We present a new method of spectroscopy for atoms cooled and trapped in an optical lattice. This method which makes use of coherent transients permit to improve the signal to noise ratio by more than one order of magnitude by comparison with the previous optical detection methods such as probe transmission or atomic fluorescence [1]. We apply this method to the spectroscopy of cesium atoms first in a four-beam lattice [2] and second in a quasi-periodic structure obtained by adding supplementary incident beams. These structures are strongly connected with the field of quasi-crystals [3] which is very active in solid-state physics. Because of the topological invariance of the optical potential, the same spectra are obtained whatever the phases of the incident beams. Additional information about distribution of atoms among the potential wells can be deduced from the analysis of the coherent transients.
We present a new method of spectroscopy for atoms cooled and trapped in an optical lattice. This method which makes use of coherent transients permit to improve the signal to noise ratio by more than one order of magnitude by comparison with the previous optical detection methods such as probe transmission or atomic fluorescence [1]. We apply this method to the spectroscopy of cesium atoms first in a four-beam lattice [2] and second in a quasi-periodic structure obtained by adding supplementary incident beams. These structures are strongly connected with the field of quasi-crystals [3] which is very active in solid-state physics. Because of the topological invariance of the optical potential, the same spectra are obtained whatever the phases of the incident beams. Additional information about distribution of atoms among the potential wells can be deduced from the analysis of the coherent transients.
We use a method based on optical coherent transients to study the vibrational coherence lifetimes of atoms trapped in the potential wells of a near-resonant optical lattice in the oscillating regime. The dependence of the positions and widths of the vibrational Raman resonances of the coherent transient spectra on the intensity, detuning, and geometry of the lattice beams is investigated and the results are compared with theoretical predictions. It is shown that the principal source of broadening of the vibrational Raman resonances is the anharmonicity of the light-shift potential wells. We also perform time-resolved measurements of the vibrational excitation of atoms equilibrating in an optical lattice.
Optical lattices are periodic arrangements of laser cooled atoms trapped in potentials created by the interference of multiple laser beams. In this dissertation, we describe a series of experiments performed using optical lattices that exploit the coherence of atoms and we also look at new ways to cool the atoms. With a sudden shift of the optical lattice, atomic wavepackets can be created that evolve much like a classical particle. Using a photon redistribution technique, we have characterized the oscillation of wavepackets in the anharmonic potential wells. Atoms will quantum mechanically tunnel between lattice sites with a sufficiently shallow potential. Due to the structure of the optical lattices that are used, while the atom is tunneling, its internal angular momentum state must change. We use this change to detect and characterize the tunneling. The change in internal state leads to the formation of a new potential that acts on the atom, which is known as a gauge potential, which does not depend on the light intensity, but depends only on the geometry of the lattice. We have for the first time measured and characterized this gauge potential. Finally, by randomly modulating the lattice potential, we have demonstrated that tunneling can be suppressed. We have shown that an enhancement of the Sisyphus cooling process, which localizes atoms in the wells of an optical lattice, is possible using a bichromatic standing wave. A time of flight technique is used to verify the cooling improvement. We combine the techniques developed in these experiments and apply them to the cooling of the trapped atoms using a feedback mechanism, which is analogous to the well known technique of stochastic cooling in the field of beam physics. Lastly, we have laid the theoretical basis for using the ponderomotive force to create optical lattices for laser cooled Rydberg atoms. Rydberg atoms are attractive because of their many extreme properties, and the ability to trap Rydberg atoms into lattice sites will increase the range of experiments and measurements that can be made with them.
A theory of coherent transients is developed in which a sequence of optical pulses is incident on a sample of trapped atoms and gives rise to phase-matched emission from the sample. The trapping potential for the atoms can be state dependent, necessitating a quantum treatment of the center-of-mass motion. A source-field approach is followed, modified to account for the quantized motion of the atoms. The theory is illustrated with two examples, one involving the creation of ground-Rydberg level coherence in an optical lattice and the second Raman coherence between two ground-state sublevels of atoms in a dipole trap. For state-independent potentials, a comparison is made with a theory in which the center-of-mass motion is treated classically.
