The interaction of light and matter can be described by a set of coupled nonlinear evolution equations for the material and electromagnetic fields. In order to account for the effects of vacuum fluctuations, noise forces which cause spontaneous transitions have to be included. In these macroscopic systems various sources of noise besides fundamental quantum fluctuations exist which are of macroscopic origin. These cause fluctuations of the cavity dissipation as well as of the external pumping power. In the course of an adiabatic elimination procedure, these fluctuations appear as multiplicative noise in the equations of motion (e.g. for the field intensity, due to the nonlinearity of the interaction). While fluctuations of the cavity damping create noise linear in the field intensity, randomness in the pump strength causes fluctuations that depend nonlinearly on the light intensity. In this respect, the noise terms enter the equations of motion quite differently and have to be distinguished from spontaneous emission noise which is independent of the field strength, and is the basis of all traditional laser models.
The interaction of light and matter can be described by a set of coupled nonlinear evolution equations for the material and electromagnetic fields. In order to account for the effects of vacuum fluctuations, noise forces which cause spontaneous transitions have to be included. In these macroscopic systems various sources of noise besides fundamental quantum fluctuations exist which are of macroscopic origin. These cause fluctuations of the cavity dissipation as well as of the external pumping power. In the course of an adiabatic elimination procedure, these fluctuations appear as multiplicative noise in the equations of motion (e.g. for the field intensity, due to the nonlinearity of the interaction). While fluctuations of the cavity damping create noise linear in the field intensity, randomness in the pump strength causes fluctuations that depend nonlinearly on the light intensity. In this respect, the noise terms enter the equations of motion quite differently and have to be distinguished from spontaneous emission noise which is independent of the field strength, and is the basis of all traditional laser models.
The basic equations governing noise phenomena are derived from first principles and applied to examples in optical communications. Quantum noise arises from two sources, the momentum fluctuations of electrons at optical frequencies and the uncertainty-related fluctuations of the electromagnetic field. Shot noise results from the beating of the noise sources with the signal field. In high-gain amplifiers, the spontaneous-emission noise dominates shot noise and results in a noise figure of at least 3 dB. It is shown explicitly how, at high power, both the laser field and the laser noise source become classical. The increase in noise in lasers with open cavities is not due to enhanced spontaneous emission as once thought, but to single-pass amplification. The noise fields and spontaneous currents have Gaussian distributions, while nonlasing modes have exponential photon-number distributions. Low-frequency intensity fluctuations arise from the electric current driving the laser and can be sub-Poissonian, in contrast to shot noise, which has a Poissonian distribution. The calculational tools are a wave equation for the field operator and a rate equation for the carrier-number operator, each containing spontaneous current noise sources. The correlation functions of these sources are determined by the fluctuation-dissipation theorem. [S0034-6861(96)00503-X]
Abstract This book is an introduction to quantum optics for students who have studied electromagnetism and quantum mechanics at an advanced undergraduate or graduate level. It provides detailed expositions of theory with emphasis on general physical principles. Foundational topics in classical and quantum electrodynamics, including the semiclassical theory of atom-field interactions, the quantization of the electromagnetic field in dispersive and dissipative media, uncertainty relations, and spontaneous emission, are addressed in the first half of the book. The second half begins with a chapter on the Jaynes-Cummings model, dressed states, and some distinctly quantum-mechanical features of atom-field interactions, and includes discussion of entanglement, the no-cloning theorem, von Neumann’s proof concerning hidden variable theories, Bell’s theorem, and tests of Bell inequalities. The last two chapters focus on quantum fluctuations and fluctuation-dissipation relations, beginning with Brownian motion, the Fokker-Planck equation, and classical and quantum Langevin equations. Detailed calculations are presented for the laser linewidth, spontaneous emission noise, photon statistics of linear amplifiers and attenuators, and other phenomena. Van der Waals interactions, Casimir forces, the Lifshitz theory of molecular forces between macroscopic media, and the many-body theory of such forces based on dyadic Green functions are analyzed from the perspective of Langevin noise, vacuum field fluctuations, and zero-point energy. There are numerous historical sidelights throughout the book, and approximately seventy exercises.
