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Review of Scientific Instruments

A new magnetic state selection method in high-performance optically detected compact cesium beam clocks

Sifei Chen, Chen Liu, Lifeng Fan, Chaojie Li, Yuanhao Li, Chang Liu, Yanhui Wang

Published Apr 1, 2023• 5 citations
Publisher

Abstract

We perform a new scheme of magnetic state selection in optically detected compact cesium beam clocks. Unlike the conventional method, we select atoms in the ground state |F = 4, mF ≠ -4⟩ by pointing the atomic collimator to the convex pole of the magnet realizing the two-wire magnetic field and detect atoms in |F = 3⟩ after interacting with the microwave field using a distributed feedback laser. The fluorescence background is greatly reduced as the inherent residual atoms |F = 4, mF = -4⟩ are avoided in this reversed scheme. The velocity distribution is narrowed, and the most probable velocity is decreased, since atomic trajectories are close to the weak-field region. We also investigate the relationship between the position of the atomic collimator and the distributions of the atomic beam, which is consistent with the Monte Carlo-based simulation model. By applying the reversed scheme and setting the deviated position of the collimator to 1.3 mm, the signal contrast is improved from 0.7 to 3, and the short-term frequency stability reaches 3.0 × 10-12 τ-1/2, nearly three times better than that of the high-performance version of Microsemi 5071A.

DOI
10.1063/5.0147451

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We perform a new scheme of magnetic state selection in optically detected compact cesium beam clocks. Unlike the conventional method, we select atoms in the ground state |F = 4, mF ≠ -4⟩ by pointing the atomic collimator to the convex pole of the magnet realizing the two-wire magnetic field and detect atoms in |F = 3⟩ after interacting with the microwave field using a distributed feedback laser. The fluorescence background is greatly reduced as the inherent residual atoms |F = 4, mF = -4⟩ are avoided in this reversed scheme. The velocity distribution is narrowed, and the most probable velocity is decreased, since atomic trajectories are close to the weak-field region. We also investigate the relationship between the position of the atomic collimator and the distributions of the atomic beam, which is consistent with the Monte Carlo-based simulation model. By applying the reversed scheme and setting the deviated position of the collimator to 1.3 mm, the signal contrast is improved from 0.7 to 3, and the short-term frequency stability reaches 3.0 × 10-12 τ-1/2, nearly three times better than that of the high-performance version of Microsemi 5071A.
We propose and realize a new optical state selection method on a cesium atomic fountain clock by applying a two-laser 3–3′ optical pumping configuration to spin polarize atoms. The atoms are prepared in |F = 3, mF = 0〉 clock state with optical pumping directly after being launched up, followed by a pushing beam to push away the atoms remaining in the |F = 4〉 state. With a state selection efficiency exceeding 92%, this optical method can substitute the traditional microwave state selection, and helps to develop a more compact physical package. A Ramsey fringe has been achieved with this optical state selection method, and a contrast of 90% is obtained with a full width half maximum of 0.92 Hz. The short-term frequency stability of 6.8 × 10−14 (τ/s)−1/2 is acquired. In addition, the number of detected atoms is increased by a factor of 1.7 with the optical state selection.
Light detection is widely used in atomic clocks. The simple detecting structure induces the light shift which influences the clock's long-term stability. We introduce a new method to suppress light shift by using pulsed light instead of continuous light to detect atomic states. Under a suitable pulsed sequence, the part of the atoms which do not simultaneously interact with light and microwave field are detected. We demonstrate the validity of our approach in a magnetic-state-selected cesium beam clock. Using a well-tuned sequence, the light shift coefficient is reduced by a factor of about 10, in comparison with the continuous light detection scheme. In a clock stability test with extra light power noise, the result shows good immunity of the method to laser power fluctuations. We also analyze the sources of the clock short-term stability degradation, including the Dick effect and the fact that a reduced number of atoms is detected in the pulsed detection case.
To improve the signal to noise ratio (SNR) and the short-term stability of cesium atomic fountain clocks, the work of two-laser optical pumping is presented theoretically and experimentally. The short-term stability of the NIM6 fountain clock has been improved by preparing more cold atoms in the | F = 4, mF = 0〉 clock state with a shortened cycle time. Two π-polarized laser beams overlapped in the horizontal plane have been applied after launching, one is resonant with | F = 4〉 → | F′ = 4〉 transition and the other is resonant with | F = 3〉 → | F′ = 4〉 transition. With optical pumping, the population accumulated in the | mF = 0〉 clock state is improved from 11% to 63%, and the detection signal is increased by a factor of 4.2, the SNR of the clock transition probability and the short-term stability are also improved accordingly.
The realisation of cold and slow atomic beams has opened the way to a series of precision measurements of high scientific interest, as atom interferometry, Bose-Einstein Condensation and atomic fountain clocks. The latter are used since several years as reference clocks, given the high performance that they can reach both in accuracy and stability. The common philosophy in the construction of atomic fountains has been the pulsed technique, where an atoms sample is launched vertically and then falls down under the effect of the gravity. The Observatoire de Neuchâtel had a different approach and has built a fountain clock (FOCS1) operating in a continuous mode. This technique offers two main advantages: the diminution of the undesirable effects due to the atomic density (e.g. collisions between the atoms and cavity pulling) and to the noise of the local oscillator (intermodulation effect). To take full advantage of the continuous fountain approach however, we need to increase the atomic flux. The techniques chosen to reach this goal are an efficient transverse collimation together with more atoms to begin with. Here we report on a study of different transverse collimation techniques performed in a two-dimensional phase stable optical lattice (namely gray molasses and magnetically induced laser cooling) as well as the development and characterisation of a 2D-magneto-optical trap used to load the fountain. Best performances are reached in a 2D+-MOT configuration of such a pre-source, for which we detect an atomic flux 20 times greater than the one measured when the fountain is loaded by a Cs vapour. This gain could improve the atomic clock stability by a factor 6. An even better stability is expected after introducing a pre-cooling stage before performing the transverse collimation. This new configuration is currently under investigation and will be implemented in a second continuous fountain (FOCS2).
Herein, we report the scheme of an optically pumped atomic clock based on a cold cesium atomic beam source. We propose the laser system and physical mechanism of this atomic clock, wherein the atomic beam travels in an upper parabolic trajectory, thereby eliminating the light shift effect. In the experiments, when the length of the free evolution region was 167 mm, the line width of the Ramsey fringe was 37 Hz. When the expected signal-to-noise ratio of the Ramsey fringe that can be achieved is 36,000, the expected short-term frequency stability is about 3.6 × 10–14/√τ, which is significantly higher than that of a conventional optically pumped cesium clock of similar volume.