Pulsed photoionization of laser-cooled atoms in a magneto-optical trap (MOT) has the potential to create cold electron beams of few meV bandwidths and few ps pulse lengths. Such a source would be highly attractive for the study of fast low-energy processes like coherent phonon excitation. To study the suitability of MOT-based sources for the production of simultaneously cold and fast electrons, we study the photoionization dynamics of trapped Cs atoms. A momentum-microscope-like setup with a delay-line detector allows for the simultaneous measurement of spatial and temporal electron distributions. The measured patterns are complex, due to the Lorentz force inducing spiral trajectories. Ray-tracing simulations reproduce the main features. We find that the production of electron bunches with bandwidths of a few meV is straightforward; however, pulses in the ps-range are more demanding and require beam blanking or partial blocking.
Pulsed photoionization of laser-cooled atoms in a magneto-optical trap (MOT) has the potential to create cold electron beams of few meV bandwidths and few ps pulse lengths. Such a source would be highly attractive for the study of fast low-energy processes like coherent phonon excitation. To study the suitability of MOT-based sources for the production of simultaneously cold and fast electrons, we study the photoionization dynamics of trapped Cs atoms. A momentum-microscope-like setup with a delay-line detector allows for the simultaneous measurement of spatial and temporal electron distributions. The measured patterns are complex, due to the Lorentz force inducing spiral trajectories. Ray-tracing simulations reproduce the main features. We find that the production of electron bunches with bandwidths of a few meV is straightforward; however, pulses in the ps-range are more demanding and require beam blanking or partial blocking.
This thesis presents details of a new type of cold atom electron source (CAES) that uses an alternating current magneto-optical trap (AC-MOT). Cold atom electron sources produce electron bunches by threshold photoionisation from a population of laser-cooled atoms. The electrons extracted from the atoms are made into a beam which has an ultra-low transverse velocity distribution. The low velocity distribution increases the brightness and reduces the energy spread of the beam, making CAESs potential sources for future electron diffraction and electron spectroscopy studies.
The newly commissioned source detailed here produces focused electron bunches with characteristic temperatures as low as 12.6 ± 0.8 K, at a rate of up to 10 Hz, and with a bunch charge of 2.2±0.2fC, comparable to other state-of-the-art cold atom electron sources. The AC-MOT CAES can also produce cold bunches with energies <200 eV, which is lower than has previously been reported for this type of source.
The electrons originate from a population of laser-cooled 85Rb atoms held in an AC- MOT. The AC-MOT CAES design allows the magnetic trapping fields to be switched to zero in 32 μs, more than ��175 times faster than is possible using a comparable DC-MOT source. This means that electron bunches can be created and extracted in a magnetic field-free environment without any reduction in trap density and hence bunch charge, as occurs in conventional DC-MOT sources.
The design, development, characterisation, and operation of the systems needed for the new AC-MOT CAES are detailed in this thesis. This includes details of the atom trapping system, the photoionisation system, the electron extraction system and the various timing systems for creation and characterisation of the resultant cold electron bunches.
Finally, the characterisation of the AC-MOT CAES itself is presented, and the measured beam metrics are used to compare the new AC-MOT CAES with other CAES designs which are under development.
