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Latin America Optics and Photonics Conference

Laser Induced Fluorescence Spectroscopy of the Rb 5S - 6S One- and Two-Photon M1 Transition

Randy Knize, Carson McLaughlin, M. D. Lindsay

Published Jan 1, 2022• 0 citations
Publisher

Abstract

We measure the Rb 5S-6S M1 transition, in a cell or atomic beam. We find the two-photon hyperfine transitions, and splittings with accuracy 10 kHz. We report progress on the one-photon highly forbidden transition measurements.
DOI
10.1364/laop.2022.tu1d.6

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Abstract Using a Rb cell and a wavemeter, with a Doppler-free two-photon transition near 993 nm, we have measured the four hyperfine components (two isotopes, Δ F = 0) of the 5S–6S transition, finding the absolute energies of those transitions to a spectral resolution of 0.002 cm −1 = 60 MHz. We find the (87 minus 85) isotope shift of the 5S–6S transition to be +94(12) MHz. Using our single frequency cw laser with focused intensity up to 10 4 W cm −2 at the cell, we find no AC Stark or light shift of the lines at 6 MHz spectral resolution. We find no density shift of the lines at 6 MHz spectral resolution, for a range of Rb atom densities from 3 × 10 11 to 5 × 10 13 atoms/cm 3 .
Frequency-modulation spectroscopy was employed successfully to measure the Doppler-free absorption and dispersion signals originating from several two-photon transitions in (85)Rb and (87)Rb. The two-photon cross section of the hyperfine transition 5S(1/2) (F = 2) ? 5D(5/2) (F = 4) in (87)Rb was determined to be sigma((2)) asymptotically equal to 4 x 10(-20) cm(4)/W. The transition isotope shift (TIS) of the transition 5S(1/2) ? 5D(5/2) between (87)Rb and (85)Rb was found to be Deltanu(TIS) = +166 +/- 2 MHz.
A high-resolution two-photon spectrum of 5S 1/2 → 5P 3/2 → 5D 5/2 transitions in a thermal 85 Rb vapor cell is presented by using an optical frequency comb and a cw laser. The fluorescence of 6P 3/2 → 5S 1/2 spontaneous emission is detected when the cw laser frequency is scanned from the 5S 1/2 ground state to 5P 3/2 hyperfine levels and the optical frequency comb repetition rate is fixed. The hyperfine splittings (F f = 2–5) of the 5D 5/2 excited state are well resolved. The dependences of fluorescence intensities on the cw laser intensity and temperature of 85 Rb vapor cell are studied, respectively. The experimental results are in good agreement with the theoretical analyses.
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