousands electrons per pulse for nanosecond pulse lengths. This can be combined with delicate shaping of the charge distribution to counteract emittance growth due to non-linear self fields. Using ultrafast lasers for the ionization step, shorter electron pulses can be achieved, but an interesting question is whether the concomitant spread in photon energy still allows for low electron temperature. Recent experiments have shown that few-Kelvin temperatures combined with picosecond pulse lengths are indeed possible. It turns out that this can be understood with a classical model for electron trajectories resulting from photoionization. In addition, experimentally observed polarization effects are in general agreement with model results. --------------------------------------------------------------------------------
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We have implemented an approach to investigate the space charge effect (SCE) in the ultracold ion bunch produced through the near-threshold photoionization of laser-cooled rubidium atoms trapped in a magneto-optical trap. The non-linear broadening of spatial profile of the ultracold ion bunch induced by SCE within the initial density range of 3.7 × 106–4.5 × 107/cm3 was explored using a time-of-flight spectrometer coupled with an imaging detector. A charged particle tracing simulation accounting for all pairwise ion–ion Coulomb interactions and an analytical model calculation, which predicts the dependence of the ion bunch density on time evolution and initial density, reproduced the experimental results successfully, indicating that the study could capture the evolution dynamics of ion bunch dominated by SCE. The aim of this work is to extend the investigation on SCE to extreme low-density regions of the order of 106 /cm3 and is expected to be useful in optimizing the performance of ultracold ion/electron sources.