Nonlinear optics is a fairly young science, having taken off with the advent of the laser in 1960. Nonlinear optics (NLO) deals with the interaction of electromagnetic waves and matter in the infrared, visible, and ultraviolet domains. The frontiers of NLO are somewhat blurred, but microwaves and γ-rays are clearly outside its domain. This book is entirely devoted to a study of NLO in a resonant cavity and when the quantum nature of the electromagnetic field is not of prime importance. More precisely, we study those aspects of cavity NLO in which fluctuations in the number of photons and atoms are not relevant. This particular area of optics is dominated by the Maxwell–Bloch equations, which constitute its paradigm in the sense of T. S. Kuhn. The status of the Maxwell–Bloch equations is quite peculiar. From a fundamental viewpoint, they describe the laws of evolution of the first moments of a density operator, which verifies the von Neumann equation. However, to account for the finite lifetime of the atoms and of the field in the necessarily lossy cavity, some legerdemains have to be introduced to obtain the Maxwell–Bloch equations. Stated more explicitly, the von Neumann equation for a large but finite system does not explain irreversibility, whereas the Maxwell–Bloch equations fully include the irreversible decay of the atoms and of the cavity field. This problem is not specifically related to optics but reflects the general failure of statistical mechanics to explain convincingly the irreversible evolution of macroscopic systems.
The Dicke model describes the coherent interaction of a laser-driven ensemble of two-level atoms with a quantized light field. It is realized within cavity QED experiments, which in addition to the coherent Dicke dynamics feature dissipation due to, e.g., atomic spontaneous emission and cavity photon loss. Spontaneous emission supports the uncorrelated decay of individual atomic excitations as well as the enhanced collective decay of an excitation that is shared by N atoms and whose strength is determined by the cavity geometry. We derive a many-body master equation for the dissipative Dicke model including both spontaneous emission channels and analyze its dynamics on the basis of Heisenberg-Langevin and stochastic Bloch equations. We find that the collective loss channel leads to a region of bistability between the empty and the superradiant state. Transitions between these states are driven by nonthermal Markovian noise. The interplay between dissipative and coherent elements leads to a genuine nonequilibrium dynamics in the bistable regime, which is expressed via a nonconservative force and a multiplicative noise kernel appearing in the stochastic Bloch equations. We present a semiclassical approach, based on stochastic nonlinear optical Bloch equations, which for the infinite-range Dicke model become exact in the large-N-limit. The absence of an effective free-energy functional, however, necessitates the inclusion of fluctuation corrections with O(1/N) for finite $N<\ensuremath{\infty}$ to locate the nonthermal first-order phase transition between the superradiant and the empty cavity.
Adopting a new classical approach, the additive noise power generated in optical amplifiers is calculated in terms of power spectral density. The classical formalism used combines a coruscular approach to a phase-amplitude description of the optical field. The noise contributions of the input field fluctuations, including zero-point fluctuations, and of the electron momentum fluctuations at optical frequency linked to the amplifier itself, are clearly identified. The excess of noise associated to coupling or built-in losses is determinated. The well-known result of the Amplified Spontaneous Emission (ASE) is obtained for the laser amplifiers. This description is applied to linear phase-insensitive amplifiers and to inhomogeneous, nonlinear phase-insensitive Raman amplifier, pointing out the effects of gain compression and gain distribution. This new approach makes possible the treatment of the squeezed-state of light and the quadrature reduced noise amplifications.
