Floquet engineering offers a compelling approach for designing the time evolution of periodically driven systems. We implement a periodic atom-light coupling to realize Floquet atom optics on the strontium ^{1}S_{0}-^{3}P_{1} transition. These atom optics reach pulse efficiencies above 99.4% over a wide range of frequency offsets between light and atomic resonance, even under strong driving where this detuning is on the order of the Rabi frequency. Moreover, we use Floquet atom optics to compensate for differential Doppler shifts in large momentum transfer atom interferometers and achieve state-of-the-art momentum separation in excess of 400 ℏk. This technique can be applied to any two-level system at arbitrary coupling strength, with broad application in coherent quantum control.Floquet engineering offers a compelling approach for designing the time evolution of periodically driven systems. We implement a periodic atom-light coupling to realize Floquet atom optics on the strontium ^{1}S_{0}-^{3}P_{1} transition. These atom optics reach pulse efficiencies above 99.4% over a wide range of frequency offsets between light and atomic resonance, even under strong driving where this detuning is on the order of the Rabi frequency. Moreover, we use Floquet atom optics to compensate for differential Doppler shifts in large momentum transfer atom interferometers and achieve state-of-the-art momentum separation in excess of 400 ℏk. This technique can be applied to any two-level system at arbitrary coupling strength, with broad application in coherent quantum control.

arXiv:2205.06965Physical Review LettersOct 24, 202249 citations

Optimal Floquet state engineering for large scale atom interferometers

Tangui Rodzinka, E Dionis, L. Calmels +6 more

The effective control of atomic coherence with cold atoms has made atom interferometry an essential tool for quantum sensors and precision measurements. The performance of these interferometers is closely related to the operation of large wave packet separations. We present here a novel approach for atomic beam splitters based on the stroboscopic stabilization of quantum states in an accelerated optical lattice. The corresponding Floquet state is generated by optimal control protocols. In this way, we demonstrate an unprecedented Large Momentum Transfer (LMT) interferometer, with a momentum separation of 600 photon recoils (600 ℏk) between its two arms. Each LMT beam splitter is realized in a remarkably short time (2 ms) and is highly robust against the initial velocity dispersion of the wave packet and lattice depth fluctuations. Our study shows that Floquet engineering is a promising tool for exploring new frontiers in quantum physics at large scales, with applications in quantum sensing and testing fundamental physics. Large-scale atom interferometers enable precise measurements of fundamental constants and novel sensors. This study uses Floquet formalism to create an optimal transported state, resulting in an efficient large-momentum-transfer interferometer, advancing largescale interferometers.The effective control of atomic coherence with cold atoms has made atom interferometry an essential tool for quantum sensors and precision measurements. The performance of these interferometers is closely related to the operation of large wave packet separations. We present here a novel approach for atomic beam splitters based on the stroboscopic stabilization of quantum states in an accelerated optical lattice. The corresponding Floquet state is generated by optimal control protocols. In this way, we demonstrate an unprecedented Large Momentum Transfer (LMT) interferometer, with a momentum separation of 600 photon recoils (600 ℏk) between its two arms. Each LMT beam splitter is realized in a remarkably short time (2 ms) and is highly robust against the initial velocity dispersion of the wave packet and lattice depth fluctuations. Our study shows that Floquet engineering is a promising tool for exploring new frontiers in quantum physics at large scales, with applications in quantum sensing and testing fundamental physics. Large-scale atom interferometers enable precise measurements of fundamental constants and novel sensors. This study uses Floquet formalism to create an optimal transported state, resulting in an efficient large-momentum-transfer interferometer, advancing largescale interferometers.

