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Annual Meeting Optical Society of America

Photon localization In parametric downconversion

John G. Rarity, P. R. Tapster

Published Jan 1, 1988• 0 citations
Publisher

Abstract

Quantum mechanical models of beam splitters1 predict interesting fourth-order interference effects when nonclassical light is used. If indistinguishable one-photon states are simultaneously input into each port of a 50/50 beam splitter, the theory predicts that each output will contain either two photons or none. A naive (particle) theory would predict a mixture of two’s and one’s. The required |1,1〉 photon state can be selected in nondegenerate parametric downconversion experiments by photon-counting coincidence detection. The disappearance of this coincidence after a beam splitter has recently been studied,1-2 and the range of path length differences over which the effect can be seen is related by Fourier transform to the photon bandwidth. In our work the bandwidth is not limited by external filters, and we have developed a theory which relates the measured photon length to the geometry of the apparatus and the detailed phase matching conditions at the parametric crystal. This theory of phase matching viewed through a beam splitter produces some unexpected results when the beam splitter is tilted and when large aperture detectors are considered.

DOI
10.1364/oam.1988.mm1

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Annual Meeting Optical Society of America•Jan 1, 1991•0 citations
Quantum mechanical models of beam splitters1 predict interesting fourth-order interference effects when nonclassical light is used. If indistinguishable one-photon states are simultaneously input into each port of a 50/50 beam splitter, the theory predicts that each output will contain either two photons or none. A naive (particle) theory would predict a mixture of two’s and one’s. The required |1,1〉 photon state can be selected in nondegenerate parametric downconversion experiments by photon-counting coincidence detection. The disappearance of this coincidence after a beam splitter has recently been studied,1-2 and the range of path length differences over which the effect can be seen is related by Fourier transform to the photon bandwidth. In our work the bandwidth is not limited by external filters, and we have developed a theory which relates the measured photon length to the geometry of the apparatus and the detailed phase matching conditions at the parametric crystal. This theory of phase matching viewed through a beam splitter produces some unexpected results when the beam splitter is tilted and when large aperture detectors are considered.
A two-photon state can be selected by coincidence detection of photon pairs created in parametric downconversion. We demonstrate a reduction in the coincidence-count rate when pairs of photons are combined in a beam splitter. This reduction occurs only when photon wave functions overlap and can permit accurate (subpicosecond) relative timing measurements. We relate the width of the coincidence reduction to the bandwidth of the downconverted light and thence to the detailed phase-matching conditions in the parametric downconversion crystal. We also demonstrate that the loss of coincidences is associated with an increased probability of detection of photon pairs in each output of the beam splitter.
Angle-separated pair photons emitted in spontaneous parametric fluorescence are superimposed at a beamsplitter and detected by coincidence techniques. The coincidence disappears when the photon path lengths to the beamsplitter are equal to within their inverse bandwidth due to fourth-order interference. The photon bandwidth is set by wide apertures placed to satisfy phase-matching conditions at the nonlinear crystal. The resulting broadband photons are short (39-fs full width at half maximum) and show an oscillatory tail resulting from the hard-edge apertures. Two-color photons are created by blocking the central portion of the apertures leading to strong oscillations of the coincidence rate as a function of path-length difference. Both effects are predicted by the theory of fourth-order interference coupled with the detailed phase-matching conditions in the nonlinear crystal used as a source. The two colors overlap at different positions on the beamsplitter. We show how this could be used as a test of local realistic theories by formulating a Bell inequality based on relative phases between the colors.
In parametric downconversion the quantum effects arise because two photons are created from one pump photon. Detection of photons in one train can be used to modify the quantum statistics of the other train to produce antibunched and/or sub-poissonian light. This chapter reports on two experiments of this type. The first employs single photon detection techniques and a fast optical shutter to create antibunched and slightly sub-poissonian light. The second uses analogue detection and feedback to produce sub-poissonian light at picowatt power levels with a Fano factor of 0.78 over a limited bandwidth. Sub-poissonian light is potentially useful in finite dose transmission measurements and the high degree of temporal coincidence of the downconverted photon pairs can be exploited in absolute measurement of detector quantum efficiency. The detailed shape of the fourth order interference effect can be related to the fourier transform of the photon bandwidth determined by the phase matching uncertainty and aperture size.
The quantum theory of fourth-order interference of light is presented in a general format and compared with classical wave theory. The conditions under which nonclassical phenomena occur are discussed. In particular, the interference between the quantum field and classical field may give rise to a nonclassical effect. For some special states of light, the interference pattern does not disappear even though one field is much stronger than the other, for which no classical analog exists. Fourth-order effects in the interference between two independent fields are analyzed in detail. It is pointed out that the fourth-order interference between independent fields will not disappear when the integration time of detection is of the order of the reciprocal bandwidth of the two light fields as long as the spectra of the two fields are symmetric around the same center frequency, and for some correlated fields, the interference does not vanish even if the detection time is much larger than the reciprocal bandwidth of the fields. A new type of fourth-order interference experiment involving a beam splitter is proposed in which local realism of the Einstein-Podolsky-Rosen form is violated for quantum mechanics. This general argument is then applied to the interference between two photons generated in the parametric down-conversion process. The possibility of violations of Bell's inequalities in interference experiments is investigated.
With regard to the system of parametric downconversion, we analyze a recently proposed experiment for demonstrating the nonlocal property of a single photon.1 In the original proposal by Tan et al., a light field in a single photon-number state is split into two beams, which are then homodyned with two spatially separated weak local oscillators. The two-photon detection probability with the two homodyned beams provides evidence for nonlocality. It is shown that this phenomenon is in essence a phase-sensitive fourth-order interference effect. A single photonnumber state can be achieved from the pair of photons produced in parametric downconversion processes.2 A multimode model for the downconversion process is used to carry out the calculation of three-photon detection probability that is associated with nonlocality of a single photon.