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arXiv:1611.06550 · Physical Review A

Noncritical generation of nonclassical frequency combs via spontaneous rotational symmetry breaking

Carlos Navarrete–Benlloch, Giuseppe Patera, Germán J. de Valcárcel

Published Oct 2, 2017• 8 citations
arXivHTMLPDF

Abstract

Synchronously pumped optical parametric oscillators (SPOPOs) are optical cavities driven by mode-locked lasers, and containing a nonlinear crystal capable of down-converting a frequency comb to lower frequencies. SPOPOs have received a lot of attention lately because their intrinsic multimode nature makes them compact sources of quantum correlated light with promising applications in modern quantum information technologies. In this work we show that SPOPOs are also capable of accessing the challenging and interesting regime where spontaneous symmetry breaking confers strong nonclassical properties to the emitted light, which has eluded experimental observation so far. Apart from opening the possibility of studying experimentally this elusive regime of dissipative phase transitions, our predictions will have a practical impact, since we show that spontaneous symmetry breaking provides a specific spatiotemporal mode with large quadrature squeezing for any value of the system parameters, turning SPOPOs into robust sources of highly nonclassical light above threshold.

DOI
10.1103/physreva.96.043801

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Synchronously pumped optical parametric oscillators (SPOPOs) are optical cavities driven by mode-locked lasers, and containing a nonlinear crystal capable of down-converting a frequency comb to lower frequencies. SPOPOs have received a lot of attention lately because their intrinsic multimode nature makes them compact sources of quantum correlated light with promising applications in modern quantum information technologies. In this work we show that SPOPOs are also capable of accessing the challenging and interesting regime where spontaneous symmetry breaking confers strong nonclassical properties to the emitted light, which has eluded experimental observation so far. Apart from opening the possibility of studying experimentally this elusive regime of dissipative phase transitions, our predictions will have a practical impact, since we show that spontaneous symmetry breaking provides a specific spatiotemporal mode with large quadrature squeezing for any value of the system parameters, turning SPOPOs into robust sources of highly nonclassical light above threshold.
Multimode nonclassical states of light are an essential resource in quantum computation with continuous variables [1]. They can be generated either by mixing different squeezed light sources using linear optical operations [2], or directly in a multimode optical device [3, 4]. Synchronously Pumped Optical Parametric Oscillators (SPOPO) — which correspond to an OPO pumped by a train of ultrashort pulses that are synchronized with the cavity round-trip time — have been theoretically shown to be promising devices for the generation of multimode nonclassical frequency combs, since a SPOPO is a sole optical cavity acting as an assembly of independent squeezers in a particular basis called the supermodes basis [5]. The supermodes are optical frequency combs with specific spectrum and phase profiles that are determined by the length of the intracavity nonlinear crystal and the pulse shape of the pump.
We predict squeezed light generation through the spontaneous rotational symmetry breaking occurring in a degenerate optical parametric oscillator (DOPO) pumped above threshold. We show, within the linearized theory, that a DOPO with spherical mirrors, in which the signal and idler fields correspond to first-order Laguerre-Gauss modes, produces a perfectly squeezed vacuum with the shape of a Hermite-Gauss mode. This occurs at any pumping level above threshold; hence, the phenomenon is noncritical. Imperfections of the rotational symmetry, due, e.g., to cavity anisotropy, are shown to have a small impact.
In a series of articles we studied the quantum properties of a degenerate optical parametric oscillator tuned to the first family of transverse modes at the subharmonic. We found that, for a cavity having rotational symmetry with respect to the optical axis, a TEM10{}_{10}10​ mode with an arbitrary orientation in the transverse plane is emitted above threshold. We proved then that quantum noise induces a random rotation of this bright TEM10{}_{10}10​ mode in the transverse plane, while the orthogonal mode, the so-called dark mode, has perfect quadrature squeezing irrespective of the distance to threshold (noncritical squeezing). This result was linked to the spontaneous rotational symmetry breaking which occurs when the bright mode is generated, and here we analyze how the squeezing of the dark mode is degraded when the cavity is not perfectly symmetric. We will show that large levels of squeezing are still attainable for reasonable values of this anisotropy, with the advantage that the orientation of the bright and dark modes is basically fixed, a very attractive situation from the experimental point of view.
