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Acta Physica Sinica

Effect of spatial walk-off on squeezing properties of quantum optical frequency combs

Juan Li, Peng Liu, Xiao Xiang, Tao Liu, Ruifang Dong, Shougang Zhang

Published Jan 1, 2023• 1 citation
Publisher

Abstract

Quantum optical frequency combs are of great significance in the fields of quantum computing, quantum information, and high precision quantum measurement, which can be produced by using a degenerate type-I synchronously pumped optical parametric oscillator (SPOPO). When anisotropic crystal is used as a nonlinear medium in the SPOPO, the spatial walk-off effect will occur due to the birefringence effect, which cannot be ignored and will adversely affect the generation of squeezed state. In this work, we investigate the influence of spatial walk-off effect on the squeezing level of quantum optical frequency combs both theoretically and experimentally. A Ti∶sapphire mode-locked femtosecond pulsed laser which produces 130 fs pulse trains at 815 nm with a repetition rate of 76 MHz is utilized as a fundamental source. Its second harmonic at 407.5 nm is used to pump the collinear BiB3O6 (BIBO) crystal for generating the squeezed vacuum frequency comb. It is indicated that as the crystal length increases, the area of interaction between pump light and signal light decreases gradually. Thus the enhancement of squeezing is eventually limited by the spatial walk-off effect. According to the simulations, the squeezing level reaches a maximum value when the crystal length is 1.49 mm. The quantum properties of squeezed vacuum optical frequency combs obtained for four crystal lengths (0.5, 1.0, 1.5 and 2.0 mm) are subsequently measured experimentally. When the length of BIBO is 1.5 mm, the maximum vacuum squeezing of (3.6±0.2) dB is obtained, which is (7.0±0.2) dB after being corrected for detection loss. The experimental results are consistent with the numerical simulations. This study demonstrates that the spatial walk-off effect in nonlinear crystal is a significant factor affecting the quantum optical frequency comb, and the theoretical model presented in this paper can be used to provide a guideline for optimizing the experimental implementation.

