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Annual Meeting Optical Society of America

Mechanism of inversionless amplification in four-level atoms with Raman pumping

Heide Doss, Olga A. Kocharovskaya, C. H. Keitel, S.-Y. Zhu, L. M. Narducci, Marlan O. Scully

Published Jan 1, 1992• 0 citations
Publisher

Abstract

Two essentially different mechanisms are known for inversionless amplification. The first is based on coherent population trapping, while the second is connected with the existence of quantum interference effects among dressed states of the coupled atom-field system. Previous investigations of four-level atoms with Raman pumping have emphasized the existence of noninversion lasing by way of the first mechanisms and have interpreted the gain as a result of a population inversion between dressed states. In this case the quantum interference generally hinders the amplification process. By extending this analysis to a broader range of parameters we find that the second mechanism can also become effective. The purpose of this presentation is to show that four-level atoms with a Raman pump can generally support both amplification mechanisms and to define the conditions under which either process may dominate.

DOI
10.1364/oam.1992.tujj4

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Annual Meeting Optical Society of America•Jan 1, 1991•0 citations
Two essentially different mechanisms are known for inversionless amplification. The first is based on coherent population trapping, while the second is connected with the existence of quantum interference effects among dressed states of the coupled atom-field system. Previous investigations of four-level atoms with Raman pumping have emphasized the existence of noninversion lasing by way of the first mechanisms and have interpreted the gain as a result of a population inversion between dressed states. In this case the quantum interference generally hinders the amplification process. By extending this analysis to a broader range of parameters we find that the second mechanism can also become effective. The purpose of this presentation is to show that four-level atoms with a Raman pump can generally support both amplification mechanisms and to define the conditions under which either process may dominate.
We analyze the physical origin of the inversionless amplification in four-level atoms driven by a Raman field and identify the existence of two different mechanisms for the predicted gain. The first mechanism is connected with the appearance of a population inversion between the atomic states dressed by the coherent pump, while the second is linked to the buildup of coherence among these states. Proper selection of the relaxation parameters can make either the first or the second mechanism dominant over the other although usually both coexist.
This thesis is concerned with the amplification of coherent radiation from an active medium under conditions which require no population inversion between the energy levels. Gain without population inversion may be obtained by creating a sufficiently strong correlation between pairs of atomic states, usually with the help of external sources of resonant electromagnetic radiation. Our main objective is to investigate two possible selections for the active medium: a three level atom in a lambda configuration and a Raman-driven four level model. For both we identify the conditions that lead to inversionless laser action, we calculate the small signal gain and investigate the physical mechanisms which are responsible for the emergence of gain. While the ultimate cause of the gain is quantum interference, we propose attractive alternative pictures based on the dressed states of the coupled atom-driving field systems. We address the important practical issue of the effect of atomic motion and related Doppler broadening on the inversionless gain profile and we also analyze the transient response of each laser model with the help of the appropriate Maxwell-Bloch equations. Finally we develop a fully quantum mechanical description of the lambda model and find that the radiated field can display unique quantum features which manifest themselves with sub-Poissonian photon fluctuations.
We show lasing without population inversion in a closed four-level atomic system which is no longer incoherently pumped on the transition at which lasing occurs. The four-level system can overcome some limits in the typical lambda-type and V-type three-level systems, furthermore it is possible to achieve lasing even in the absence of the inversion condition for the thermal radiation fields or of the inversion of spontaneous decay rate. We find that when the detuning of probe field is equal to that of coherent coupling field, there is a peak value along with the increase of the detuning. To explain it, we bring forward that there are adiabatic and nonadiabatic stimulated Raman processes when a three-level atomic system is interacted with two coherent fields, so there are two mechanisms influencing the change of probe field. We believe that it can explain more general lasing without inversion processes because of quantum interference induced by coherent fields.
Considerable attention has been directed recently to the study of lasing without the need of population inversion. The optical coherence and quantum interference associated with the light amplification may lead to interesting statistical properties in inversionless lasers. Here we analyze a laser model that consists of an ensemble of closed multi-level (three or four levels) atoms driven by a single coherent field. Unlike conventional lasers where population inversion is maintained and kept at the threshold value for arbitrary laser output, the multi-level laser analyzed here can start lasing from population inversion and evolves from population inversion into non-inversion with the increasing atomic pumping. In other words, the system makes transition from light amplification by population inversion into light amplification by coherence. On the other hand, the system can be also made to start lasing without population inversion in any state basis. In both cases, initial inversion and non-inversion, which are controlled by the ratio of spontaneous decay rates, the laser well above threshold is always maintained by lasing without inversion (light amplification by coherence), and the laser intensity fluctuations may drop below the shot noise limit. Two factors contribute to the noise reduction: first, the disappearance of the population inversion leads to the depleted atomic population in the upper lasing state, which reduces the spontaneous emission noises; second, the fast coherent cycling of electrons between excited states leads to the highly regulated absorption and emission processes. We found that the combination of these two mechanisms can lead to the noise reduction in the laser output more than 50% below the shot-noise limit.
We consider a four-level atomic system with a degenerate or quasidegenerate ground-state doublet and two excited states. One of the upper levels is coupled to the ground doublet by a coherent field of variable strength, which we refer to as the Raman field, whose role is to create atomic coherence between the driven atomic states. The other higher lying state is coupled to the ground states when laser action develops. This model includes an incoherent pump mechanism to create some population in the top lasing state. In appropriate conditions, for the incoherent pump rate and the Raman field strength, the absorption profile of the laser transition develops gain features. We discuss the physical origin of this gain which we find to be the consequence of a population inversion between dressed atomic states. It is interesting to compare the results of this analysis with a similar study of a three-level lambda system which was previously recognized to yield lasing without inversion.1 In this case the appearance of gain can be attributed to the induced atomic coherence.