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Photorefractive Effects, Materials, and Devices

Dynamic Solutions and Instabilities of the Four-wave Mixing Interaction Utilising the Underlying SU(2) Group Symmetry

G. R. Barrett, A. K. Powell, Trevor J. Hall

Published Jan 1, 1991• 0 citations
Publisher

Abstract

Optical phase conjugation is an important nonlinear process, with many applications in the areas of optical communications and optical processing. This is as a result of the wave-front correction properties that phase conjugation offers and this has generated much interest in the area. A common method of producing phase conjugated wavefronts is the four-wave mixing interaction and many publications on the steady state solution to this problem have appeared over the last decade. More recently, however, interest has been focussed upon the temporal behaviour of four-wave mixing systems, with instabilities and chaos being both demonstrated by Gauthier et al [1] and predicted by Królikowski et al [2]. To date, the analysis for the temporal behaviour of anisotropic four wave mixing, in the transmission grating regime, has involved the direct numerical integration of the equations describing four wave mixing. This analysis however, does not utilise the symmetries of the four wave mixing process, and thus results in a more complex problem. Through exploitation of these symmetries the complexity of the problem has been reduced from one containing four complex variables, to one containing three real variables. This has been accomplished through the use of the Special Unitary Group 2, a group providing a two dimensional matrix, whose elements are functions of three real variables. The multiplication of this matrix, together with one containing the boundary conditions for the problem, thus enables the four complex beam amplitudes to be reexpressed in terms of three real quantities. Using this technique, the temporal nature of anisotropic four wave mixing has been studied, and shown under certain conditions, to exhibit chaotic behaviour when an electric field is present. The effect of any material absorption on the chaotic nature is also demonstrated.

DOI
10.1364/pmed.1991.tuc21

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Optical phase conjugation is an important nonlinear process, with many applications in the areas of optical communications and optical processing. This is as a result of the wave-front correction properties that phase conjugation offers and this has generated much interest in the area. A common method of producing phase conjugated wavefronts is the four-wave mixing interaction and many publications on the steady state solution to this problem have appeared over the last decade. More recently, however, interest has been focussed upon the temporal behaviour of four-wave mixing systems, with instabilities and chaos being both demonstrated by Gauthier et al [1] and predicted by Królikowski et al [2]. To date, the analysis for the temporal behaviour of anisotropic four wave mixing, in the transmission grating regime, has involved the direct numerical integration of the equations describing four wave mixing. This analysis however, does not utilise the symmetries of the four wave mixing process, and thus results in a more complex problem. Through exploitation of these symmetries the complexity of the problem has been reduced from one containing four complex variables, to one containing three real variables. This has been accomplished through the use of the Special Unitary Group 2, a group providing a two dimensional matrix, whose elements are functions of three real variables. The multiplication of this matrix, together with one containing the boundary conditions for the problem, thus enables the four complex beam amplitudes to be reexpressed in terms of three real quantities. Using this technique, the temporal nature of anisotropic four wave mixing has been studied, and shown under certain conditions, to exhibit chaotic behaviour when an electric field is present. The effect of any material absorption on the chaotic nature is also demonstrated.
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One more promising application of the four-wave mixing process is the correction of arbitrary phase aberrations in an optical beam. In such applications, the fidelity as well as the efficiency of the phase-conjugation process needs to be considered in practice. The process which has received the most extensive attention to date is degenerate four-wave mixing (DFWM). The nonlinear interaction in this case is known to result in a perfect phase-conjugate provided high-quality pump beams are available and competing effects such as local self-focusing (or defocusing) can be neglected.
The phase-conjugate reflectivity produced by degenerate four-wave mixing in a Kerr medium in the Bragg scattering regime is shown to be unstable when the intensity of the external pump beams is greater than a threshold value that can be predicted analytically. Below this threshold, a single branch of the reflectivity curve is stable, eliminating any possibility for bistability. A numerical simulation indicates that the unstable regime is characterized by fast oscillations with a period related to the transit time in the nonlinear medium. A finite relaxation time of the nonlinearity eliminates the high-frequency oscillations but can increase the amplitude of the low-frequency components. The insertion of a phase-conjugate mirror into an optical cavity leads to an instability whose threshold can be evaluated analytically. The temporal evolution of the field intensity in the cavity is shown to change from a stable regime to periodic oscillations and then to quasi-periodic oscillations as the pump intensity is increased.
Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].
Optical phase conjugation is concerned with the use of nonlinear optical effects to precisely reverse the direction of propagation of each plane wave in an arbitrary beam of light. This causes the return beam to exactly retrace the path of the incident beam, leading to many applications of automatic pointing and tracking (even in the presence of an inhomogeneous medium). The main goals of this course are familiarization with how each of the many nonlinear optical effects gives rise to a phase conjugate signal, and understanding and appreciation of the many potential applications for optical phase conjugation. Conjugation techniques involving Kerr-like degenerate four-wave mixing, resonant degenerate four-wave mixing, stimulated Brillouin scattering, photorefractive effects, surface phenomena, and others will be carefully reviewed. Applications of particular importance to this course will include distortion correction, pointing, tracking, laser-resonator design, optical information processing, etc. Throughout the course, key references will be identified for those wishing to pursue any topic more vigorously.