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Annual Meeting Optical Society of America

Self-pumped phase conjugation in sodium vapor

Celestino J. Gaeta, Juan Francisco Lam, R. C. Lind

Published Jan 1, 1988• 1 citation
Publisher

Abstract

We have used a two-wave mixing gain process in sodium vapor to construct a self-pumped phase conjugator. This was done by forming a resonator around a quartz sodium cell equipped with Brewster angle windows. A pump beam is then directed into the sodium cell at a small angle to the longitudinal axis of the resonator. At sufficiently high cw pump intensities, the ac-Stark effect pro- vides sufficient gain to achieve oscillation. Although this gain is unidirectional it occurs on the wings of the sodium resonance so that the backward traveling optical field in the resonator does not experience loss due to sodium absorption. The counterpropagating optical fields in the resonator interact with the pump in an internal four- wave mixing process to produce a fourth optical field (phase conjugate to the pump field). Our experiment was conducted at the sodium D2 resonance. The pump laser was a 699 autoscan single frequency ring dye laser providing pump intensities up to several hundred watts per square centimeter.

DOI
10.1364/oam.1988.fl4

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We have used a two-wave mixing gain process in sodium vapor to construct a self-pumped phase conjugator. This was done by forming a resonator around a quartz sodium cell equipped with Brewster angle windows. A pump beam is then directed into the sodium cell at a small angle to the longitudinal axis of the resonator. At sufficiently high cw pump intensities, the ac-Stark effect pro- vides sufficient gain to achieve oscillation. Although this gain is unidirectional it occurs on the wings of the sodium resonance so that the backward traveling optical field in the resonator does not experience loss due to sodium absorption. The counterpropagating optical fields in the resonator interact with the pump in an internal four- wave mixing process to produce a fourth optical field (phase conjugate to the pump field). Our experiment was conducted at the sodium D2 resonance. The pump laser was a 699 autoscan single frequency ring dye laser providing pump intensities up to several hundred watts per square centimeter.
Two spectral regions of gain exist for a weak probe beam propagating through a medium of two-level-atoms pumped by a strong near-resonance field. Experimentally a cw ring-dye laser is used to explore this gain at the Na D₂ resonance in a vapor. Plane-wave calculations of probe-gain spectra which include the Doppler broadening inherent in a vapor agree well with experimental spectra obtained with a Fabry-Perot interferometer. Such two-beam-coupling gain might have applications as optical pre- or power amplifiers. The gain is also the primary step in four-wave-mixing. Mixing of the pump and sideband which experiences gain produces the medium polarization from which the fourth-wave arises. For phase-matched propagation the fourth-wave, which is at a frequency that experiences little or negative probe-gain (i.e., absorption), grows at nearly the same rate as the primary sideband. Together the two sidebands extract far more than twice as much energy from the pump than does the primary sideband acting alone. Experimentally four-wave-mixing which arises from noise at the gain-sideband-frequency is sometimes accompanied by conical emission at the fourth-wave sideband. Since this sideband is also seen on axis the explanation cannot be simply phase-matching. Simulations which include the full transverse nature of the experiment are currently running on a CRAY supercomputer. These simulations indicate that the radial variation of the medium index of refraction is responsible for conical emission.
Summary form only given. Previously, we have used four-wave mixing via coherent population trapping to achieve optical phase conjugation (OPC) with high gain, using two dye lasers and a sodium vapor cell. The /spl Lambda/ transition used involved the two hyperfine ground states and one excited state, so that two different optical frequencies were needed to satisfy the two-photon resonant condition between the probe and one of the pump beams. Later, we demonstrated in rubidium that a single hyperfine transition with Zeeman sublevels is enough to achieve OPC with equally high gain, thus eliminating the need for high-frequency sideband generation. However, in order to guarantee that the diffraction from the grating is primarily dispersive, the backward pump beam had to be detuned by about 60 MHz from the probe and the forward pump. One of the key disadvantages of such a nondegenerate scheme is that applications such as phase-conjugate mirrors are hard to implement. Here, we report the observation of optical phase conjugation in rubidium with equally high gain, but all the frequencies are degenerate.
There is presently a growing interest in nearly degenerate four-wave mixing, both for application in optical phase conjugation and the generation of squeezed states. In particular, the self-oscillation of a system interacting with one or two pump beams has been investigated in great detail in the case of photorefractive materials, but very few experiments have been done in vapors in the cw regime. The results that we obtained using sodium are presented here. They are strikingly different from the results obtained with photorefractive materials. For example, the oscillating beam and pump beam frequencies coincide with a precision better than 10−2 Hz. Another interesting aspect of this oscillating beam is that it exhibits a phase sensitive noise: just above threshold, the noise on one quadrature of the field can be 10−2 times smaller than the noise on the other quadrature.
Investigations of self-pumped phase conjugation using Brillouin-enhanced four-wave mixing in TiCl4 at 1 μm are presented. We have (1) observed both forward and backward Brillouin scattering into the optical cavity used for self-pumped phase conjugation during a single pump laser pulse and enhanced the forward-scattered component relative to the backward-scattered component by changing the angle of incidence of the pump beam, (2) demonstrated up to 80% coupling of pump radiation into cavity radiation, (3) examined quenching of the radiation in the optical cavity and eliminated both multiple Stokes orders from Brillouin scattering and Raman scattering as possible mechanisms, (4) observed mode beating in the cavity intensity profile coincident with the quenching, and (5) studied ring-resonator geometries, demonstrating both forward and backward scattering, unidirectional oscillation, and bidirectional oscillation leading to a triple-shifted phase conjugate.