arXiv:2403.14337Nature CommunicationsNov 27, 202427 citations

Floquet engineering of optical nonlinearities: a quantum many-body approach

Nathan Goldman

Subjecting a physical system to a time-periodic drive can substantially modify its properties and applications. This Floquet-engineering approach has been extensively applied to a wide range of classical and quantum settings in view of designing synthetic systems with exotic properties. Considering a general class of two-mode nonlinear optical devices, we show that effective optical nonlinearities can be created by subjecting the light field to a repeated pulse sequence, which couples the two modes in a fast and time-periodic manner. The strength of these drive-induced optical nonlinearities, which include an emerging four-wave mixing, can be varied by simply adjusting the pulse sequence. This leads to topological changes in the system's phase space, which can be detected through light intensity and phase measurements. Our proposal builds on an effective-Hamiltonian approach, which derives from a parent quantum many-body Hamiltonian describing driven interacting bosons. As a corollary, our results equally apply to Bose-Einstein condensates in driven double-well potentials, where pair tunneling effectively arises from the periodic pulse sequence. Our scheme offers a practical route to engineer and finely tune exotic nonlinearities and interactions in photonics and ultracold quantum gases.Subjecting a physical system to a time-periodic drive can substantially modify its properties and applications. This Floquet-engineering approach has been extensively applied to a wide range of classical and quantum settings in view of designing synthetic systems with exotic properties. Considering a general class of two-mode nonlinear optical devices, we show that effective optical nonlinearities can be created by subjecting the light field to a repeated pulse sequence, which couples the two modes in a fast and time-periodic manner. The strength of these drive-induced optical nonlinearities, which include an emerging four-wave mixing, can be varied by simply adjusting the pulse sequence. This leads to topological changes in the system's phase space, which can be detected through light intensity and phase measurements. Our proposal builds on an effective-Hamiltonian approach, which derives from a parent quantum many-body Hamiltonian describing driven interacting bosons. As a corollary, our results equally apply to Bose-Einstein condensates in driven double-well potentials, where pair tunneling effectively arises from the periodic pulse sequence. Our scheme offers a practical route to engineer and finely tune exotic nonlinearities and interactions in photonics and ultracold quantum gases.

arXiv:2203.05554Mar 10, 20223 citations

Floquet Engineering Hz-Level Rabi Spectra in Shallow Optical Lattice Clock

Mo-Juan Yin, Xiaotong Lu, Ting Li +4 more

Quantum metrology with ultrahigh precision usually requires atoms prepared in an ultrastable environment with well-defined quantum states. Thus, in optical lattice clock systems deep lattice potentials are used to trap ultracold atoms. However, decoherence, induced by Raman scattering and higher order light shifts, can significantly be reduced if atomic clocks are realized in shallow optical lattices. On the other hand, in such lattices, tunneling among different sites can cause additional dephasing and strongly broadening of the Rabi spectrum. Here, in our experiment, we periodically drive a shallow ^{87}Sr optical lattice clock. Counterintuitively, shaking the system can deform the wide broad spectral line into a sharp peak with 5.4 Hz linewidth. With careful comparison between the theory and experiment, we demonstrate that the Rabi frequency and the Bloch bands can be tuned, simultaneously and independently. Our work not only provides a different idea for quantum metrology, such as building shallow optical lattice clock in outer space, but also paves the way for quantum simulation of new phases of matter by engineering exotic spin orbit couplings.Quantum metrology with ultrahigh precision usually requires atoms prepared in an ultrastable environment with well-defined quantum states. Thus, in optical lattice clock systems deep lattice potentials are used to trap ultracold atoms. However, decoherence, induced by Raman scattering and higher order light shifts, can significantly be reduced if atomic clocks are realized in shallow optical lattices. On the other hand, in such lattices, tunneling among different sites can cause additional dephasing and strongly broadening of the Rabi spectrum. Here, in our experiment, we periodically drive a shallow ^{87}Sr optical lattice clock. Counterintuitively, shaking the system can deform the wide broad spectral line into a sharp peak with 5.4 Hz linewidth. With careful comparison between the theory and experiment, we demonstrate that the Rabi frequency and the Bloch bands can be tuned, simultaneously and independently. Our work not only provides a different idea for quantum metrology, such as building shallow optical lattice clock in outer space, but also paves the way for quantum simulation of new phases of matter by engineering exotic spin orbit couplings.

