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Physical Review A

Quantum theory of fourth-order interference

Z. Y. Ou

Published Mar 1, 1988• 81 citations
Publisher

Abstract

The quantum theory of fourth-order interference of light is presented in a general format and compared with classical wave theory. The conditions under which nonclassical phenomena occur are discussed. In particular, the interference between the quantum field and classical field may give rise to a nonclassical effect. For some special states of light, the interference pattern does not disappear even though one field is much stronger than the other, for which no classical analog exists. Fourth-order effects in the interference between two independent fields are analyzed in detail. It is pointed out that the fourth-order interference between independent fields will not disappear when the integration time of detection is of the order of the reciprocal bandwidth of the two light fields as long as the spectra of the two fields are symmetric around the same center frequency, and for some correlated fields, the interference does not vanish even if the detection time is much larger than the reciprocal bandwidth of the fields. A new type of fourth-order interference experiment involving a beam splitter is proposed in which local realism of the Einstein-Podolsky-Rosen form is violated for quantum mechanics. This general argument is then applied to the interference between two photons generated in the parametric down-conversion process. The possibility of violations of Bell's inequalities in interference experiments is investigated.

DOI
10.1103/physreva.37.1607

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The quantum theory of fourth-order interference of light is presented in a general format and compared with classical wave theory. The conditions under which nonclassical phenomena occur are discussed. In particular, the interference between the quantum field and classical field may give rise to a nonclassical effect. For some special states of light, the interference pattern does not disappear even though one field is much stronger than the other, for which no classical analog exists. Fourth-order effects in the interference between two independent fields are analyzed in detail. It is pointed out that the fourth-order interference between independent fields will not disappear when the integration time of detection is of the order of the reciprocal bandwidth of the two light fields as long as the spectra of the two fields are symmetric around the same center frequency, and for some correlated fields, the interference does not vanish even if the detection time is much larger than the reciprocal bandwidth of the fields. A new type of fourth-order interference experiment involving a beam splitter is proposed in which local realism of the Einstein-Podolsky-Rosen form is violated for quantum mechanics. This general argument is then applied to the interference between two photons generated in the parametric down-conversion process. The possibility of violations of Bell's inequalities in interference experiments is investigated.
A new fourth-order interference experiment has been carried out and analyzed theoretically in classical and in quantum terms. Two photons produced in the process of parametric down-conversion provide the two inputs to a Mach-Zehnder type of interferometer, while two photodetectors coupled to a coincidence counter measure the output. The coincidence rate, after subtraction of accidentals, exhibits a cosine variation with the optical path difference, in agreement with quantum mechanics, but in disagreement with a classical analysis. By contrast, when two coherent light beams from a He:Ne laser are used as inputs to the interferometer, no fourth-order interference is observed.
A theoretical treatment is given of the process in which the two photons produced simultaneously in the parametric frequency splitting of light are allowed to interfere. It is shown that, while there is no interference in the usual sense involving quantities that are of the second order in the field, fourth-order interference effects are present. These may be revealed by measuring the joint probability of detecting two photons at two points x,x' in the interference plane with photoelectric detectors as a function of the separation x-x'. The probability exhibits a cosine modulation with x-x', with visibility that can approach 100%, even though the integration time in the experiment may greatly exceed the reciprocal bandwidth of the photons. The interference effect has a nonclassical origin and implies a violation of local realism in the highly correlated two-photon state.
Although we tend to think of optical interference as a classical wave phenomenon, recent experiments have revealed a number of effects that are not describable in classical terms. This is particularly true of interference effects involving the detection of a photon pair. We shall refer to them as fourth order interference, on the grounds that the joint probability density for the detection of one photon at r sub 1 at time t and another r sub 2 at time t is proportional to the fourth order correlation function of the field. This probability is readily measured when two photodetectors are positioned at r sub 1 and r sub 2 and the signals from the two detectors are fed to a coincidence counter that registers 'simultaneous' detections by the two detectors in coincidence. The topics covered include: fourth order interference measurements; the Franson experiment; and experimental test of the de Broglie guided wave theory.
A new fourth-order interference experiment based on detecting photon pairs in coincidence has been carried out. A Mach-Zehnder type of interferometer is used, with the two photons generated simultaneously in the process of down-conversion as inputs and two photon counting detectors at the two outputs. The optical path difference can be varied piezoelectrically. It is found that the coincidence counting rate, after subtraction of accidentals, exhibits a sinusoidal variation with the optical path difference as predicted by quantum mechanics, but in violation of the laws of classical optics. This is another non-classical interference effeet. By contrast, two light beams derived from a He:Ne laser used as inputs to the interferometer, do not produce any fourth order interference.
A theoretical treatment is given of the situation in which two photons produced in the parametric frequency splitting of light in a nonlinear medium are allowed to interfere. It is shown that there is no interference pattern in the usual sense of quantities that are of the second order in the field, but that fourth-order interference effects are present. These could be demonstrated by placing two photodetectors at positions x,x′ in the interference plane and measuring the joint probability of two detections as a function of x – x′. The probability is predicted to exhibit a cosine modulation with separation x – x′ of close to 100% visibility, even when the integration time in the experiment greatly exceeds the reciprocal bandwidth of the accepted photons. As a result two photons cannot be detected at two points separated by a distance corresponding to an odd number of half-interference fringes. This is an interference effect that violates the laws of classical probability.
In a series of experiments performed by Mandel and co-workers, nonclassical effects have been demonstrated in the interference of two photons generated in a process of parametric down-conversion. The nonclassical effects in the two-photon interference effects can be discussed in the framework of two different descriptions. In the first description, a stochastic theory of electromagnetic field fluctuations can be used in order to calculate the interference pattern. In the second description, a theory of hidden-variable fluctuations can be applied in order to calculate correlations of the interference pattern. A stochastic theory leads to statistical inequalities for the light intensities, while a local hidden-variable theory leads to Bell's inequalities. Using the Schwinger-boson representation of the angular momentum, we show that the two-photon interference effects can be described in terms of spin-correlated states. In particular, we show that the action of a beam splitter on the photons in a parametric down-conversion is equivalent to the production of an entangled state that is very similar to the well-known Einstein, Podolsky, and Rosen spin-singlet state. We show that the stochastic theory of two-photon fluctuations is not equivalent to a hidden-variable theory of photon correlations. We establish a range for which the stochastic theory fails but the hidden-variable theory is still possible. We compare our theoretical predictions with the experimental results and conclude that a violation of the stochastic theory has been clearly observed, while the violation of the hidden-variable theory is less pronounced.