Present-day experiments have started to couple traditional simulations of ultracold atom experiments with quantum light-fields in cavities. This has provided a wealth of op- portunities to enlarge the number of interaction potentials: cavity mediated long-range interactions compete with kinetic energies, longitudinal fields, short-ranged collisional or magnetic spin-spin interactions. The intracavity many-body lattice models often have to be maintained far from equilibrium through the presence of external driving lasers that help to boost and engineer the various interaction potentials. The steady influx of energy is compensated by a steady stream of energy out of the atom-cavity system for example by photon losses or atomic spontaneous emission. Several experiments have demonstrated that such environments can give rise to new competing quantum phases. \nBut this long-standing ambition to push for models with tailorable interaction potentials can bring with it also considerable challenges in their theoretical description, since sponta- neous symmetry breaking transitions in many body lattice systems coupled to dynamical light-fields with single-photon character occur in the presence of drive and dissipation for the photonic force carriers. This clearly calls for model systems where the above men- tioned interplay of interactions, drive, dissipation and cooperative many-body behaviour can be theoretically studied to provide simple, experimentally verifiable predictions. \nThe Dicke model is, through its simplicity (an exactly solved ferromagnet with infinite range atom-atom interactions mediated by a single cavity mode), an exceptionally well- suited candidate. As the generic model for atom-light interactions, it has been experimen- tally realized in a variety of modern quantum optical systems, highlighting its relevance for present-day research. The Dicke model is also highly versatile itself. It has been extended into the dissipative realm, was promoted to account for multiple optical light modes and was used to describe multiple, coupled single-mode cavity structures. It was adapted to treat spin-selective coupling to a cavity to describe superradiance phase tran- sitions in multi-level atomic systems. Moreover, it was realised in electronic circuits where the dipole coupling of real atoms to single mode fields is replaced by a capacitive cou- pling of artificial atoms to a resonator mode. This illustrates that the Dicke model and its extended variants are ’future-proof’ and continue to be of relevance for fundamental light-matter interactions and for driven-dissipative phase transitions. \nIn this thesis, we investigate magnetic phase transitions in driven-dissipative atomic en- sembles interacting with quantum light. We present three research projects on variants of cooperative radiation of an ensemble of laser driven two-level atoms in a single mode optical cavity, as described by the Dicke model. \nThroughout the chapters 2,3 and 4 that contain the main body of research of this thesis, we investigate phase transitions between non-equilibrium stationary states in engineered quantum-optical systems each of which extends the conventional Dicke model physics. As a starting point, we map the quantum equations of motion onto a set of semiclassical nonlinear stochastic equations and analyse their stationary states and instabilities with master equations for atomic spin and photon mean-field amplitudes. These are used to obtain experimentally relevant parameters such as critical atom-light couplings for phase transitions, phase diagrams and properties of stationary non-equilibrium states in addition to cavity output spectra that identify the imprint of magnetic correlations in the light-field. \nIn chapter 2, we help resolve a discrepancy between earlier experimental investigations of the critical atom-light coupling strength for the superradiance transition in the Dicke model: higher external pumping strengths than theoretically predicted were needed to observe a coherent, superradiant state of the light field in an optical cavity. By including incoherent spontaneous emission of atomic excitations, we extend the dissipative Dicke model to a two loss channel variant containing both photon leakage and atomic decay that reproduces the experimentally observed critical atom-light coupling. \nRecent experiments have started to interface quantum many body lattice models with coherent cavity fields, thereby allowing to realize new quantum phases through competing atom-cavity and atom-atom interactions. In chapter 3, we consider a simplified model for such a set-up where a single quantized mode of the light-field interacts with an ensemble of Rydberg-dressed atoms inside a high finesse optical cavity. This model provides a base case for further studies of quantum magnets in optical cavities. At the heart of this model is a competition of short- (dipolar atom-atom) and long-range (atom-light) interactions at the Hamiltonian level in the presence of both spontaneous emission and photon leak- age through the cavity mirrors. We show that different magnetic phases can coexist with coherent atomic radiation and provide clear experimental signatures to identify the mag- netic structure and intra-cavity dynamics. We suggest an experimental level-scheme for a quantum optical implementation of our model. \nIn chapter 4 we consider a generic, collective decay for many-body excitations in the paradigmatic Dicke model. This extension drastically enriches the dynamics as it induces a bicritical point and a bistable regime dominated by true non-equilibrium fluctuations that induce a dissipative first-order phase transition that can only be resolved by including finite fluctuation corrections with the help of stochastic Langevin equations. We investigate the hysteretic response to time-dependent ramps of the atom-light coupling. Discontinuous first-order phase transitions where metastable states coexist in a hysteresis domain have been investigated in recent dissipative quantum-optical experiments. We review noise- activation far from thermal equilibrium in chapter 5.