This thesis describes experiments which investigate ultracold atom \nensembles in an optical lattice. Such quantum gases are powerful models for solid state physics. Several novel methods are demonstrated that probe the special properties of strongly correlated states in lattice potentials. Of these, quantum noise spectroscopy reveals spatial correlations in such states, which are hidden when using the usual methods of probing atomic gases. Another spectroscopic technique makes it possible to demonstrate the existence of a shell structure of regions with constant densities. Such coexisting phases separated by sharp boundaries had been theoretically predicted for the Mott insulating state.\nThe tunneling processes in the optical lattice in the strongly correlated regime are probed by preparing the ensemble in an optical superlattice potential. This allows the time-resolved observation of the tunneling dynamics, and makes it possible to directly identify correlated tunneling processes.\n
An optical lattice is the periodic potential that atoms experience via the ac-Stark shift when they are illuminated by counter-propagating laser beams that form a standing-wave pattern. Optical lattices have been widely used as a versatile platform in cooling, trapping, controlling atoms, and also for the study of a variety of problems in physics. The many-body states of ultracold atoms in optical lattices can be characterized by the quantum-correlations encoded in time-of-flight images. In this thesis, we mainly discuss the use of correlations function as a natural framework for characterizing quantum states in optical lattices.\nThe outline of the thesis is as follows. Chapter 1 gives a brief introduction to optical lattice potentials and ways for describing particles moving in a periodic potential. Chapter 2 explains the importance of correlations and discusses common methods to detect them in cold atom experiments.\nChapter 3 presents work done to study the many-body Schrödinger equation in a quasiperiodic potential and discusses its connection with the Kolmogorov-Arnold-Moser (KAM) problem of classical mechanics. We posed a possible visualization of such a connection in experimentally accessible many-body observables. These observables are useful probes for the three characteristic phases of the problem: the metallic, Anderson, and band-insulator phases. In addition, they exhibit fingerprints of nonlinear phenomena such as bifurcations and devil's staircases. Our numerical treatment is complemented with a perturbative analysis that provides insight on the underlying physics. The perturbative-theory approach is particularly useful in illuminating the distinction between the Anderson-insulator and the band-insulator phases in terms of paired sets of dimerized states.\nChapter 4 discusses several theoretical procedures developed to understand a recent experiment on macroscopic quantum self-trapping (ST) performed in a 2D optical lattice. Mean field and truncated-Wigner-approximation (TWA) calculations are performed trying to reproduce the experimental observations. The discrepancy between the theory and the experiment lead to the hypothesis of a new type of ST caused by strong correlations. We analyze toy models to support it.
A complete laser cooling setup was built, with focus on threedimensional near-resonant optical lattices for cesium. These consist of regularly ordered micropotentials, created by the interference of four laser beams. One key feature of optical lattices is an inherent ”Sisyphus cooling” process. It efficiently extracts kinetic energy from the atoms, leading to equilibrium temperatures of a few µK. The corresponding kinetic energy is lower than the depth of the potential wells, so that atoms can be trapped. We performed detailed studies of the cooling processes in optical lattices by using the time-of-flight and absorption-imaging techniques. We investigated the dependence of the equilibrium temperature on the optical lattice parameters, such as detuning, optical potential and lattice geometry. The presence of neighbouring transitions in the cesium hyperfine level structure was used to break symmetries in order to identify, which role “red” and “blue” transitions play in the cooling. We also examined the limits for the cooling process in optical lattices, and the possible difference in steady-state velocity distributions for different directions. Moreover, in collaboration with ´Ecole Normale Sup´erieure in Paris, numerical simulations were performed in order to get more insight in the cooling dynamics of optical lattices. Optical lattices can keep atoms almost perfectly isolated from the environment and have therefore been suggested as a platform for a host of possible experiments aimed at coherent quantum manipulations, such as spin-squeezing and the implementation of quantum logic-gates. We developed a novel way to trap two different cesium ground states in two distinct, interpenetrating optical lattices, and to change the distance between sites of one lattice relative to sites of the other lattice. This is a first step towards the implementation of quantum simulation schemes in optical lattices.