In a Magneto-Optical Trap (MOT), realized for the first time in 1987, one can trap and cool neutral atoms to temperatures below a mK. The invention of this device caused a revolution in atomic physics. With an MOT collision and spectroscopy experiments could be performed with unprecedented accuracy. The main breakthrough came about 10 years later when the atom from an MOT were used to create a Bose Einstein Condensate (BEC), a source of coherent matter. All this work has been rewarded with no less than two Nobel prizes: in 1997, Chu, Cohen-Tannoudji and Phillips received the Nobel prize for the practical and theoretical development of laser cooling, and in 2001 Cornell, Ketterle and Wieman received the Nobel prize for the realization of a Bose Einstein Condensate in a dilute gas. In 1999 Killian et al. took trapped atoms in an entirely new direction when they succeeded in creating the very first Ultracold Plasma (UCP) from the atoms in an MOT. The temperature of such a plasma is more than 1000 times lower than the temperatures in conventional cold plasmas. As a result, this type of plasmas received a lot of attention, both theoretically and experimentally. So far studies of UCPs have mainly been of a fundamental kind. In this thesis we study both the fundamental aspects of atoms excited from a magneto-optical as well as the feasibility of using the electrons and ions from a UCP as a source for charged particle accelerators. The work in this thesis therefore pioneers the line between atom physics, plasma physics and accelerator physics. The first part of this thesis deals with an experimental study of the effect of an ionizing laser on cold neon atoms. Here we study the loss of atoms from a Magneto-Optical Trap caused by photionization. From these measurements we deduce a new value for the near threshold photoionization cross section 2:05±0:25x10-18 cm2 at ¿ = 351 nm and 2:05±0:25x10-18 cm2 at ¿ = 364 nm, which is a factor of four more accurate than previous measurements. The measured valuesagree with earlier measurements but differ signi¯cantly from theoretical values. The value of this cross section has a practical relevance for the realization of a continuous ion source. The second part of this thesis has been conducted at the University of Virginia. We study the role of dipole-dipole interactions in the formation of a UCP from a gas of cold Rydberg atoms, and the effect of dipole-dipole interactions on the broadening of microwave transitions. We find that the broadening scales linearly with the density en scales with the fourth power of n, the principal quantum number. These results show the great importance of dipole-dipole interactions in gas of cold Rydberg atoms and are also relevant for the possible realization of a quantum computer from Rydberg atoms. In a third part we studied the potential of using a UCP as a source for electron accelerators. This was done based upon elaborate simulations performed with the General Particle Tracer Code. The main result of these simulations is that, based upon realistic parameters, the brightness, i.e., the figure of merit for charged particle sources defined as the current divided by the emittance squared, of such a source can be up to two orders of magnitude larger than the brightness of conventional sources, which is a major advance. The emittance is a measure for the the focusability of the bunch, and scales as p T, with T the electron temperature. The increase in brightness is mainly attributed to the low electron temperatures of approximately 10 K in an UCP, resulting in an initial emittance of 0.01 mm mrad, compared to 1 mm mrad in a conventional source. With experimentally proven techniques it is possible to extract 10 nC/s from the source, which is a competitive repetition rate. In the next part we describe the design, construction and testing of the first setup with which we want to build an electron accelerator based upon cold atoms. For this we first built a vapor-cell magneto-optical trap, in which we can trap over 109 rubidium atoms with a temperature of 200 ¹K, straight from a background vapor, we also designed an atomic beam that will be implemented in the near future and can provide an increased repetition rate. In the last chapter we show how Rydberg atoms excited from an MOT, evolve into an UCP spontaneously. We extracted a minimum of 1 pC from the plasma. As a main result, we were one of the ¯rst to show how the ions and electrons from a UCP can be imaged on a phosphor screen. From these images we can deduct an upper value for the electron and the ion temperature, we extract for both the electrons and the ions an upper temperature of 40 K, when we translate this temperature to an initial emittance, we obtain a value of 0.01 mm mrad, proving the potential of the electrons extracted from atoms excited out of an MOT as a low emittance source. Our measured current of 1 ¹A is not yet competitive and results from the small electric field, but is expected to increase dramatically in the near future. We will implement a 30 kV 10 ns risetime accelerator with which it should be possible to get a current of about 50 mA. Furthermore we will implement the proper diagnostics to measure the proper charge, current and emittance. In the very last chapter we speculate charged particle sources from cold atoms might advance the state of the art in achievable brightness for both electron and ion beams.