DOI
10.7498/aps.72.20222343

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Quantum optical frequency combs are of great significance in the fields of quantum computing, quantum information, and high precision quantum measurement, which can be produced by using a degenerate type-I synchronously pumped optical parametric oscillator (SPOPO). When anisotropic crystal is used as a nonlinear medium in the SPOPO, the spatial walk-off effect will occur due to the birefringence effect, which cannot be ignored and will adversely affect the generation of squeezed state. In this work, we investigate the influence of spatial walk-off effect on the squeezing level of quantum optical frequency combs both theoretically and experimentally. A Ti∶sapphire mode-locked femtosecond pulsed laser which produces 130 fs pulse trains at 815 nm with a repetition rate of 76 MHz is utilized as a fundamental source. Its second harmonic at 407.5 nm is used to pump the collinear BiB3O6 (BIBO) crystal for generating the squeezed vacuum frequency comb. It is indicated that as the crystal length increases, the area of interaction between pump light and signal light decreases gradually. Thus the enhancement of squeezing is eventually limited by the spatial walk-off effect. According to the simulations, the squeezing level reaches a maximum value when the crystal length is 1.49 mm. The quantum properties of squeezed vacuum optical frequency combs obtained for four crystal lengths (0.5, 1.0, 1.5 and 2.0 mm) are subsequently measured experimentally. When the length of BIBO is 1.5 mm, the maximum vacuum squeezing of (3.6±0.2) dB is obtained, which is (7.0±0.2) dB after being corrected for detection loss. The experimental results are consistent with the numerical simulations. This study demonstrates that the spatial walk-off effect in nonlinear crystal is a significant factor affecting the quantum optical frequency comb, and the theoretical model presented in this paper can be used to provide a guideline for optimizing the experimental implementation.
Multimode squeezed light is a key resource for quantum technologies, enabling applications in boson sampling, quantum networks, and optical quantum computation [1],[2]. Parametric down-conversion in synchronously pumped optical parametric oscillators (SPOPOs) offers a versatile platform for generating multimode squeezed states across the time-frequency domain. In these systems, supermodes manifest as independent quantum states in the temporal domain and as frequency combs in the spectral domain [3]. Precise control of these states is crucial for quantum applications and requires an experimental setup capable of fine-tuning multiple parameters to optimize squeezing properties. In this work, we present an experimental setup for generating and characterizing multimode vacuum squeezed states using a SPOPO and a balanced homodyne detection scheme. Two spatial light modulators (SLMs) placed on the pump and local oscillator (LO) beams provide full control over their spectral properties, including amplitude and phase shaping. This flexibility allows us to optimize the experimental conditions and investigate squeezing dependence on key parameters such as the LO spectral detuning and bandwidth. By introducing a programmableπ\piπ-phase shift to the LO via the SLM, we selectively probe the multimode structure, distinguishing between even and odd supermodes. Additionally, the SLM on the pump can introduce an arbitrary chirp, further enhancing control over the system. Our setup, schematized in Figure 1a, is based on a commercial mode-locked Yb-fiber laser operating at 93MHz, emitting pulses centered at 1035nm with a 10nm bandwidth. A portion of the radiation is frequency-doubled to 517.5nm via an LBO crystal to serve as the pump for the SPOPO, while the remaining part is used as the LO for homodyne detection after transmission through the SPOPO cavity, ensuring high beam quality. The SPOPO cavity is frequency-locked to the laser via a Pound-Drever-Hall technique, ensuring stable and optimized operation. Figure 1b presents representative measurements of squeezing levels as a function of the LO spectral bandwidth, showing how its symmetric or antisymmetric phase influences the detection of different supermodes and, consequently, the squeezing level depending on their structure. The measurements were performed using lithium niobate (LNB) nonlinear crystals of 3.0mm and 1.5mm lengths. Our setup allows for future investigations of dispersion effects on squeezing, thus far only theoretically predicted [4], by introducing chirped mirrors for dispersion compensation. Moreover, different nonlinear crystals, such as lithium niobate, beta barium borate (BBO), and lithium triborate (LBO) of various lengths, will be tested to explore the multimode properties of the squeezed states. These investigations will provide insights into the experimental conditions required to achieve single-mode squeezing, crucial for applications such as Gaussian Boson Sampling, with results to be presented at the conference.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables [1]. They can be generated either by mixing different squeezed light sources using linear optical operations [2], or directly in a multimode optical device [3, 4]. Synchronously Pumped Optical Parametric Oscillators (SPOPO) — which correspond to an OPO pumped by a train of ultrashort pulses that are synchronized with the cavity round-trip time — have been theoretically shown to be promising devices for the generation of multimode nonclassical frequency combs, since a SPOPO is a sole optical cavity acting as an assembly of independent squeezers in a particular basis called the supermodes basis [5]. The supermodes are optical frequency combs with specific spectrum and phase profiles that are determined by the length of the intracavity nonlinear crystal and the pulse shape of the pump.
Nonclassical optical frequency combs find tremendous utility in quantum information and high-precision quantum measurement.The characteristics of a type-I synchronously pumped optical parametric oscillator with the TEM 01 transverse mode below threshold are investigated and a squeezing of 0.7 dB for an optical frequency comb squeezed light field with the TEM 01 transverse mode is obtained under the pump power of 130 mW.This work has a promising application in three-dimensional space-time measurement.
We have developed the full theory of a synchronously pumped type I optical parametric oscillator (SPOPO). We derive expressions for the oscillation threshold and the characteristics of the generated mode-locked signal beam. We calculate the output quantum fluctuations of the device, and find that, in the degenerate case (coincident signal and idler set of frequencies), perfect squeezing is obtained when one approaches threshold from below for a well defined "super-mode', or frequency comb, consisting of a coherent linear superposition of signal modes of different frequencies which are resonant in the cavity.
The field of squeezed state is an important quantum resource in the study of quantum optics. In the application of quantum information, the spectrum bandwidth of the squeezed light field is an important index to limit the information transmission capacity. Currently, the optical parametric oscillator (OPO) is one of the most efficient ways to generate high squeezed non-classical optical fields. In this paper, the degenerate singly-resonant and doubly-resonant OPO structures are introduced. Both OPOs are composed of concave mirrors and periodically poled potassium titanyl phosphate crystals (PPKTP). The length of PPKTP crystal is 10 mm. The curvature radius of the curved surface is 12 mm, and it has high reflectivity at 1550 nm and 775 nm. The plane surface is coated with anti-reflection coating. The air gap length is 21 mm. The concave mirror is an output coupling mirror, and its radius of curvature is 25 mm. In the singly-resonant OPO, only the signal light resonates in the cavity, and the pump light passes through the nonlinear crystal twice and then outputs out of the cavity. The reflectivity of OPO output coupling mirror to the wavelength of 1550 nm is 88%. The linewidth of the corresponding fundamental frequency wave is 77.4 MHz. For doubly-resonant OPO, both the signal light and the pump light resonate simultaneously in the cavity. The reflectivity of OPO output coupling mirror to 1550 nm and 775 nm is 85% and 97.5%, respectively. The linewidth of the corresponding fundamental frequency wave and harmonic is 97.1 MHz and 15.6 MHz, respectively. Then the threshold of OPO is calculated. The threshold pump power of OPO increases with signal light transmittance increasing, but the threshold value of doubly-resonant OPO is obviously smaller than that of singly-resonant OPO. After that, the variation of the squeezing bandwidth of the squeezed light field generated by OPO with the transmittance of the signal is analyzed. Finally, we complete the design of quantum squeezer with low threshold (18 mW), broadband (84.2 MHz) and high stability (the standard deviation of locking baseline is 0.32 MHz) experimentally. The results show that compared with the singly-resonant optical parametric oscillator, the doubly-resonant cavity has the characteristics of low threshold and high stability, which is more suitable for the preparation and practical application of broadband squeezed light field.
Synchronously pumped optical parametric oscillators (SPOPOs) are optical cavities driven by mode-locked lasers, and containing a nonlinear crystal capable of down-converting a frequency comb to lower frequencies. SPOPOs have received a lot of attention lately because their intrinsic multimode nature makes them compact sources of quantum correlated light with promising applications in modern quantum information technologies. In this work we show that SPOPOs are also capable of accessing the challenging and interesting regime where spontaneous symmetry breaking confers strong nonclassical properties to the emitted light, which has eluded experimental observation so far. Apart from opening the possibility of studying experimentally this elusive regime of dissipative phase transitions, our predictions will have a practical impact, since we show that spontaneous symmetry breaking provides a specific spatiotemporal mode with large quadrature squeezing for any value of the system parameters, turning SPOPOs into robust sources of highly nonclassical light above threshold.