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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Self-phase conjugation technique via four wave mixing of middle infrared radiation in a laser active medium

Alexander A. Ageichik, Oleg G. Kotyaev, Yu. A. Rezunkov, Alexander L. Safronov, Vladimir V. Stepanov

Published Jan 1, 1996• 0 citations
Publisher

Abstract

As it is known, self-conjugation of the IR laser beam via Brillouin radiation stimulated scattering phenomenon is not realised because of some physical limits on radiation intensity which are the principal limitations, to the present time. That is why, one of the promising technique of phase conjugation of infrared radiation is a self-conjugation of a laser beam wavefront via four wave interaction in a nonlinear medium with feed-back loop (FWMF) [1]. Unlike conventional our wave mixing schemes, the FWMF self-conjugation is supposed to be realised without any additional beams pumping a phase conjugation mirror.

DOI
10.1364/cleo_europe.1996.ctuk37

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As it is known, self-conjugation of the IR laser beam via Brillouin radiation stimulated scattering phenomenon is not realised because of some physical limits on radiation intensity which are the principal limitations, to the present time. That is why, one of the promising technique of phase conjugation of infrared radiation is a self-conjugation of a laser beam wavefront via four wave interaction in a nonlinear medium with feed-back loop (FWMF) [1]. Unlike conventional our wave mixing schemes, the FWMF self-conjugation is supposed to be realised without any additional beams pumping a phase conjugation mirror.
To the best of our knowledge, a novel self-phase-conjugation technique for laser radiation is proposed, which is based on the self-filtration of the phase-conjugate component in a nonlinear absorbing medium, bleached by a pump wave with the intricate spatial structure in the region of location of its speckles. Similar to the stimulated Brillouin scattering (SBS) case, the mechanism of the phase-conjugate wave discrimination against the noise background is based on the coincidence of the speckles in the pump and conjugate waves throughout the bulk of the medium. To compensate for a drop in the signal power due to total absorption, the amplification in conventional laser gain cells is used. The feasibility of the phase conjugation with reflectivities from unity to tens of percent is demonstrated by analytical estimates and numerical calculations. The technique can find application in the middle and far IR spectral regions, where the implementation of phase conjugation via SBS is either hindered or impossible at all.
Nonlinear optics normally involves the change in the susceptibility of a material due to the presence of optical radiation. In many cases, the light-matter interaction produces a change in the refractive index of the medium, as occurs in photorefractive media, as well as in Kerr-like media, Brillouin-active media and absorbing media with thermallyinduced refractive index changes. Such nonlinear refractive index variation corresponds to a change in the real part of the optical susceptibility %. In resonant materials, the optical radiation induces stimulated emission (or absorption) causing transfer of population between different energy states of the medium. This can lead to saturation of the amplification (or absorption) corresponding to changes in the imaginary part of the susceptibility x= i2odk where the amplitude gain coefficient a(I) is a saturable function of the intensity /, and k is the magnitude of the wavevector of the optical radiation. The interference of two (or more) coherent beams I(x) in the laser amplifier can cause a modulation of the population inversion N(x). This modulation of the inversion is commonly known as spatial hole burning in lasers and leads to formation of a gain-grating a(x) = 1/2GN(X) where G is the stimulated emission cross-section. The gain grating can act as a very efficient diffractive optical element exhibiting high diffraction efficiency that may be even greater than unity [16] and also very high phase conjugate reflectivity using four-wave mixing (FWM) geometries [5-7].
Theoretical and experimental investigations were made of a four-wave interaction of middle-infrared radiation based on a thermal nonlinearity of absorbing liquids and gases. A study was made of the influence of parasitic effects associated with heating of a nonlinear medium (such as the thermal lens effect, frequency sweeping of interacting waves, thermal expansion of the medium, and convection) on the efficiency of the four-wave interaction and the quality of phase conjugation utilizing this interaction. The conditions under which this influence is minimal were identified. An experimental study was made of phase conjugation of CO 2 laser radiation by a four-wave interaction in CCl 4 with a high reflection coefficient (up to 20% in the cw regime). The attained phase conjugation was limited the thermal lens effect, but this could be compensated.
Investigations of self-pumped phase conjugation using Brillouin-enhanced four-wave mixing in TiCl4 at 1 μm are presented. We have (1) observed both forward and backward Brillouin scattering into the optical cavity used for self-pumped phase conjugation during a single pump laser pulse and enhanced the forward-scattered component relative to the backward-scattered component by changing the angle of incidence of the pump beam, (2) demonstrated up to 80% coupling of pump radiation into cavity radiation, (3) examined quenching of the radiation in the optical cavity and eliminated both multiple Stokes orders from Brillouin scattering and Raman scattering as possible mechanisms, (4) observed mode beating in the cavity intensity profile coincident with the quenching, and (5) studied ring-resonator geometries, demonstrating both forward and backward scattering, unidirectional oscillation, and bidirectional oscillation leading to a triple-shifted phase conjugate.