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arXiv:2301.02004 · SciPost Physics

Optimizing Floquet engineering for non-equilibrium steady states with gradient-based methods

Alberto Castro, Shunsuke A. Sato

Published Jul 26, 2023• 4 citations
arXivHTMLPDF

Abstract

Non-equilibrium steady states are created when a periodically driven quantum system is also incoherently interacting with an environment - as it is the case in most realistic situations. The notion of Floquet engineering refers to the manipulation of the properties of systems under periodic perturbations. Although it more frequently refers to the coherent states of isolated systems (or to the transient phase for states that are weakly coupled to the environment), it may sometimes be of more interest to consider the final steady states that are reached after decoherence and dissipation take place. In this work, we demonstrate how those final states can be optimally tuned with respect to a given predefined metric, such as for example the maximization of the temporal average value of some observable, by using multicolor periodic perturbations. We show a computational framework that can be used for that purpose, and exemplify the concept using a simple model for the nitrogen-vacancy center in diamond: the goal in this case is to find the driving periodic magnetic field that maximizes a time-averaged spin component. We show that, for example, this technique permits to prepare states whose spin values are forbidden in thermal equilibrium at any temperature.

DOI
10.21468/scipostphys.15.1.029

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Non-equilibrium steady states are created when a periodically driven quantum system is also incoherently interacting with an environment - as it is the case in most realistic situations. The notion of Floquet engineering refers to the manipulation of the properties of systems under periodic perturbations. Although it more frequently refers to the coherent states of isolated systems (or to the transient phase for states that are weakly coupled to the environment), it may sometimes be of more interest to consider the final steady states that are reached after decoherence and dissipation take place. In this work, we demonstrate how those final states can be optimally tuned with respect to a given predefined metric, such as for example the maximization of the temporal average value of some observable, by using multicolor periodic perturbations. We show a computational framework that can be used for that purpose, and exemplify the concept using a simple model for the nitrogen-vacancy center in diamond: the goal in this case is to find the driving periodic magnetic field that maximizes a time-averaged spin component. We show that, for example, this technique permits to prepare states whose spin values are forbidden in thermal equilibrium at any temperature.
A procedure to find optimal regimes for quantum thermal engines (QTMs) is described and demonstrated. The QTMs are modelled as the periodically-driven non-equilibrium steady states of open quantum systems, whose dynamics is approximated in this work with Markovian master equations. The action of the external agent and the couplings to the heat reservoirs can be modulated with control functions, and it is the time-dependent shape of these control functions the object of optimisation. Those functions can be freely parameterised, which permits to constrain the solutions according to experimental or physical requirements. • Description of a procedure to find optimal regimes for quantum thermal engines. • The engines are modelled as the periodically-driven non-equilibrium steady states of open quantum systems. • The action of the external agent and the couplings to the heat reservoirs can be modulated with control functions. • Those functions can be freely parameterised to constrain the solutions according to experimental requirements.
Laser technology has developed and accelerated photo-induced nonequilibrium physics, from both the scientific and engineering viewpoints. Floquet engineering, i.e., controlling material properties and functionalities by time-periodic drives, is at the forefront of quantum physics of light-matter interaction. However, it is limited to ideal dissipationless systems. Extending Floquet engineering to various materials requires understanding of the quantum states emerging in a balance of the periodic drive and energy dissipation. Here, we derive a general description for nonequilibrium steady states (NESSs) in periodically driven dissipative systems by focusing on systems under high-frequency drive and time-independent Lindblad-type dissipation. Our formula correctly describes the time average, fluctuation, and symmetry properties of the NESS, and can be computed efficiently in numerical calculations. This approach will play fundamental roles in Floquet engineering in a broad class of dissipative quantum systems from atoms and molecules to mesoscopic systems, and condensed matter.
Nonequilibrium steady states (NESSs) in periodically driven dissipative quantum systems are vital in Floquet engineering. We develop a general theory for high-frequency drives with Lindblad-type dissipation to characterize and analyze NESSs. This theory is based on the high-frequency (HF) expansion with linear algebraic numerics and without numerically solving the time evolution. Using this theory, we show that NESSs can deviate from the Floquet-Gibbs state depending on the dissipation type. We also show the validity and usefulness of the HF-expansion approach in concrete models for a diamond nitrogen-vacancy (NV) center, a kicked open XY spin chain with topological phase transition under boundary dissipation, and the Heisenberg spin chain in a circularly-polarized magnetic field under bulk dissipation. In particular, for the isotropic Heisenberg chain, we propose the dissipation-assisted terahertz (THz) inverse Faraday effect in quantum magnets. Our theoretical framework applies to various time-periodic Lindblad equations that are currently under active research.
