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Optics

Recent Progress in Short and Mid-Infrared Single-Photon Generation: A Review

Arianna Elefante, Stefano Dello Russo, Fabrizio Sgobba, Luigi Santamaria Amato, Deborah Katia Pallotti, Daniele Dequal, Mario Siciliani de Cumis

Published Jan 12, 2023• 7 citations
Publisher

Abstract

The generation of single photons in the mid-infrared spectral region is attracting the interest of scientific and technological research, motivated by the potential improvements that many important and emerging applications, such as quantum sensing, metrology and communication, could benefit from. This review reports the progress in short and mid-infrared single photon generation, focusing on probabilistic sources based on the two non-linear processes of spontaneous parametric downconversion (SPDC) and four wave mixing (FWM). On one hand, numerical simulations of mid-infrared SPDC are described as a powerful tool to assist and guide the experimental realization, along with the implementation and engineering of novel non-linear materials. On the other hand, the advantages offered by FWM in silicon waveguides in terms of integration, miniaturization and manufacturability are presented, providing an optimal technology for integrated quantum applications.

DOI
10.3390/opt4010003

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The generation of single photons in the mid-infrared spectral region is attracting the interest of scientific and technological research, motivated by the potential improvements that many important and emerging applications, such as quantum sensing, metrology and communication, could benefit from. This review reports the progress in short and mid-infrared single photon generation, focusing on probabilistic sources based on the two non-linear processes of spontaneous parametric downconversion (SPDC) and four wave mixing (FWM). On one hand, numerical simulations of mid-infrared SPDC are described as a powerful tool to assist and guide the experimental realization, along with the implementation and engineering of novel non-linear materials. On the other hand, the advantages offered by FWM in silicon waveguides in terms of integration, miniaturization and manufacturability are presented, providing an optimal technology for integrated quantum applications.
Single-photon creation through parametric downconversion underpins quantum technology for quantum sensing and imaging. Here we numerically study the creation of single photons in the near- and mid-infrared regime from 1.5 - 12 um in a range of novel nonlinear semiconductor and chalcopyrite materials. We identify phase-matching conditions and single out regimes in which group-velocity matching can be achieved with commercially available pump lasers. Finally, we discuss how mid-infrared single photons can be detected. Using our numerical results, we identify materials and pump lasers for up-conversion detection in conventional wavelength bands. Our study provides a complete recipe for mid-IR single-photon generation and detection, opening up quantum enhancements for mid-IR applications such as bio-medical imaging, communication, and remote sensing.
We report an experimental demonstration of wavelength variable generation and detection of photon pairs in the visible and mid-infrared (MIR) regions over a wide spectral range of 2–5 µm via spontaneous parametric downconversion. Despite the recent increase in interest in such a photon-pair source, there have been few detailed evaluations of emitted photons generated via the downconversion process in the low gain regime, due to the lack of suitable single-photon detectors. By changing the angle of the nonlinear crystal, we continuously tune the phase-matching condition and generate photon pairs as signal photons in the wavelength range of 600–965 nm and idler photons in the wavelength range of 1186–4694 nm. We evaluate the generated photon pairs using single and coincidence counts by superconducting nanowire single-photon detectors up to a wavelength of 2 µm and detect the intensity using an InSb detector with a lock-in detection system up to 5 µm. From this analysis, a pair generation rate of 10 5 s − 1 per mW of pump power is experimentally obtained for this wavelength range. This work provides a basis for the realization of applications such as heralded MIR single-photon sources, infrared imaging, and infrared spectroscopy based on quantum technologies in the MIR region.
Abstract Satellite quantum key distribution technology has developed rapidly using near-infrared wavelengths and is expected to enable global quantum communication. However, link availability is still hampered by detrimental effects in the free-space channel, such as background noise from solar radiation and attenuation from turbulence and weather such as haze and fog. One potential mitigation technique is to move to the mid-infrared atmospheric transmission window (3–5 µ ms) where background noise and turbulence effects are significantly reduced. While mid-infrared quantum technology is not as well developed, advancements in mid-infrared entangled photon pair generation and nonlinear upconversion single-photon detectors could be poised to enable daytime satellite downlinks with increased reliability. This review compares the state of the art for quantum transmitters and receivers in the mid-infrared to the more established near-infrared technology. The goal is to identify gaps in transmitter and/or receiver technology in the mid-infrared, and to determine if the mid-infrared can offer significant advantages over the near infrared for quantum communication.
Sources of quantum correlated photons pairs bridging the 3um-4um Mid-infrared (MIR) band and Telecom/Near-Infrared/Visible band are of high importance for quantum technologies. Spontaneous Parametric Down Conversion is generally used for realizing such sources, but requires costly implementation platforms with reduced versatility. Here, we explore the potentialities of Spontaneous Four-Wave Mixing (SFWM) in all-solid Silicon On Insulator (SOI) waveguides thanks to an experimentally validated model and propose designs ensuring the production of correlated photon pairs bridging the 3um-4um Mid-infrared band and Telecom C-band. Choosing a pump with a wavelength in the range 2100nm-2210nm and a pulse duration of 5ps, we quantitatively performed simulations targeting a probability of photon pair generation per pulse of 0.05, and we found realistic conditions of utilization (2cm-length straight waveguides, intra-modal Four Wave Mixing with the fundamental TE00 mode) with a pump peak power in between 9.2mW and 32mW. A first design (wCOM) reaches a signal wavelength as high as 3.905um, which is situated in an atmospheric transparency window, while maintaining an idler in the Telecom C-band, making it of high interest for atmospheric Quantum Key Distribution. Two other designs wCH4 and wNO2 aim precise CH4 and NO2 gas sensing with a signal wavelength of 3265nm and 3461nm respectively. In terms of signal/idler wavelength separation, wCOM attains the value of 2364nm which is well above the current record of ~1125nm obtained in quantum regime with SFWM in all-solid SOI waveguides.
Metrology with undetected photons is an emerging technique that leverages quantum effects and photon correlations (entanglement) to retrieve valuable information in a target spectral range (e.g., mid-infrared, mid-IR) using measurements in an easily accessible domain (e.g., visible, near-IR). The underlying quantum process of spontaneous parametric down-conversion (SPDC) is utilized to generate non-degenerate correlated signal and idler photons to serve as detection and probing photons, respectively. Sensing with undetected photons enables important advantages, such as ultra-low probe powers, room-temperature operation, and shot-noise-limited detection. In this contribution, we apply a quantum nonlinear interferometer based on an SPDC source to perform applied mid-IR spectroscopy, mid-IR microscopy, and mid-IR optical coherence tomography (OCT) as among the most promising techniques for quantum-based routine non-destructive testing. Moreover, we characterize the system, benchmark it against classical systems, and provide a prospective outlook for this new technology.
Quantum information science has recently attracted a lot of attention. Its applications include secure communication, quantum computation, quantum simulation, and quantum metrology. In these applications, photons are one of the most important physical quanta for their tolerance to decoherence. In this manuscript, we review the recent progress in single-photon/entangled-photon emitters and their applications: heralded single-photon sources using parametric downconversion and their application to quantum key distribution, highly indistinguishable heralded single-photon sources, fiber-coupled solid-state single-photon sources, and ultrabroadband-frequency entanglement generation.