Multimode squeezed light is a key resource for quantum technologies, enabling applications in boson sampling, quantum networks, and optical quantum computation [1],[2]. Parametric down-conversion in synchronously pumped optical parametric oscillators (SPOPOs) offers a versatile platform for generating multimode squeezed states across the time-frequency domain. In these systems, supermodes manifest as independent quantum states in the temporal domain and as frequency combs in the spectral domain [3]. Precise control of these states is crucial for quantum applications and requires an experimental setup capable of fine-tuning multiple parameters to optimize squeezing properties. In this work, we present an experimental setup for generating and characterizing multimode vacuum squeezed states using a SPOPO and a balanced homodyne detection scheme. Two spatial light modulators (SLMs) placed on the pump and local oscillator (LO) beams provide full control over their spectral properties, including amplitude and phase shaping. This flexibility allows us to optimize the experimental conditions and investigate squeezing dependence on key parameters such as the LO spectral detuning and bandwidth. By introducing a programmableπ\piπ-phase shift to the LO via the SLM, we selectively probe the multimode structure, distinguishing between even and odd supermodes. Additionally, the SLM on the pump can introduce an arbitrary chirp, further enhancing control over the system. Our setup, schematized in Figure 1a, is based on a commercial mode-locked Yb-fiber laser operating at 93MHz, emitting pulses centered at 1035nm with a 10nm bandwidth. A portion of the radiation is frequency-doubled to 517.5nm via an LBO crystal to serve as the pump for the SPOPO, while the remaining part is used as the LO for homodyne detection after transmission through the SPOPO cavity, ensuring high beam quality. The SPOPO cavity is frequency-locked to the laser via a Pound-Drever-Hall technique, ensuring stable and optimized operation. Figure 1b presents representative measurements of squeezing levels as a function of the LO spectral bandwidth, showing how its symmetric or antisymmetric phase influences the detection of different supermodes and, consequently, the squeezing level depending on their structure. The measurements were performed using lithium niobate (LNB) nonlinear crystals of 3.0mm and 1.5mm lengths. Our setup allows for future investigations of dispersion effects on squeezing, thus far only theoretically predicted [4], by introducing chirped mirrors for dispersion compensation. Moreover, different nonlinear crystals, such as lithium niobate, beta barium borate (BBO), and lithium triborate (LBO) of various lengths, will be tested to explore the multimode properties of the squeezed states. These investigations will provide insights into the experimental conditions required to achieve single-mode squeezing, crucial for applications such as Gaussian Boson Sampling, with results to be presented at the conference.
A synchronously pumped optical parametric oscillator (SPOPO) operating at 93 MHz is used to generate squeezed states at 1035 nm. The system features a counter-propagating beam at the same wavelength as the quantum state, which simultaneously actively stabilizes the cavity and, after transmission, acts as the local oscillator for homodyne detection. By deriving the local oscillator directly from the SPOPO cavity, the setup establishes an intrinsically excellent spatial mode overlap and high interference visibility, forming a distinctive self-referenced architecture. Two spatial light modulators enable precise spectral shaping of both the pump and the local oscillator in amplitude and phase, allowing investigation of the spectral properties of the generated states. The versatility of the setup further allows exploration of different SPOPO configurations, including regimes with varied finesse and escape efficiency. Representative measurements, including homodyne traces and squeezing levels as functions of pump power and local oscillator bandwidth, demonstrate the performance of the system. Theoretical simulations based on a multimode singular-value-decomposition model reproduce well the measured dependence of squeezing on pump power and LO bandwidth, confirming the accuracy of the description and the robustness of the setup. Measured squeezing levels up to − 3.3 dB are achieved, corresponding to − 5.7 dB at SPOPO output, evidencing the robustness and versatility of this platform for stable pulsed squeezed-light generation and advanced quantum optical applications.