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New Journal of Physics

Floquet engineering with quantum optimal control theory

Alberto Castro, Umberto De Giovannini, Shunsuke A. Sato, Hannes Hübener, Ángel Rubio

Published Apr 1, 2023• 19 citations
Publisher

Abstract

Abstract Floquet engineering consists in the modification of physical systems by the application of periodic time-dependent perturbations. The search for the shape of the periodic perturbation that best modifies the properties of a system in order to achieve some predefined metastable target behavior can be formulated as an optimal control problem. We discuss several ways to formulate and solve this problem. We present, as examples, some applications in the context of material science, although the methods discussed here are valid for any quantum system (from molecules and nanostructures to extended periodic and non periodic quantum materials). In particular, we show how one can achieve the manipulation of the Floquet pseudo-bandstructure of a transition metal dichalcogenide monolayer (MoS2).

DOI
10.1088/1367-2630/accb05

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•Jan 1, 2019•0 citations
Abstract Floquet engineering consists in the modification of physical systems by the application of periodic time-dependent perturbations. The search for the shape of the periodic perturbation that best modifies the properties of a system in order to achieve some predefined metastable target behavior can be formulated as an optimal control problem. We discuss several ways to formulate and solve this problem. We present, as examples, some applications in the context of material science, although the methods discussed here are valid for any quantum system (from molecules and nanostructures to extended periodic and non periodic quantum materials). In particular, we show how one can achieve the manipulation of the Floquet pseudo-bandstructure of a transition metal dichalcogenide monolayer (MoS2).
Non-equilibrium steady states are created when a periodically driven quantum system is also incoherently interacting with an environment - as it is the case in most realistic situations. The notion of Floquet engineering refers to the manipulation of the properties of systems under periodic perturbations. Although it more frequently refers to the coherent states of isolated systems (or to the transient phase for states that are weakly coupled to the environment), it may sometimes be of more interest to consider the final steady states that are reached after decoherence and dissipation take place. In this work, we demonstrate how those final states can be optimally tuned with respect to a given predefined metric, such as for example the maximization of the temporal average value of some observable, by using multicolor periodic perturbations. We show a computational framework that can be used for that purpose, and exemplify the concept using a simple model for the nitrogen-vacancy center in diamond: the goal in this case is to find the driving periodic magnetic field that maximizes a time-averaged spin component. We show that, for example, this technique permits to prepare states whose spin values are forbidden in thermal equilibrium at any temperature.
This paper describes an approach to construct temporally shaped control pulses that drive a quantum system toward desired properties. A parametrization in terms of periodic functions with predefined frequencies permits us to realize a smooth, typically simple shape of the pulses; their optimization can be performed based on a variational analysis with Floquet theory. As we show with selected specific examples, this approach permits us to control the dynamics of interacting spins, such that gate operations and entanglement dynamics can be implemented with very high accuracy.
Abstract A primer on the Floquet theory of periodically time-dependent quantum systems is provided, and it is shown how to apply this framework for computing the quasienergy band structure governing the dynamics of ultracold atoms in driven optical cosine lattices. Such systems are viewed here as spatially and temporally periodic structures living in an extended Hilbert space, giving rise to spatio-temporal Bloch waves whose dispersion relations can be manipulated at will by exploiting ac-Stark shifts and multiphoton resonances. The elements required for numerical calculations are introduced in a tutorial manner, and some example calculations are discussed in detail, thereby illustrating future prospects of Floquet engineering.
Considering the example of superconducting circuits, we show how Floquet engineering can be combined with reservoir engineering for the controlled preparation of target states. Floquet engineering refers to the control of a quantum system by means of time-periodic forcing, typically in the high-frequency regime, so that the system is governed effectively by a time-independent Floquet Hamiltonian with novel interesting properties. Reservoir engineering, on the other hand, can be achieved in superconducting circuits by coupling a system of artificial atoms (or qubits) dispersively to pumped leaky cavities, so that the induced dissipation guides the system into a desired target state. It is not obvious that the two approaches can be combined, since reaching the dispersive regime, in which system and cavities exchange excitations only virtually, can be spoiled by driving-induced resonant transitions. However, working in the extended Floquet space and treating both system-cavity coupling as well as driving-induced excitation processes on the same footing perturbatively, we identify regimes, where reservoir engineering of targeted Floquet states is possible and accurately described by an effective time-independent master equation. We successfully benchmark our approach for the preparation of the ground state in a system of interacting bosons subjected to Floquet-engineered magnetic fields in different lattice geometries.
Abstract Floquet engineering or coherent time-periodic driving of quantum systems has been successfully used to synthesize Hamiltonians with novel properties. In ultracold atomic systems, this has led to experimental realizations of artificial gauge fields, topological bandstructures, and observation of dynamical localization, to name a few. Here we present a Floquet-based framework to stroboscopically engineer Hamiltonians with spatial features and periodicity below the diffraction limit of light used to create them by time-averaging over various configurations of a 1D optical Kronig–Penney (KP) lattice. The KP potential is a lattice of narrow subwavelength barriers spaced by half the optical wavelength (λ/2) and arises from the nonlinear optical response of the atomic dark state. Stroboscopic control over the strength and position of this lattice requires time-dependent adiabatic manipulation of the dark-state spin composition. We investigate adiabaticity requirements and shape our time-dependent light fields to respect the requirements. We apply this framework to show that a λ/4-spaced lattice can be synthesized using realistic experimental parameters as an example, discuss mechanisms that limit lifetimes in these lattices, explore candidate systems and their limitations, and treat adiabatic loading into the ground band of these lattices.
Floquet engineering is a versatile tool that uses periodic driving of a quantum system to build novel many-body quantum states with drive-dependent properties. In this thesis I will detail experiments performed in the Weld group which explore a many-body Floquet system consisting of tunably-interacting ultracold atoms in an optical lattice amplitude-modulated at up to a thousand percent. I will discuss experiments in which we use Floquet engineering to coherently control long-range quantum transport in hybridized Floquet-Bloch bands. I will also discuss our use of a double quench protocol to experimentally control and quantitatively characterize Floquet prethermalization associated with a periodic generalized Gibbs ensemble.