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Annual Meeting Optical Society of America

Quantum correlation and absorption spectroscopy in an optical parametric oscillator

N. C. Wong, K. W. Leong, Jeffrey H. Shapiro

Published Jan 1, 1990• 0 citations
Publisher

Abstract

We have carried out a linearized quantum analysis of the steady-state operation of an optical parametric oscillator (OPO) without cavity detunings; our analysis emphasizes the effects of pump quantum noise and pump excess noise. We show that pump excess noise reduces the observable signal/idler intensity correlation at low frequencies only in the presence of a cavity-loss mismatch between these subharmonic waves. This effect is so strong that the combination of pump excess noise and cavity-loss mismatch explains the rapid low-frequency noise increase well above the shot-noise level that has been seen in recent signal/idler correlation measurements. Moreover, the critical dependence of intensity correlation on cavity-loss mismatch opens a new possibility for ultrasensitive intracavity absorption spectroscopy. Specifically, sinusoidal amplitude modulation of the OPO pump beam with lock-in amplification of the signal/idler photocurrent affords a sensitive probe of subharmonic cavity-loss mismatch. Although this robust measurement capability exploits the strong intracavity correlation between the signal and idler waves, it does not require that nonclassical correlation be externally observable, nor is it limited to near-threshold OPO operation.

DOI
10.1364/oam.1990.mc6

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We have carried out a linearized quantum analysis of the steady-state operation of an optical parametric oscillator (OPO) without cavity detunings; our analysis emphasizes the effects of pump quantum noise and pump excess noise. We show that pump excess noise reduces the observable signal/idler intensity correlation at low frequencies only in the presence of a cavity-loss mismatch between these subharmonic waves. This effect is so strong that the combination of pump excess noise and cavity-loss mismatch explains the rapid low-frequency noise increase well above the shot-noise level that has been seen in recent signal/idler correlation measurements. Moreover, the critical dependence of intensity correlation on cavity-loss mismatch opens a new possibility for ultrasensitive intracavity absorption spectroscopy. Specifically, sinusoidal amplitude modulation of the OPO pump beam with lock-in amplification of the signal/idler photocurrent affords a sensitive probe of subharmonic cavity-loss mismatch. Although this robust measurement capability exploits the strong intracavity correlation between the signal and idler waves, it does not require that nonclassical correlation be externally observable, nor is it limited to near-threshold OPO operation.
We have constructed a mode-locked optical parametric oscillator (OPO), synchronously pumped by the second harmonic of a continuously mode-locked Nd:YAG laser and based on type II phase matching in a KTP crystal. The two subharmonics (signal and idler waves) are nearly degenerate in frequency but are distinct orthogonal polarization states, and the oscillator is thus a nondegenerate OPO. Above threshold, the intensities of the signal and idler output beams should be highly correlated, as recently demonstrated for a similar single-frequency OPO.1 Ideally, the quantum noise on the corresponding photocurrent difference signal is completely suppressed for frequencies that are small compared to the OPO cavity bandwidth. Since this configuration produces intense light beams with potentially very good noise suppression, it is an important prototype for possible applications, e.g., to spectroscopy. Initial results with our OPO show an excess uncorrelated polarization noise, possibly due to depolarized light scattering in the KTP crystal. When the OPO cavity is stabilized with the signal and idler degenerate in frequency, they can be mixed to form a superposition by manipulating their polarization. When the oscillator is pumped below threshold, a pulsed squeezed vacuum state is produced in two such mixtures.2 When the polarizations are mixed inside the OPO cavity by a Faraday rotator, the backaction evasion necessary for a quantum nondemolition (QND) measurement of one of the field quadratures of an externally injected beam is obtained.3 The pulsed local oscillator used in observing the squeezing or QND effects is derived from the fundamental output of the pump laser. Progress in implementing these experiments with our mode-locked OPO is described as well as possible applications to time-domain measurements with noise below the shot-noise limit.
We perform a theoretical analysis of steady-state solutions and quantum noise in a below-threshold optical parametric oscillator (OPO) operating as an amplifier with an input seed wave. Both the amplitude-squeezed and phase-squeezed states of the output field are considered. We take into account the intracavity nonlinear losses due to intracavity frequency doubling of the signal wave and the quantum fluctuations of the seed and pump waves. Unlike the preceding theoretical studies of the problem, we show that squeezing in bright beams produced by the OPO depends on their intensity. For the amplitude-squeezed state, squeezing strongly degrades with increasing output intensity. In contrast, one can obtain good squeezing for phase-squeezed beams of high output intensity.
A quantum analysis of the intensity fluctuations is given for the nondegenerate parametric oscillator both above and below threshold. Theoretical analysis and experiments by Heidmann, Horowicz, Reynaud, Giacobino, and Fabre [Phys. Rev. Lett. 59, 2555 (1987)] have shown that a noise suppression below the vacuum level is possible in the difference of the intensities of the signal and idler modes. The effect of nonequal cavity decay rates and intracavity losses is shown to modify significantly the fluctuation spectra for the difference in the intensity of the signal and idler beams. The results of exact nonlinear solutions for the internal cavity modes are discussed. We demonstrate that a very sensitive absorption detector may be made by operating the oscillator near threshold.
The dependence of quantum correlations of twin beams on the pump finesse of an optical parametric oscillator is studied via a semi-classical analysis. It is found that the phase-sum correlation of the output signal and idler beams from an optical parametric oscillator operating above threshold depends on the finesse of the pump field when the spurious pump phase noise generated inside the optical cavity and the excess noise of the input pump field are involved in the Langevin equations. The theoretical calculations can explain the previously experimental results quantitatively.
Optical parametric amplifiers (OPA's) and optical parametric oscillators (OPO's) can exhibit squeezed amplification when an injected signal beam is used to elicit small-signal gain saturation. This paper extends previous work on OPA/OPO noise behavior under signal injection. Doubly resonant and triply resonant, single-ended cavities are considered in the good-cavity limit. Owing to the nonlinear coupling between the signal and idler beams within the cavity, both are sensitive to the detuning of each beam from its respective resonance. Signal and idler output noise spectra are found by linearizing the quantum coupled-mode equations about the classical mean-field solutions. Cavity detunings lead to frequency dependent phase shifts between the low-noise and high-noise quadratures of both the signal and idler beams. Moreover, the phase of the low-noise quadrature need not coincide with that of the corresponding mean field. The resulting large-signal, signal-to-noise ratio improvement afforded by squeezed amplification is therefore sensitive to the cavity detunings. The effects of classical excess noise on the pump beam and the injected signal beam are also considered.