arXiv:2110.07169Physical Review LettersFeb 17, 202235 citations

Polychromatic atom optics for atom interferometry

Samuel Lellouch, Oliver Ennis, Ramiz Haditalab +2 more

Abstract Coherent manipulation of atoms with atom-optic light pulses is central to atom interferometry. Achieving high pulse efficiency is essential for enhancing fringe contrast and sensitivity, in particular for large-momentum transfer interferometers which use an increased number of pulses. We perform an investigation of optimizing the frequency domain of pulses by using tailored polychromatic light fields, and demonstrate the possibility to deliver high-efficiency and resilient atom-optic pulses even in the situation of inhomogeneous atomic clouds and laser beams. We find that this approach is able to operate over long interrogation times despite spontaneous emission and to achieve experimentally relevant pulse efficiencies for clouds up to $100~\mu \text{K}$ 100 μ K . This overcomes some of the most stringent barriers for large-momentum transfer and has the potential to reduce the complexity of atom interferometers. We show that polychromatic light pulses could enhance single-photon-based large-momentum transfer atom interferometry—achieving $850\,\hbar k$ 850 ħ k of momentum splitting with experimentally accessible parameters, which represents a significant improvement over the state-of-the art. The benefits of the method extend beyond atom interferometry and could enable groundbreaking advances in quantum state manipulation.Abstract Coherent manipulation of atoms with atom-optic light pulses is central to atom interferometry. Achieving high pulse efficiency is essential for enhancing fringe contrast and sensitivity, in particular for large-momentum transfer interferometers which use an increased number of pulses. We perform an investigation of optimizing the frequency domain of pulses by using tailored polychromatic light fields, and demonstrate the possibility to deliver high-efficiency and resilient atom-optic pulses even in the situation of inhomogeneous atomic clouds and laser beams. We find that this approach is able to operate over long interrogation times despite spontaneous emission and to achieve experimentally relevant pulse efficiencies for clouds up to $100~\mu \text{K}$ 100 μ K . This overcomes some of the most stringent barriers for large-momentum transfer and has the potential to reduce the complexity of atom interferometers. We show that polychromatic light pulses could enhance single-photon-based large-momentum transfer atom interferometry—achieving $850\,\hbar k$ 850 ħ k of momentum splitting with experimentally accessible parameters, which represents a significant improvement over the state-of-the art. The benefits of the method extend beyond atom interferometry and could enable groundbreaking advances in quantum state manipulation.

EPJ Quantum TechnologyMar 8, 20234 citations

Spectral-Domain Coherent Control of Broadband Raman Coupling in Atom Interferometry

Shengzhe Wang, Weichen Jia, Yue Xin +3 more

The performance of atom interferometers is commonly limited by the finite spectral acceptance of atomic beam splitters and mirrors, which restricts efficient coupling to atoms with large Doppler shifts and reduces the usable atomic flux. Here, we demonstrate spectral-domain coherent control of Raman coupling by engineering its effective two-photon spectrum. By synthesizing multiple frequency components, the Raman interaction simultaneously addresses a broad range of atomic velocities, effectively overcoming the conventional transit-time-limited linewidth. Implemented in a continuous atomic-beam Mach-Zehnder interferometer, where the transverse Doppler broadening is 17 times larger than the intrinsic Raman linewidth, this approach enhances the fringe contrast from 5.9(2)% to 15.1(2)%, indicating a substantial increase in effective atomic participation. Our results establish spectral-domain coherent control as a general strategy for achieving spectrally robust atom interferometry and open new opportunities for quantum sensing in systems with strong inhomogeneous broadening.The performance of atom interferometers is commonly limited by the finite spectral acceptance of atomic beam splitters and mirrors, which restricts efficient coupling to atoms with large Doppler shifts and reduces the usable atomic flux. Here, we demonstrate spectral-domain coherent control of Raman coupling by engineering its effective two-photon spectrum. By synthesizing multiple frequency components, the Raman interaction simultaneously addresses a broad range of atomic velocities, effectively overcoming the conventional transit-time-limited linewidth. Implemented in a continuous atomic-beam Mach-Zehnder interferometer, where the transverse Doppler broadening is 17 times larger than the intrinsic Raman linewidth, this approach enhances the fringe contrast from 5.9(2)% to 15.1(2)%, indicating a substantial increase in effective atomic participation. Our results establish spectral-domain coherent control as a general strategy for achieving spectrally robust atom interferometry and open new opportunities for quantum sensing in systems with strong inhomogeneous broadening.

arXiv:2604.03629Apr 4, 20260 citations

100~\mu \text{K}

100 μ K . This overcomes some of the most stringent barriers for large-momentum transfer and has the potential to reduce the complexity of atom interferometers. We show that polychromatic light pulses could enhance single-photon-based large-momentum transfer atom interferometry—achieving

850\,\hbar k

850 ħ k of momentum splitting with experimentally accessible parameters, which represents a significant improvement over the state-of-the art. The benefits of the method extend beyond atom interferometry and could enable groundbreaking advances in quantum state manipulation.