In a Magneto-Optical Trap (MOT), realized for the first time in 1987, one can trap and cool neutral atoms to temperatures below a mK. The invention of this device caused a revolution in atomic physics. With an MOT collision and spectroscopy experiments could be performed with unprecedented accuracy. The main breakthrough came about 10 years later when the atom from an MOT were used to create a Bose Einstein Condensate (BEC), a source of coherent matter. All this work has been rewarded with no less than two Nobel prizes: in 1997, Chu, Cohen-Tannoudji and Phillips received the Nobel prize for the practical and theoretical development of laser cooling, and in 2001 Cornell, Ketterle and Wieman received the Nobel prize for the realization of a Bose Einstein Condensate in a dilute gas. In 1999 Killian et al. took trapped atoms in an entirely new direction when they succeeded in creating the very first Ultracold Plasma (UCP) from the atoms in an MOT. The temperature of such a plasma is more than 1000 times lower than the temperatures in conventional cold plasmas. As a result, this type of plasmas received a lot of attention, both theoretically and experimentally. So far studies of UCPs have mainly been of a fundamental kind. In this thesis we study both the fundamental aspects of atoms excited from a magneto-optical as well as the feasibility of using the electrons and ions from a UCP as a source for charged particle accelerators. The work in this thesis therefore pioneers the line between atom physics, plasma physics and accelerator physics. The first part of this thesis deals with an experimental study of the effect of an ionizing laser on cold neon atoms. Here we study the loss of atoms from a Magneto-Optical Trap caused by photionization. From these measurements we deduce a new value for the near threshold photoionization cross section 2:05±0:25x10-18 cm2 at ¿ = 351 nm and 2:05±0:25x10-18 cm2 at ¿ = 364 nm, which is a factor of four more accurate than previous measurements. The measured valuesagree with earlier measurements but differ signi¯cantly from theoretical values. The value of this cross section has a practical relevance for the realization of a continuous ion source. The second part of this thesis has been conducted at the University of Virginia. We study the role of dipole-dipole interactions in the formation of a UCP from a gas of cold Rydberg atoms, and the effect of dipole-dipole interactions on the broadening of microwave transitions. We find that the broadening scales linearly with the density en scales with the fourth power of n, the principal quantum number. These results show the great importance of dipole-dipole interactions in gas of cold Rydberg atoms and are also relevant for the possible realization of a quantum computer from Rydberg atoms. In a third part we studied the potential of using a UCP as a source for electron accelerators. This was done based upon elaborate simulations performed with the General Particle Tracer Code. The main result of these simulations is that, based upon realistic parameters, the brightness, i.e., the figure of merit for charged particle sources defined as the current divided by the emittance squared, of such a source can be up to two orders of magnitude larger than the brightness of conventional sources, which is a major advance. The emittance is a measure for the the focusability of the bunch, and scales as p T, with T the electron temperature. The increase in brightness is mainly attributed to the low electron temperatures of approximately 10 K in an UCP, resulting in an initial emittance of 0.01 mm mrad, compared to 1 mm mrad in a conventional source. With experimentally proven techniques it is possible to extract 10 nC/s from the source, which is a competitive repetition rate. In the next part we describe the design, construction and testing of the first setup with which we want to build an electron accelerator based upon cold atoms. For this we first built a vapor-cell magneto-optical trap, in which we can trap over 109 rubidium atoms with a temperature of 200 ¹K, straight from a background vapor, we also designed an atomic beam that will be implemented in the near future and can provide an increased repetition rate. In the last chapter we show how Rydberg atoms excited from an MOT, evolve into an UCP spontaneously. We extracted a minimum of 1 pC from the plasma. As a main result, we were one of the ¯rst to show how the ions and electrons from a UCP can be imaged on a phosphor screen. From these images we can deduct an upper value for the electron and the ion temperature, we extract for both the electrons and the ions an upper temperature of 40 K, when we translate this temperature to an initial emittance, we obtain a value of 0.01 mm mrad, proving the potential of the electrons extracted from atoms excited out of an MOT as a low emittance source. Our measured current of 1 ¹A is not yet competitive and results from the small electric field, but is expected to increase dramatically in the near future. We will implement a 30 kV 10 ns risetime accelerator with which it should be possible to get a current of about 50 mA. Furthermore we will implement the proper diagnostics to measure the proper charge, current and emittance. In the very last chapter we speculate charged particle sources from cold atoms might advance the state of the art in achievable brightness for both electron and ion beams.
