We study the impact of the diagonal frustrating couplings on the quantum phase diagram of a two-leg ladder composed of alternating spin-1 and spin-
21 rungs. As the coupling strength is increased the system successively exhibits two gapped paramagnetic phases (a rung-singlet and a Haldane-type nondegenerate states) and two ferrimagnetic phases with different ferromagnetic moments per rung. The first two states are similar to the phases studied in the frustrated spin-
21 ladder, whereas the magnetic phases appear as a result of the mixed-spin structure of the model. A detailed characterization of these phases is presented using density-matrix renormalization-group calculations, exact diagonalizations of periodic clusters, and an effective Hamiltonian approach inspired by the analysis of numerical data. The present theoretical study was motivated by the recent synthesis of the quasi-one-dimensional ferrimagnetic material
FeIIFeIII (trans-1,4-cyclohexanedicarboxylate) exhibiting a similar ladder structure.
Dimerized spin-1/2 ladders exhibit a variety of phase structures, which depend on the intra-chain and inter-chain spin exchange energies as well as on the dimerization pattern of the ladder. Using the density matrix renormalization group (DMRG) algorithm, we study critical properties of the bond-alternating two-leg Heisenberg spin ladder with diagonal interaction J ×. Two types of spin systems, staggered dimerized antiferromagnetic ladder and columnar dimerized ferro-antiferromagnetic couplings ladder, are investigated. To clarify the phase transition behaviors, we simultaneously analyze the string order parameter (SOP), the twisted order parameter (TOP), as well as a measurement of the quantum information analysis. Based on measuring this different observables, we establish the phase diagram accurately and give the fitting functions of the phase boundaries. In addition, the phase transition of cross-coupled spin ladder (in the absence of intrinsic dimerization) is also discussed.
Abstract We study a frustrated two-leg spin ladder with alternate isotropic Heisenberg and Ising rung exchange interactions, whereas, interactions along legs and diagonals are Ising-type. All the interactions in the ladder are anti-ferromagnetic in nature and induce frustration in the system. This model shows four interesting quantum phases: (i) stripe rung ferromagnetic (SRFM), (ii) stripe rung ferromagnetic with edge singlet (SRFM-E), (iii) anisotropic antiferromagnetic (AAFM), and (iv) stripe leg ferromagnetic (SLFM) phase. We construct a quantum phase diagram for this model and show that in stripe rung ferromagnet (SRFM), the same type of sublattice spins (either isotropic S -type or discrete anisotropic σ -type spins) are aligned in the same direction. Whereas, in anisotropic antiferromagnetic phase, both S and σ -type of spins are anti-ferromagnetically aligned with each other, two nearest S spins along the rung form an anisotropic singlet bond whereas two nearest σ spins form an Ising bond. In large Heisenberg rung exchange interaction limit, spins on each leg are ferromagnetically aligned, but spins on different legs are anti-ferromagnetically aligned. The thermodynamic quantities like specific heat C v ( T ), magnetic susceptibility χ ( T ) and thermal entropy S ( T ) are also calculated using the transfer matrix method for various phases. The magnetic gap in the SRFM and the SLFM can be noticed from χ ( T ) and C v ( T ) curves.
The frustrated ladder with alternate ferromagnetic(F) exchange
−JF and AF exchange
JA to first neighbors and F exchange
−JL to second neighbors is studied by exact diagonalization (ED) and density matrix renormalization group (DMRG) calculations in systems of
2N spins-1/2 with periodic boundary conditions. The ground state is a singlet
(S=0) and the singlet-triplet gap
εT is finite for the exchanges considered. Spin-1/2 string correlation functions
g1(N) and
g2(N) are defined for an even number
N of consecutive spins in systems with two spins per unit cell; the ladder has string order
g2(∞)>0 and
g1(∞)=0. The minimum
N∗ of
g2(N) is related to the range of ground-state spin correlations. Convergence to
g2(∞) is from below, and
g1(N) decreases exponentially for
N≥N∗. Singlet valence bond (VB) diagrams account for the size dependencies. The frustrated ladder at special values of
JF,
JL and
JA reduces to well-known models such as the spin-1 Heisenberg antiferromagnet and the
J1−J2 model, among others. Numerical analysis of ladders matches previous results for spin-1 gaps or string correlation functions and extends them to spin-1/2 systems. The nondegenerate singlet ground state of ladder is a bond-order wave, a Kekulé VB diagrams at
JL=JF/2≤JA, that is reversed on interchanging
−JF and
JA. Inversion symmetry is spontaneously broken in the dimer phase of the
J1−J2 model where the Kekulé diagrams are the doubly degenerate ground states at
J2/J1=1/2.
Abstract Ladders with 2 N spins-1/2 and singlet ( S = 0) ground states are studied numerically using exact diagonalization and density matrix renormalization group (DMRG) calculations. The curvatures E ″ ( s ) of states with the lowest energy E ( s ) at spin s = S / N ≤ 1 are obtained in the thermodynamic limit. All states have E ″ ( s ) > 0 in two phases, one with strong F exchange J F in rungs, the other with strong F exchange J L in legs. The Dimer phase with frustrated F exchanges has one or more states with E ″ ( s ) < 0. All three phases have finite gaps to the lowest triplet state. The ladder at J F → ∞ is adiabatically connected to the spin-1 Heisenberg AF chain, and at J L → ∞ to the J 1 − J 2 model.
We obtain the phase diagram in the parameter space $({J}^{\ensuremath{'}}∕J,\ensuremath{\gamma})$ and an accurate estimate of the critical line separating the different phases. We show several measurements of the magnetization, dimerization, nearest neighbor correlation, and density of energy in the different zones of the phase diagram, as well as a measurement of the string order parameter proposed as the nonvanishing phase order parameter characterizing Haldane phases. All these results will be compared in the limit ${J}^{\ensuremath{'}}∕J⪢1$ with the behavior of the
S=1 bond alternated Heisenberg chain (BAHC). The analysis of our data supports the existence of a dimer phase separated by a critical line from a Haldane one, which has exactly the same nature as the Haldane phase in the
S=1 BAHC.