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Theory of lasing without population inversion

Heide Doss, Lorenzo M. Narducci

Published Jan 1, 1992• 1 citation
Publisher

Abstract

This thesis is concerned with the amplification of coherent radiation from an active medium under conditions which require no population inversion between the energy levels. Gain without population inversion may be obtained by creating a sufficiently strong correlation between pairs of atomic states, usually with the help of external sources of resonant electromagnetic radiation. Our main objective is to investigate two possible selections for the active medium: a three level atom in a lambda configuration and a Raman-driven four level model. For both we identify the conditions that lead to inversionless laser action, we calculate the small signal gain and investigate the physical mechanisms which are responsible for the emergence of gain. While the ultimate cause of the gain is quantum interference, we propose attractive alternative pictures based on the dressed states of the coupled atom-driving field systems. We address the important practical issue of the effect of atomic motion and related Doppler broadening on the inversionless gain profile and we also analyze the transient response of each laser model with the help of the appropriate Maxwell-Bloch equations. Finally we develop a fully quantum mechanical description of the lambda model and find that the radiated field can display unique quantum features which manifest themselves with sub-Poissonian photon fluctuations.

DOI
10.17918/00000666

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We consider a four-level atomic system with a degenerate or quasidegenerate ground-state doublet and two excited states. One of the upper levels is coupled to the ground doublet by a coherent field of variable strength, which we refer to as the Raman field, whose role is to create atomic coherence between the driven atomic states. The other higher lying state is coupled to the ground states when laser action develops. This model includes an incoherent pump mechanism to create some population in the top lasing state. In appropriate conditions, for the incoherent pump rate and the Raman field strength, the absorption profile of the laser transition develops gain features. We discuss the physical origin of this gain which we find to be the consequence of a population inversion between dressed atomic states. It is interesting to compare the results of this analysis with a similar study of a three-level lambda system which was previously recognized to yield lasing without inversion.1 In this case the appearance of gain can be attributed to the induced atomic coherence.

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The emergence of laser action from an atomic system without population inversion is beginning to attract theoretical and experimental attention as a possible way of generating useful coherent radiation at unusual wavelengths. The goal of this communication is to clarify the physical origin of this phenomenon using a four-level system whose ground state consists of two quasidegenerate levels that are coupled to a higher-lying state by a Raman-like transition. In the presence of the ground-state coherence induced by the Raman field, we calculate the absorption spectrum of a weak probe whose tunable frequency scans across the transition frequencies between the two ground-state levels and another higher-lying state that may or may not be weakly excited by an incoherent pump mechanism. Our calculation, based on a dressed atomic state approach, clarifies the conditions that must be satisfied to produce gain, identifies the frequency (or frequencies) at which the gain is maximum, and elucidates the functions of the incoherent pump, the Raman field, and the coherence between the ground-state levels in this process. An appropriate set of Maxwell- Bloch equations for a ring-cavity model of this system confirms the appearance of laser action when the small-signal gain conditions are satisfied.