Collisions between ultracold neutral atoms have for some time been the subject of investigation, initially with hydrogen and more recently with laser cooled alkali atoms. Advances in laser cooling and trapping of neutral atoms in a Magneto-Optic Trap (MOT) have made cold atoms available as the starting point for many laser cooled atomic physics investigations. The most spectacularly successful of these, the observation of Bose-Einstein Condensation (BEC) in a dilute ultra-cold spin polarized atomic vapor, has accelerated the study of cold collisions. Experimental and theoretical studies of BEC and the long range interaction between cold alkali atoms is at the boundary of atomic and low temperature physics. Such studies have been difficult and would not have been possible without the development and advancement of laser cooling and trapping of neutral atoms. By contrast, ion-atom interactions at low temperature, also very difficult to study prior to modern day laser cooling, have remained largely unexplored. But now, many laboratories worldwide have almost routine access to cold neutral atoms. The combined technologies of ion trapping, together with laser cooling of neutrals has made these studies experimentally feasible and several very important, novel applications might come out of such investigations . This paper is an investigation of ion-atom interactions in the cold and ultra-cold temperature regime. Some of the collisional ion-atom interactions present at room temperature are very much reduced in the low temperature regime. Reaction rates for charge transfer between unlike atoms, A + B(+) approaches A(+) + B, are expected to fall rapidly with temperature, approximately as T(sup 5/2). Thus, cold mixtures of atoms and ions are expected to coexist for very long times, unlike room temperature mixtures of the same ion-atom combination. Thus, it seems feasible to cool ions via collisions with laser cooled atoms. Many of the conventional collisional interactions, exploited as a useful tool at room temperature and higher, are greatly enhanced at low energy. For example, collisional spin transfer from one species of polarized atoms to another has long been a useful method for polarizing a sample of atoms where no other means was available. Because optical pumping cannot be used to polarize the nuclear spin of Xe-129 or He-3 (for use in nmr imaging of the lungs), the nuclear spins are polarized via collisions with an optically pumped Rb vapor in a cell containing both gases. In another case, a spin polarized thermal Cs beam was used to polarize the hyperfine states of trapped He(+)-3 ions in order to measure their hyperfine clock transition frequency. The absence of an x-ray light source to optically pump the ground state of the He(+)-3 ion necessitated this alternative state preparation. Similarly, Cd(+) and Sr(+) ions were spin-oriented via collisions in a cell with optically pumped Rb vapor. Resonant RF spin changing transitions in the ground state of the ions were detected by changes in the Rb resonance light absorption. Because cold collision spin exchange rates scale with temperature as T(sup -1/2) this technique is expected to be a far more powerful tool than the room temperature counterpart. This factor of 100 or more enhancement in spin exchange reaction rates at low temperatures is the basis for a novel trapped ion clock where laser cooled neutrals will cool, state select and monitor the ion clock transition. The advantage over conventional direct laser cooling of trapped ions is that the very expensive and cumbersome UV laser light sources, required to excite the ionic cooling transition, are effectively replaced by simple diode lasers.
Ultracold plasmas (UCPs) represent a marriage between the seemingly distinct fields of cold atom physics and plasma physics. In cold atom physics, dilute clouds of atoms can be trapped with laser radiation and cooled to J.1Ktemperatures. In contrast, in plasma physics the constituents generally have temperatures in the 1,000K-1O,000K range as well as much higher density. In 1999,Rolston and co-workers [1] first converted a cloud of laser-cooled atoms into a plasma by photo-ionizing the atoms just above threshold. This provides very unusual circumstances:the temperature of ions and neutrals is O.OOIK,that of electrons 10K! Such ultra-cold plasmas therefore are interesting subjects for fundamentalplasma physics studies.\nIn a recent paper [2], we argued that ultracold plasmas (UCPs) may in addition provide an entirely new way of generatinghigh-brightnesscharged-particlebeams, such as used in focused-ion beams, laser synchrotrons, and ultra-fast electron microscopy.\nHere, a low temperature T is beneficial for the intrinsic (transverse) brightness B of a\nsource since B = II(A1), where I is the current and A the cross-sectional area. I will discuss an experimental investigation of the properties of ion and electron beams extracted from ultracold plasmas, which shows that such beams indeed have low temperatures, and, as a result, high angular intensity.
