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ChemPhysChem

Quantum Phase Diagram of a Frustrated Spin‐1/2 Ferro‐Antiferromagnetic Normal Ladder

Monalisa Chatterjee, Debasmita Maiti, Manoranjan Kumar

Published Oct 31, 2022• 0 citations
Publisher

Abstract

Abstract In this work, we consider a frustrated two‐leg spin‐1/2 ladder composed of Heisenberg ferromagnetic and antiferromagnetic spin‐1/2 chains, and nearest spins from different legs interact via Heisenberg type rung exchange interactions that can be either ferromagnetic or antiferromagnetic in nature. The competing exchange interactions in the system lead to five different quantum phases like ferromagnetic, non‐collinear ferrimagnetic (NCF), , antiferromagnetic and dimer phases. The quantum phase diagram is constructed for the Heisenberg spin‐1/2 model and the phases are characterized using the correlation functions which are calculated by the density matrix renormalization group method. We also analyze the stability of phase and calculate the pitch angle in the NCF phase.

DOI
10.1002/cphc.202200538

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Abstract In this work, we consider a frustrated two‐leg spin‐1/2 ladder composed of Heisenberg ferromagnetic and antiferromagnetic spin‐1/2 chains, and nearest spins from different legs interact via Heisenberg type rung exchange interactions that can be either ferromagnetic or antiferromagnetic in nature. The competing exchange interactions in the system lead to five different quantum phases like ferromagnetic, non‐collinear ferrimagnetic (NCF), , antiferromagnetic and dimer phases. The quantum phase diagram is constructed for the Heisenberg spin‐1/2 model and the phases are characterized using the correlation functions which are calculated by the density matrix renormalization group method. We also analyze the stability of phase and calculate the pitch angle in the NCF phase.
Abstract We study a frustrated two-leg spin ladder with alternate isotropic Heisenberg and Ising rung exchange interactions, whereas, interactions along legs and diagonals are Ising-type. All the interactions in the ladder are anti-ferromagnetic in nature and induce frustration in the system. This model shows four interesting quantum phases: (i) stripe rung ferromagnetic (SRFM), (ii) stripe rung ferromagnetic with edge singlet (SRFM-E), (iii) anisotropic antiferromagnetic (AAFM), and (iv) stripe leg ferromagnetic (SLFM) phase. We construct a quantum phase diagram for this model and show that in stripe rung ferromagnet (SRFM), the same type of sublattice spins (either isotropic S -type or discrete anisotropic σ -type spins) are aligned in the same direction. Whereas, in anisotropic antiferromagnetic phase, both S and σ -type of spins are anti-ferromagnetically aligned with each other, two nearest S spins along the rung form an anisotropic singlet bond whereas two nearest σ spins form an Ising bond. In large Heisenberg rung exchange interaction limit, spins on each leg are ferromagnetically aligned, but spins on different legs are anti-ferromagnetically aligned. The thermodynamic quantities like specific heat C v ( T ), magnetic susceptibility χ ( T ) and thermal entropy S ( T ) are also calculated using the transfer matrix method for various phases. The magnetic gap in the SRFM and the SLFM can be noticed from χ ( T ) and C v ( T ) curves.
Using the density matrix renormalization group method, we determine the phase diagram of a frustrated bond-alternating S = 1/2 Heisenberg ladder with ferro-antiferromagnetic couplings at zero temperature. With the interactions between spins along the rungs set, we identify three spin-gapped phases (the Haldane phase, the singlet phase and the dimer phase) in the whole parameter range. The analysis of our data shows that two-leg spin bond-alternating ladders have a rich phase diagram if both rung and diagonal couplings are taken into account.
We study a frustrated two-leg spin ladder with alternate isotropic Heisenberg and Ising rung exchange interactions, whereas, interactions along legs and diagonals are Ising-type. All the interactions in the ladder are anti-ferromagnetic in nature and induce frustration in the system. This model shows four interesting quantum phases: (i) stripe rung ferromagnetic (SRFM), (ii) stripe rung ferromagnetic with edge singlet (SRFM-E), (iii) anisotropic antiferromagnetic (AAFM), and (iv) stripe leg ferromagnetic (SLFM) phase. We construct a quantum phase diagram for this model and show that in stripe rung ferromagnet (SRFM), the same type of sublattice spins (either SSS or σσσ-type spins) are aligned in the same direction. Whereas, in anisotropic antiferromagnetic phase, both SSS and σσσ-type of spins are anti-ferromagnetically aligned with each other, two nearest SSS spins along the rung form an anisotropic singlet bond whereas two nearest σσσ spins form an Ising bond. In large Heisenberg rung exchange interaction limit, spins on each leg are ferromagnetically aligned, but spins on different legs are anti-ferromagnetically aligned. The thermodynamic quantities like Cv(T)Cv(T)Cv(T), χ(T)χ(T)χ(T) and S(T)S(T)S(T) are also calculated using the transfer matrix method for different phase. The magnetic gap in the SRFM and the SLFM can be notice from χ(T)χ(T)χ(T) and Cv(T)Cv(T)Cv(T) curves.
Dimerized spin-1/2 ladders exhibit a variety of phase structures, which depend on the intra-chain and inter-chain spin exchange energies as well as on the dimerization pattern of the ladder. Using the density matrix renormalization group (DMRG) algorithm, we study critical properties of the bond-alternating two-leg Heisenberg spin ladder with diagonal interaction J ×. Two types of spin systems, staggered dimerized antiferromagnetic ladder and columnar dimerized ferro-antiferromagnetic couplings ladder, are investigated. To clarify the phase transition behaviors, we simultaneously analyze the string order parameter (SOP), the twisted order parameter (TOP), as well as a measurement of the quantum information analysis. Based on measuring this different observables, we establish the phase diagram accurately and give the fitting functions of the phase boundaries. In addition, the phase transition of cross-coupled spin ladder (in the absence of intrinsic dimerization) is also discussed.
Abstract Ladders with 2 N spins-1/2 and singlet ( S = 0) ground states are studied numerically using exact diagonalization and density matrix renormalization group (DMRG) calculations. The curvatures E ″ ( s ) of states with the lowest energy E ( s ) at spin s = S / N ≤ 1 are obtained in the thermodynamic limit. All states have E ″ ( s ) > 0 in two phases, one with strong F exchange J F in rungs, the other with strong F exchange J L in legs. The Dimer phase with frustrated F exchanges has one or more states with E ″ ( s ) < 0. All three phases have finite gaps to the lowest triplet state. The ladder at J F → ∞ is adiabatically connected to the spin-1 Heisenberg AF chain, and at J L → ∞ to the J 1 − J 2 model.
We present the phase diagram of the S=1/2S=1/2S=1/2 Heisenberg model on the two leg ladder with cyclic four-spin exchange, determined by a combination of exact diagonalization and density-matrix renormalization group techniques. We find six different phases and regimes: the rung singlet phase, a ferromagnetic phase, two symmetry broken phases with staggered dimers and staggered scalar chiralities, and a gapped region with dominant vector chirality, or collinear spin correlations. We localize the phase transitions and investigate their nature.