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Journal of Physical & Chemical Research

Analysis of the quasi exact solvable Rydberg dressed atoms interaction model

Nabila Grar, Leila Chia

Published Jun 1, 2022• 0 citations
Publisher

Abstract

The exact solvable model of the Rydberg dressed interaction for twoparticles proposed by Kościk et al. is analyzed in the differentdimensions to single out the impact of the dimensionality. First weanalyze the effect on the energy spectrum then spatial correlations arestudied as the radial density distribution versus the position in the threedimensionalities. The results clarify the effect of the centrifugal forcesin the presence of long range interaction.

DOI
10.58452/jpcr.v1i1.19

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•Jan 1, 2007•1 citation
The exact solvable model of the Rydberg dressed interaction for twoparticles proposed by Kościk et al. is analyzed in the differentdimensions to single out the impact of the dimensionality. First weanalyze the effect on the energy spectrum then spatial correlations arestudied as the radial density distribution versus the position in the threedimensionalities. The results clarify the effect of the centrifugal forcesin the presence of long range interaction.
Exactly solvable model of two Rydberg-dressed atoms moving in a quasi-two-dimensional harmonic trap is introduced and its properties are investigated. Depending on the strength of inter-particle interactions and the critical range of the potential, the two-particle eigenstates are classified with respect to the excitations of the center-of-mass motion, relative angular momentum, and relative distance variable. Having these solutions in hand, we discuss inter-particle correlations as functions of interaction parameters. We also present a straightforward prescription of how to generalize obtained solutions to higher dimensions.
By using a step-like potential, it is possible to mimic the Rydberg short range part of the interaction between two atoms. It is easy in this case to establish an analytical solution of the Schrödinger equation. In this contribution, we are analyzing in detail this simplified model by highlighting the major players in different interaction schemes (strengths and ranges), different dimensionalities and the impact on spatial correlation. We are able to achieve an improvement to this model by applying a perturbation treatment to the potential. The dynamical aspects related to a sudden change of the potential features are also investigated.
Abstract: An analytical solution is possible for the Schrödinger equation for two particles interacting via a step-like potential and confined in a harmonic trap. This model is assumed to be very close to the real case of two confined Rydberg-dressed atoms. In this contribution, we thoroughly examine the validity of this approximation to describe the realistic situation. We analyze in detail the impact of the dimensionality on the spatial correlation of the system. The impact of the dimensionality on the dynamics of the system under a quench scenario is also investigated.
Rydberg-dressed ground state atoms are atoms with an electron off-resonantly excited to a very high energy state, i.e., a state of high principal quantum number n ≫ 1. This thesis investigates the quantum dynamics of interacting Rydberg-dressed ground state atoms trapped in several multi-well potential traps. Rydberg atoms are atoms with exaggerated properties. One of their most interesting properties is that they exhibit a strong and long-ranged interaction that can be tuned leading to a variety of different quantum behaviours. My work focuses on studying the effects of these interacting atoms when loaded in multi-well potential traps. Generally, multi-well systems are considered as the simplest example of a finite optical lattice structure. For this reason, this thesis covers three research topics that examine the effects of long-range interaction on Rydberg-dressed atoms trapped in several potential confinements. I begin, in the introduction, by discussing the theoretical background of relevance to this work. It starts with presenting the physics of Bose-Einstein condensate. Then, the fundamentals of the interaction between two-level atom and light are analytically studied. This study has the purpose of understanding both; the dressed interacting atoms and optical lattices. The definition, characteristics, and the nature of the interaction between Rydberg atoms are analysed afterwards. The second chapter examines the dynamics of an ensemble of interacting Rydberg- dressed atoms trapped in static, i.e., time-independent, multi-well potentials using a mean-field theoretical approach. I choose one-dimensional double- and triple-well in addition to a two-dimensional quadruple-well potentials. The time-dependent non-linear Gross-Pitaevskii equation is used to numerically explore the ensemble’s quantum dynamics. Solving the dynamical differential equations along with tuning the strength of the applied long-range interaction shows that the behaviour of non-interacting Rydberg-dressed atoms does not differ conceptually according to the geometry of the trapping potential. However, this changes when the interactions are switched on where the shape of the confinement leads to interesting outcomes especially in the non-linear interacting limit, such as macroscopic quantum self-trapping. After investigating an ensemble of interacting Rydberg-dressed atoms in static multi-well potential traps, the second research topic examines the dynamical evolution of these atoms when loaded in a finite optical lattice using the extended Bose-Hubbard model. In this chapter, the atoms ensemble is assumed to be in a superfluid state where I investigate both, the order parameter when the Rydberg excitation laser is applied and the interference pattern of the condensates in different dimensions. The study shows the emerging long-range interactions lead to a rapid collapse of the superfluid order parameter and in general allow only for partial revivals. In addition, the interference experiments can directly reveal the interaction between Rydberg-dressed atoms. In the fourth chapter, the dynamics of Rydberg-dressed atoms trapped in a dynamical, i.e., time-dependent, potential confinement is presented. The dynamical trap is constructed such that it begins as a harmonic oscillator and ends as a double- well potential. The analysis investigates an ensemble of contact-interacting atoms via the time-dependent non-linear GP equation.
We investigate the effects of many-body correlations on the ground-state properties of a single-component ultracold Rydberg-dressed Fermi liquid with purely repulsive interparticle interactions in both three and two spatial dimensions. We employed the Fermi-hypernetted-chain Euler-Lagrange approximation and observed that the contribution of the correlation energy on the ground-state energy becomes significant at intermediate values of the soft-core radius and large coupling strengths. For small and large soft-core radii, the correlation energy is negligible and the ground-state energy approaches the Hartree-Fock value. The positions of the main peaks in static structure factor and pair distribution function in the homogeneous fluid phase signal the formation of quantum droplet crystals with several particles confined inside each droplet.
In this thesis I present several theoretical methods to explore the excitation dynamics of Ultracold Rydberg systems in various regimes. For some applications the details of interactions between Rydberg atoms have to be carefully examined, while for others, the many-body aspect of Rydberg excitation may be crucial. In both cases, the basic prerequisite is to know the interactions sufficiently well. I will review the basic concepts how to evaluate molecular potentials in various Hund's cases and approximations. Long-range Rydberg-Rydberg interactions between Rydberg atoms induce ℓ-mixing which in certain situations gives rise to molecular resonances. For these resonances, we calculate long-range potentials in Hund's case (c) by diagonalization of an interaction matrix. The excitation dynamics of the resonances is always modeled as pair excitation. At high principal quantum number n, the interactions between Rydberg atoms can blockade the excitation of many surrounding atoms in the range of few μm. The atoms within this range are strongly correlated so that many-body treatments are, in general, needed. To describe this blockading effect and other manifestations of the collective behavior of Rydberg excitation, such as the many-body Rabi oscillations, spatial correlations between atoms and the fluctuations of the number of excited atoms, I have used three different approaches. In the mean-field approach the interactions between different atoms is modeled by a distribution of mean-field shifts for which a distribution of probabilities is calculated, A good agreement between the theoretical model and experimental measurements is found. To study the correlations between atoms the many-body wavefunction is numerically computed. The possibility of observing the many-body Rabi oscillations of Rydberg excitation and other aspects of many-body dynamics is analyzed. Although strong interactions cannot be treated perturbatively other expansions may be feasible. I will show that the expansion in powers of the single atom Rabi frequency can be evaluated in the interaction and Heisenberg picture. The expansion is expected to behave well for arbitrary strong interactions. ^