The development of atom trapping and cooling techniques has been a boon for the field of low temperature plasma physics. By forming plasmas through photoionization (PI) of cold atoms, researchers are able to create cold, dense plasmas that often lie in the strong-coupling regime. This is especially remarkable considering that many naturally-occurring plasmas in the strong-coupling regime are in inaccessible environments (e.g. the insides of stars and gas planets), whereas these laboratory-based plasmas prepared in cold-atom systems are relatively easy to produce and analyze with standard AMO techniques. In this thesis, I present my work from several projects on photoionization, plasma formation and dynamics, and plasma trap development. I first discuss an experiment that I spearheaded on expansion dynamics in cold, non-neutral plasmas. In this experiment, cold plasmas are formed by photoionizing rubidium atoms in a MOT, and the resulting plasma ions are allowed to expand for a variable wait time before being imaged with a single-ion imaging system. This ion imaging system, along with the rest of the experimental setup, was originally used to study Rydberg atoms. I have adapted the setup for plasmas by installing a new laser and changing the experimental timings. I report on plasma features seen in this experimental setup, such as shock shells and time-evolved ion pair correlations. I also present findings from a computational study of wavelength-dependent PI of Rydberg atoms, namely Rydberg-state rubidium and cesium. The main goal of the study is to find PI minima, wavelengths where the atom’s PI cross section decreases dramatically. These minima can be caused by Cooper minima or shape resonances, which each have their own telltale signs. This computational study paves the way for an informed experimental measurement of the locations of some of the identified PI minima, and comparing their experimental locations with the computational results. This is, in part, interesting because the latter depend on whether length or velocity gauge is used. An experimental measurement of PI cross sections could be a good way to explore the significance of gauge dependence in l-dependent potentials. I conclude with a discussion of a project centered on creating a small MOT with diverging cooling beams inside of a metal enclosure. This project was a collaboration with researchers at Eastern Michigan University. The idea to make a MOT with these design features was born out of plans for cryostatic plasma experiments. Now, it has potential applications in plasma experiments, precision measurements, and quantum information. Design-wise, the diverging beams are formed by sending narrow laser beams into 1.5 mm ball lenses, which cause the beams to diverge rapidly. Six ball lenses, one for each cooling beam, are mounted on a metal structure called the ball lens optical box (BLOB), which encases the trapped atom cloud. This enclosure provides immediate benefits for plasma experiments, as it offers Faraday shielding from stray electric fields. The first build successfully produced and maintained a MOT, making it the first known case of a MOT made with diverging beams from ball lenses. No further experiments are planned for this first build, but the concept of a ball lens MOT will certainly be implemented into future experimental efforts. Subsequent designs may include more design features, such as interior electrodes for custom field configurations.