Floquet engineering, the control of a quantum system by means of time-periodic driving, allows to modify the properties of a system so that it is described by an approximate effective time-independent Hamiltonian. However, in the presence of interactions the stabilization of interesting many-body ground states of such effective Hamiltonians is possible only on a certain time scale, beyond which Floquet heating sets in, as it results from unwanted driving induced resonant excitation. Moreover, the preparation of the ground state of such Floquet engineered effective Hamiltonians usually has to be accomplished adiabatically, which is another source of heating, especially when a phase transition has to be passed in a large system. Here, we propose a general dissipative strategy for the preparation and stabilization of effective ground states that are protected by an energy gap, such as topologically ordered states. It is scalable and relies on coupling the driven system to a thermal bath, the properties of which are chosen so that it both suppresses Floquet heating and guides the system into a non-equilibrium steady state with a large occupation of the effective ground-state. The small residual occupations of effective excited states are non-thermal, reflecting the non-equilibrium nature of the scheme. We use the Floquet-Born-Markov master equation to verify the proposed strategy. In particular, we discuss the preparation of both a one-dimensional Mott insulator and a two-dimensional fractional Chern insulator in strongly driven Bose-Hubbard systems.
The advancement of magnonics has facilitated the utilization of hybrid magnetic systems in quantum technologies. A hybrid magnetic lattice formed by an array of superconducting loops and magnetic particles has been devised as a quantum bus to disseminate quantum resources among magnetic quantum entities serving as nodes of a quantum network. However, the lattice also exerts a decoherence effect on the quantum entities, which impairs its practical performance. By studying the non-Markovian dynamics of nitrogen-vacancy centers and magnon modes coupled to two independent hybrid magnetic lattices, we propose a Floquet-engineering scheme via periodic driving on the quantum entities to suppress decoherence. We find that significant steady-state entanglement is preserved when a Floquet bound state exists in the quasienergy spectrum of the system consisting of each driven quantum entity and its lattice. This result enables a precise manipulation of hybrid magnetic systems and benefits their applications in quantum networks. The hybrid magnetic lattice has been proposed as a quantum bus for integrating the quantum network, but the decoherence depletes the quantum resources carried by it. By studying the non-Markovian dynamics of nitrogen-vacancy centers and magnon modes coupled to two independent hybrid magnetic lattices, the authors demonstrate a Floquet-engineering scheme using periodic driving to suppress decoherence.
Recent advances in experimental condensed matter physics suggest a powerful new paradigm for the realization of exotic phases of quantum matter in the laboratory. Rather than conducting an exhaustive search for materials that realize these phases at low temperatures, it may be possible to design quantum systems that exhibit the desired properties. With the numerous advances made recently in the fields of cold atomic gases, superconducting qubits, trapped ions, and nitrogen-vacancy centers in diamond, it appears that we will soon have a host of platforms that can be used to put exotic theoretical predictions to the test. In this dissertation, I will highlight two ways in which theorists can interact productively with this fast-emerging field. \n \nFirst, there is a growing interest in driving quantum systems out of equilibrium in order to induce novel topological phases where they would otherwise never appear. In particular, systems driven by time-periodic perturbations—known as “Floquet systems”—offer fertile ground for theoretical investigation. This approach to designer quantum matter brings its own unique set of challenges. In particular, Floquet systems explicitly violate conservation of energy, providing no notion of a ground state. In the first part of my dissertation, I will present research that addresses this problem in two ways. First, I will present studies of open Floquet systems, where coupling to an external reservoir drives the system into a steady state at long times. Second, I will discuss examples of isolated quantum systems that exhibit signatures of topological properties in their finite-time dynamics. \n \nThe second part of this dissertation presents another way in which theorists can benefit from the designer approach to quantum matter; in particular, one can design analytically tractable theories of exotic phases. I will present an exemplar of this philosophy in the form of coupled-wire constructions. In this approach, one builds a topological state of matter from the ground up by coupling together an array of one-dimensional quantum wires with local interactions. I will demonstrate the power of this technique by showing how to build both Abelian and non-Abelian topological phases in three dimensions by coupling together an array of quantum wires.