Electron microscopy and diffraction have long been used to study the structure of materials. A recent development is the achievement of ultrafast time resolution using high-repetition rate single electron sources and single-shot many-electron sources. Achieving large coherence lengths under these conditions is challenging due to intrinsic heating mechanisms including inter-particle Coulombic forces. Near-threshold, pulsed photoionization of atoms trapped and cooled with lasers is being investigated as a means to produce intense electron pulses with large intrinsic coherence length due to a low electron temperature. Photo-ionizaton sources are, of course, not an entirely new idea but recent implementations using trapped atoms offer new possibilities. Several properties of electron beams extracted from such ultracold sources have already been investigated, showing in particular that temperatures of a few Kelvin and emittances in the nanometer-radian range can be achieved with tens of thousands electrons per pulse for nanosecond pulse lengths. This can be combined with delicate shaping of the charge distribution to counteract emittance growth due to non-linear self fields. Using ultrafast lasers for the ionization step, shorter electron pulses can be achieved, but an interesting question is whether the concomitant spread in photon energy still allows for low electron temperature. Recent experiments have shown that few-Kelvin temperatures combined with picosecond pulse lengths are indeed possible. It turns out that this can be understood with a classical model for electron trajectories resulting from photoionization. In addition, experimentally observed polarization effects are in general agreement with model results. --------------------------------------------------------------------------------
We developed a magneto-optical trap reaction microscope (MOTREMI) for strontium atoms by combining multiparticle coincident detection with the laser cooling technique. The present compact injection system enables the production of cold Sr atoms in three modes of two-dimensional (2D) magneto-optical trap (MOT) beam, molasses, and three-dimensional (3D) MOT, providing adjustable densities and ratios of the ground state 5s2 (1S0) and the excited states 5s5p1P1 and 3PJ. The target profiles including temperature, density, and size of the 3D MOT as well as the 2D MOT beam cold atomic flux were characterized in detail. Using the present setup, we investigate the single photoionization of Sr atoms with molasses through few-photons absorption in 800 nm, where Sr+ and ${e}^{\ensuremath{-}}$ are detected in coincidence and most of the ionization channels are identified. The momentum resolution for coincident Sr+ and ${e}^{\ensuremath{-}}$ along time-of-flight direction are achieved up to 0.12 a.u. and 0.02 a.u., respectively. The spectra of photoelectron ionized from the ground state as well as several excited states show distinct structures manifesting prominent contributions from multiphoton absorption. Detecting complete vector momenta of electrons and recoil ions in coincidence paves a way for further investigation of two-electron correlation dynamics and multielectron effects with alkaline-earth atoms.
In a Magneto-Optical Trap (MOT), realized for the first time in 1987, one can trap and cool neutral atoms to temperatures below a mK. The invention of this device caused a revolution in atomic physics. With an MOT collision and spectroscopy experiments could be performed with unprecedented accuracy. The main breakthrough came about 10 years later when the atom from an MOT were used to create a Bose Einstein Condensate (BEC), a source of coherent matter. All this work has been rewarded with no less than two Nobel prizes: in 1997, Chu, Cohen-Tannoudji and Phillips received the Nobel prize for the practical and theoretical development of laser cooling, and in 2001 Cornell, Ketterle and Wieman received the Nobel prize for the realization of a Bose Einstein Condensate in a dilute gas. In 1999 Killian et al. took trapped atoms in an entirely new direction when they succeeded in creating the very first Ultracold Plasma (UCP) from the atoms in an MOT. The temperature of such a plasma is more than 1000 times lower than the temperatures in conventional cold plasmas. As a result, this type of plasmas received a lot of attention, both theoretically and experimentally. So far studies of UCPs have mainly been of a fundamental kind. In this thesis we study both the fundamental aspects of atoms excited from a magneto-optical as well as the feasibility of using the electrons and ions from a UCP as a source for charged particle accelerators. The work in this thesis therefore pioneers the line between atom physics, plasma physics and accelerator physics. The first part of this thesis deals with an experimental study of the effect of an ionizing laser on cold neon atoms. Here we study the loss of atoms from a Magneto-Optical Trap caused by photionization. From these measurements we deduce a new value for the near threshold photoionization cross section 2:05±0:25x10-18 cm2 at ¿ = 351 nm and 2:05±0:25x10-18 cm2 at ¿ = 364 nm, which is a factor of four more accurate than previous measurements. The measured valuesagree with earlier measurements but differ signi¯cantly