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Journal of Optics B Quantum and Semiclassical Optics•Jun 1, 2000•22 citations
This thesis is concerned with the amplification of coherent radiation from an active medium under conditions which require no population inversion between the energy levels. Gain without population inversion may be obtained by creating a sufficiently strong correlation between pairs of atomic states, usually with the help of external sources of resonant electromagnetic radiation. Our main objective is to investigate two possible selections for the active medium: a three level atom in a lambda configuration and a Raman-driven four level model. For both we identify the conditions that lead to inversionless laser action, we calculate the small signal gain and investigate the physical mechanisms which are responsible for the emergence of gain. While the ultimate cause of the gain is quantum interference, we propose attractive alternative pictures based on the dressed states of the coupled atom-driving field systems. We address the important practical issue of the effect of atomic motion and related Doppler broadening on the inversionless gain profile and we also analyze the transient response of each laser model with the help of the appropriate Maxwell-Bloch equations. Finally we develop a fully quantum mechanical description of the lambda model and find that the radiated field can display unique quantum features which manifest themselves with sub-Poissonian photon fluctuations.
We consider a four-level atomic system with a degenerate or quasidegenerate ground-state doublet and two excited states. One of the upper levels is coupled to the ground doublet by a coherent field of variable strength, which we refer to as the Raman field, whose role is to create atomic coherence between the driven atomic states. The other higher lying state is coupled to the ground states when laser action develops. This model includes an incoherent pump mechanism to create some population in the top lasing state. In appropriate conditions, for the incoherent pump rate and the Raman field strength, the absorption profile of the laser transition develops gain features. We discuss the physical origin of this gain which we find to be the consequence of a population inversion between dressed atomic states. It is interesting to compare the results of this analysis with a similar study of a three-level lambda system which was previously recognized to yield lasing without inversion.1 In this case the appearance of gain can be attributed to the induced atomic coherence.
The emergence of laser action from an atomic system without population inversion is beginning to attract theoretical and experimental attention as a possible way of generating useful coherent radiation at unusual wavelengths. The goal of this communication is to clarify the physical origin of this phenomenon using a four-level system whose ground state consists of two quasidegenerate levels that are coupled to a higher-lying state by a Raman-like transition. In the presence of the ground-state coherence induced by the Raman field, we calculate the absorption spectrum of a weak probe whose tunable frequency scans across the transition frequencies between the two ground-state levels and another higher-lying state that may or may not be weakly excited by an incoherent pump mechanism. Our calculation, based on a dressed atomic state approach, clarifies the conditions that must be satisfied to produce gain, identifies the frequency (or frequencies) at which the gain is maximum, and elucidates the functions of the incoherent pump, the Raman field, and the coherence between the ground-state levels in this process. An appropriate set of Maxwell- Bloch equations for a ring-cavity model of this system confirms the appearance of laser action when the small-signal gain conditions are satisfied.
In this paper, a quantum theory of an inversionless laser is presented. The gain medium is considered to consist of three-level atoms in a closed \ensuremath{\Lambda} configuration, with a lower-level microwave coupling. By deriving an equation of motion for the reduced density matrix for the two modes of the field, gain and diffusion are studied. In particular, two mechanisms through which inversionless amplification takes place in the context of this model, namely, the suppression of absorption and mode coupling, are discussed. Stable conditions for inversionless amplification and the attendant phase diffusion are discussed and a comparison is made with conventional, inversion-based lasers. It is shown that lasing without inversion does not necessarily result in a reduced linewidth compared to a conventional laser.
Summary form only given. We study a model for an incoherently pumped laser operating with a Doppler-broadened three-level system placed in a doubly resonant cavity and producing two laser fields, one of them without population inversion. Each laser field couples to only one of the transitions of the three-level medium. We have studied our model for parameters appropriate to two real atomic systems (i) a cascade scheme in atomic /sup 138/Ba looking for lasing with (without) inversion at /spl lambda//sub /spl beta//=554 nm (/spl lambda//sub /spl alpha//=821 nm), and (ii) a V-scheme in atomic /sup 85/Rb with ordinary lasing at /spl lambda//sub /spl alpha//=780 nm and lasing without inversion (LWI) at /spl lambda//sub /spl alpha//=4216 nm. These two cases are qualitatively different in that two-photon processes are responsible for inversionless gain in case (i) while LWI in case (ii) arises from one-photon processes. Moreover, the frequency up-conversion ratio is R=0.67 for the case of /sup 138/Ba and it is R=1.88 for the case of /sup 85/Rb. In spite of the fact that the frequencies of the two laser fields are relatively different, our results show that dual-wavelength lasing extends up to Doppler broadening values typical for optical transitions of atoms in a vapor cell. In case (i) /spl alpha/-lasing occurs without two-photon inversion only for approximately the lower half of the domain of Doppler-broadening values. However, in case (ii) one has LWI in all the domains. Some considerations for a practical realization of the dual-wavelength inversionless-conventional laser are discussed.
Two essentially different mechanisms are known for inversionless amplification. The first is based on coherent population trapping, while the second is connected with the existence of quantum interference effects among dressed states of the coupled atom-field system. Previous investigations of four-level atoms with Raman pumping have emphasized the existence of noninversion lasing by way of the first mechanisms and have interpreted the gain as a result of a population inversion between dressed states. In this case the quantum interference generally hinders the amplification process. By extending this analysis to a broader range of parameters we find that the second mechanism can also become effective. The purpose of this presentation is to show that four-level atoms with a Raman pump can generally support both amplification mechanisms and to define the conditions under which either process may dominate.
We study propagation effects on lasing without population inversion in a Doppler-broadened V -type three-level system. In particular, we focus our analysis on frequency up-conversion lasing without inversion in atomic rubidium. In an atomic beam configuration, we show that it is possible to increase notably the probe gain per single pass through the active medium by detuning driving and probe fields out of one-photon resonance but maintaining the two-photon resonance condition. In a vapour cell configuration, we show that due to propagation effects the probe gain per single pass depends strongly on the driving field intensity at the entrance of the active medium. In fact, for appropriate parameter values, it is possible to reach values of the probe gain per single pass of around 40%. For this last case, we have considered the feedback of a ring laser cavity.