In 1925, Einstein predicted the condensation of bosons into the ground state of the system for low (but finite) temperatures. Several phenomena, including superfluidity and superconductivity have been associated with Bose-Einstein condensation, but these systems interact strongly with their environment and pure Bose-Einstein condensation could not be established. It took 70 years, in which time the laser was discovered, and laser cooling techniques to manipulate atoms in a dilute atomic gas, before Bose-Einstein condensation in dilute atomic gases could be demonstrated in 1995. In the first condensation experiments, BECs were created in a magnetic trap. Since in a magnetic trap not all mF states of the atom can be trapped simultaneously, thereby limiting the number of experiments that can be done, other ways of trapping and generating BECs were sought and found. In 2001, the first all-optical BEC was made, where the dipole force was used to trap atoms in the crossing of two far red detuned laser beams. In an optical dipole trap not only atoms in different internal states can be trapped, but also different atomic species simultaneously. In this thesis, the formation of an all-optical Bose-Einstein condensate with rubidium atoms is presented. Conventional all-optical BECs are usually created in high power CO2 laser dipole traps, or have complicated laser cooling schemes and complex dipole trap setups. In our simple and straightforward setup, we load rubidium atoms from a magneto-optical trap into a crossed optical dipole trap created by a single frequency Yb:YAG laser with a wavelength at 1030 nm. The small wavelength allows for a small diffraction limit, and permits us to use standard optical materials, thus making the experimental setup cost effective. Other attempts to achieve Bose-Einstein condensation in a multi-mode (frequency) fiber laser at 1064 nm failed, because the atom loss was quite high. It is assumed that the multi-mode character of the fiber laser induces Raman transitions in rubidium atoms, thereby heating them. We can trap about ∼ 5E7 atoms in a single beam dipole trap out of ∼ 5E9 atoms trapped in theMOT, and ∼ 350,000 atoms can be trapped in a crossed beam dipole trap due to the smaller trap volume. 70% of the atoms in the dipole trap is optically pumped into one mF state. Quantum degeneracy is reached by evaporatively cooling the atoms in the crossed dipole trap by ramping down the laser power with three linear ramps. We can independently change the power of each beam by an AOM. This allows us to use one beam as an atom waveguide for future experiments. After evaporation, we typically have about 10,000 atoms at a temperature below the critical temperature. We have proved Bose-Einstein condensation by using the anisotropic expansion of a quantum degenerate gas trapped in an anisotropic potential. The aspect ratio of our atom cloud changed during a time of flight from 0.7 to 1.2 in 10 ms, thus proving that we have reached quantum degeneracy. We have about 5,000 condensed atoms in our optical dipole trap at a temperature less than 100 nK. The remaining atoms are thermal. Bose-Einstein condensation is obtained within 8 s, and we can repeat the experiment every 30 s. It should be mentioned that the Bose-Einstein experiment was moved from the ”Leibniz Universität Hannover” to the ”Technische Universität Darmstadt”, and had to be completely rebuilt. All-optical Bose-Einstein condensation was reached within one year after the move. Our Bose-Einstein condensation setup presents an ideal starting point for using our condensates in combination with miniaturized atom optical setups based on our novel microfabricated optical elements. With our microlenses, we can create a number of possible dipole trap configurations, such as the dipole trap array or the cylindrical microlens array. Using microlenses in miniaturized atom optical setups opens a completely new field of coherent atom optics. Also because the tight confinement of the microtraps allows us to load a 3D BEC, a 1D BEC, or a Tonks-Girardeau gas in the micropotentials depending on the density.
The recent development of laser cooling and trapping techniques has made possible the controlled realization of dense and cold atomic samples, thus opening the way for spectroscopic investigations in the low and ultra-low temperature regimes not accessible with conventional techniques. In our lab, an apparatus for laser cooling and Bose-Einstein condensation of rubidium atoms is in operation, producing a sample large enough to perform reliable investigations by absorption or emission techniques. Moving from previous photoionization experiments of laser-cooled atoms in a magneto-optical trap irradiated by cw-laser radiation [1] and stimulated by the interest grown recently on ultra-cold plasma [2], we have started a series of experiments aimed at investigating the interaction of intense laser pulses with the ultra-cold neutral sample, boty aboeand below the condensation temperature. Radiation from an excimer-pumped dye laser was used at a wavelength close to 594 nm, corresponding to the ionization threshold of rubidium for two photon non-resonant absorption from the ground state, with intensities in the tens of MW/cm^2 range and a pulse duration of 16 ns. Preliminary results, attained through the dynamical analysis (atom number, temperature) of the cold atom sample after the arrival of the laser pulse, suggest the occurrence of different processes, initiated by multi-photon ionization, involving collisions between cold electrons and ultra-cold neutrals, recombination at low temperatures and collective processes in the weak and cold plasma. Interpretation of those results demonstrates that this class of experiments, based on a variety of topics typical of atomic, plasma and statistical physics, can open the way for novel and intriguing investigations of laser-matter interaction. Further experimental developments will include duplication of the laser pulse frequency and one photon ionization of ground state rubidium laser-cooled atoms. [1] O. Maragò et al., Phys. Rev. A 57 R4110 (1998); E., Arimondo et al., Appl. Surf. Sci. 154-155 527 (2000); F. Fuso et al., Opt. Commun. 173 223 (2000). [2] T.C. Killian et al., Phys. Rev. Lett. 83 4776 (1999); S. Kulin et al., Phys. Rev. Lett. 85 318 (2000).
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.