from theoretical values. The value of this cross section has a practical relevance for the realization of a continuous ion source. The second part of this thesis has been conducted at the University of Virginia. We study the role of dipole-dipole interactions in the formation of a UCP from a gas of cold Rydberg atoms, and the effect of dipole-dipole interactions on the broadening of microwave transitions. We find that the broadening scales linearly with the density en scales with the fourth power of n, the principal quantum number. These results show the great importance of dipole-dipole interactions in gas of cold Rydberg atoms and are also relevant for the possible realization of a quantum computer from Rydberg atoms. In a third part we studied the potential of using a UCP as a source for electron accelerators. This was done based upon elaborate simulations performed with the General Particle Tracer Code. The main result of these simulations is that, based upon realistic parameters, the brightness, i.e., the figure of merit for charged particle sources defined as the current divided by the emittance squared, of such a source can be up to two orders of magnitude larger than the brightness of conventional sources, which is a major advance. The emittance is a measure for the the focusability of the bunch, and scales as p T, with T the electron temperature. The increase in brightness is mainly attributed to the low electron temperatures of approximately 10 K in an UCP, resulting in an initial emittance of 0.01 mm mrad, compared to 1 mm mrad in a conventional source. With experimentally proven techniques it is possible to extract 10 nC/s from the source, which is a competitive repetition rate. In the next part we describe the design, construction and testing of the first setup with which we want to build an electron accelerator based upon cold atoms. For this we first built a vapor-cell magneto-optical trap, in which we can trap over 109 rubidium atoms with a temperature of 200 ¹K, straight from a background vapor, we also designed an atomic beam that will be implemented in the near future and can provide an increased repetition rate. In the last chapter we show how Rydberg atoms excited from an MOT, evolve into an UCP spontaneously. We extracted a minimum of 1 pC from the plasma. As a main result, we were one of the ¯rst to show how the ions and electrons from a UCP can be imaged on a phosphor screen. From these images we can deduct an upper value for the electron and the ion temperature, we extract for both the electrons and the ions an upper temperature of 40 K, when we translate this temperature to an initial emittance, we obtain a value of 0.01 mm mrad, proving the potential of the electrons extracted from atoms excited out of an MOT as a low emittance source. Our measured current of 1 ¹A is not yet competitive and results from the small electric field, but is expected to increase dramatically in the near future. We will implement a 30 kV 10 ns risetime accelerator with which it should be possible to get a current of about 50 mA. Furthermore we will implement the proper diagnostics to measure the proper charge, current and emittance. In the very last chapter we speculate charged particle sources from cold atoms might advance the state of the art in achievable brightness for both electron and ion beams.
The newly developed method of time-of-flight (TOF) momentum microscopy was used to analyze the cold electron emission from a Cs three-dimensional magneto-optical trap (MOT). Three-step resonant photoionization was implemented via two intermediate states (6P3/2 pumped with an 852-nm laser and 7S1/2 with a 1470-nm laser) and a tunable femtosecond (fs) Ti:sapphire laser for the final ionization step. The magnetic field of the MOT is switched off during the photoionization step. The natural bandwidth of the fs laser is reduced to 4 meV using optical spectral filters. Precise tuning of the photon energy makes it possible to observe the transition regime between direct photoemission into the open continuum and field-induced ionization of highly excited Rydberg states. The paths can be identified by their characteristic dependency on the extraction field and on the Ti:sapphire polarization. TOF analysis allowed us to disentangle the ionization paths and the dependence of the spatiotemporal distribution of the cold electrons on the polarization of the ionizing laser.
Laser-cooled gases offer an alternative to tip-based methods for generating high-brightness ion beams for focused ion beam applications. These sources produce ions by photoionization of ultracold neutral atoms, where the narrow velocity distribution associated with microkelvin-level temperatures results in a very low emittance, high-brightness ion beam. In a magneto-optical trap-based ion source, the brightness is ultimately limited by the transport of cold neutral atoms, which restricts the current that can be extracted from the ion-generating volume. We explore the dynamics of this transport in a 7Li magneto-optical trap ion source by performing time-dependent measurements of the depletion and refilling of the ionization volume in a pulsed source. An analytic microscopic model for the transport is developed, and this model shows excellent agreement with the measured results.