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Physical Review A

Experiment on nonclassical fourth-order interference

Z. Y. Ou, X. Y. Zou, L. J. Wang, L. Mandeļ

Published Sep 1, 1990• 117 citations
Publisher

Abstract

A new fourth-order interference experiment has been carried out and analyzed theoretically in classical and in quantum terms. Two photons produced in the process of parametric down-conversion provide the two inputs to a Mach-Zehnder type of interferometer, while two photodetectors coupled to a coincidence counter measure the output. The coincidence rate, after subtraction of accidentals, exhibits a cosine variation with the optical path difference, in agreement with quantum mechanics, but in disagreement with a classical analysis. By contrast, when two coherent light beams from a He:Ne laser are used as inputs to the interferometer, no fourth-order interference is observed.

DOI
10.1103/physreva.42.2957

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A new fourth-order interference experiment has been carried out and analyzed theoretically in classical and in quantum terms. Two photons produced in the process of parametric down-conversion provide the two inputs to a Mach-Zehnder type of interferometer, while two photodetectors coupled to a coincidence counter measure the output. The coincidence rate, after subtraction of accidentals, exhibits a cosine variation with the optical path difference, in agreement with quantum mechanics, but in disagreement with a classical analysis. By contrast, when two coherent light beams from a He:Ne laser are used as inputs to the interferometer, no fourth-order interference is observed.
A new fourth-order interference experiment based on detecting photon pairs in coincidence has been carried out. A Mach-Zehnder type of interferometer is used, with the two photons generated simultaneously in the process of down-conversion as inputs and two photon counting detectors at the two outputs. The optical path difference can be varied piezoelectrically. It is found that the coincidence counting rate, after subtraction of accidentals, exhibits a sinusoidal variation with the optical path difference as predicted by quantum mechanics, but in violation of the laws of classical optics. This is another non-classical interference effeet. By contrast, two light beams derived from a He:Ne laser used as inputs to the interferometer, do not produce any fourth order interference.
A two-photon interference experiment is presented in which an entangled pair of photons generated from a parametric down-conversion was incident on two input ports of a Mach-Zehnder interferometer. The experiment was carried out using two photon coincidence detection with two detectors at the two output ports of the interferometer. The measured coincidence counts exhibit an interference effect with visibility of 0.75 at simultaneous inputs and 0.38 at inputs with different arrival times according to the degree of photon number entanglement.
Pairs of 826.8-nm correlated photons, generated by parametrically down-converting 413.4-nm krypton-ion laser light, are directed into a single Mach-Zehnder interferometer such that each photon of the pair enters a different input port. The rate of coincidence at the two output ports displays oscillations (as the path-length difference is swept) with a spatial period equal to the 413-nm wavelength of the pump photons, and with a visibility of 62% when the path-length difference exceeds the coherence length of the individual photon beams. This unequivocally demonstrates the nonclassical and entangled nature of the two-photon state.
By using an intensity correlation, or photon coincidence, technique and a Mach-Zehnder interferometer with artificially applied phase fluctuations in one arm, we measured the coherence time of a thermal light beam. The light was derived from the filtered fluorescence of a rhodamine 6G dye solution. The two-photon coincidence rate was measured as a function of path difference and was found to dip 50% when the two arms of the interferometer are balanced. The coherence time of ~100 fs is determined from the measured width of the dip and is consistent with the passband of the filters. The method does not require the stability needed in second-order interference measurements, and its time resolution can be much shorter than that of the photodetectors. The theory of this type of fourth-order interference technique is discussed.
Although we tend to think of optical interference as a classical wave phenomenon, recent experiments have revealed a number of effects that are not describable in classical terms. This is particularly true of interference effects involving the detection of a photon pair. We shall refer to them as fourth order interference, on the grounds that the joint probability density for the detection of one photon at r sub 1 at time t and another r sub 2 at time t is proportional to the fourth order correlation function of the field. This probability is readily measured when two photodetectors are positioned at r sub 1 and r sub 2 and the signals from the two detectors are fed to a coincidence counter that registers 'simultaneous' detections by the two detectors in coincidence. The topics covered include: fourth order interference measurements; the Franson experiment; and experimental test of the de Broglie guided wave theory.
A pair of light quanta with different colors (155.9-nm difference in center wavelength) generated from parametric down-conversion was injected collinearly into one input port of a Mach-Zehnder interferometer. Coincidence interference behavior was studied over a wide range of optical path differences of the interferometer. A measurement of 75% interference visibility with oscillation of the pump frequency for a large optical path difference of the interferometer (43 cm) is the signature of a quantum two-photon entangled state, which reflects both particle and wave nature of the light quanta in one experiment.