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Nature

An optical innovation for metrology at the quantum limit of precision

Published Oct 17, 2022• 0 citations
Publisher

Abstract

Frequency-comb lasers are measuring sticks of the optical world and are used in metrology and sensing applications owing to their rigid, comb-like light spectra and metronomic pulsed output. A frequency comb with time-programmable pulses breaks this rigid mould and, in a demonstration of its utility, measures distances at the quantum limit of precision. A frequency-comb laser can be programmed to change pulse timing with high precision, to improve the sensitivity of distance measurements.

DOI
10.1038/d41586-022-03153-1

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Frequency-comb lasers are measuring sticks of the optical world and are used in metrology and sensing applications owing to their rigid, comb-like light spectra and metronomic pulsed output. A frequency comb with time-programmable pulses breaks this rigid mould and, in a demonstration of its utility, measures distances at the quantum limit of precision. A frequency-comb laser can be programmed to change pulse timing with high precision, to improve the sensitivity of distance measurements.
The measurement and manipulation of coherent optical fields have been transformed by the optical frequency comb. Today, the optical frequency comb grants measurements precise enough to count individual cycles of light as well as the generation of nearly any coherent electromagnetic field from the ultraviolet through the infrared. These capabilities have enabled the most precise realizations and comparisons of time, precision spectroscopy over broad bandwidths, and the ability to convert stable signals between optical and microwave fields–seamlessly connecting the entire electromagnetic spectrum from hertz (100 ) to petahertz (1015). These applications involve the interference of a frequency comb with another coherent light source, such as another frequency comb or a single-frequency continuous-wave laser. However, coherent light represents only one type of light. The vast majority of light emanates from “black bodies” such as stars, which is in a thermal state as opposed to a coherent state, and carries profound information about the universe and humanity’s place within it. Other types of light defy classical electromagnetism and are known as non-classical or quantum light. Such quantum light may play central roles in quantum communication, quantum computation, and quantum-enhanced metrology. In this thesis, the use of the optical frequency comb in the interferometric measurement of thermal and quantum light is investigated, with a focus on assessing fundamental limits to the sensitivity of such measurements. In order to measure thermal light, a technique called dual-comb correlation spectroscopy is explored. This technique entails heterodyne measurement of the field of thermal light and subsequent correlation of the field in time. This process reveals the spectrum of thermal light at high resolution and across broad bandwidths. New theoretical work uncovers previously unknown fundamental limits on sensitivity when measuring realistically weak thermal light. Experimental investigation verifies this scaling and is accompanied by a demonstration of spectroscopy at the equivalent power spectral density of our Sun, realizing a greater than 1000-fold sensitivity increase over past demonstrations of this technique. These insights pave the way for expansion of this technique to comb-based spatial correlation of thermal fields. This advancement would allow for extended baseline synthetic aperture hyperspectral imaging throughout the optical spectrum, facilitating novel and profound observations of the universe. The use of frequency combs for the measurement of quantum light is also investigated. This scenario breaks typical quantum optics assumptions, such as large, mode-matched local oscillators, and necessitates new quantum measurement operators. Such measurement operators are derived, which not only describe homodyne measurements on any quantum state of light with a frequency comb local oscillator, but also indicate that the shot noise limit generally reached in comb-based measurements of coherent light (such as in continuous-wave laser heterodyne and dual-comb spectroscopy) does not correspond to the quadrature or coherent state-overlap description standard in quantum optics. Efforts to experimentally reach this “standard” quantum limit demonstrate a significant improvement in the signal-to-noise ratio over the conventional comb-based shot noise limit, paving the way for lower-power portable optical clocks and quantum-enhanced frequencycomb metrology.
Optical frequency combs combine ultrashort pulse duration and phase stability, making them powerful resources for high-precision ranging even when affected by atmospheric dispersion. It has been established that by classical modal engineering and mode-sensitive detection, sensitivity to distance at the standard limit can be achieved; however, attaining improved uncertainties by the use of squeezing has not been explored. Here, we apply an effective Hamiltonian framework to the problem of ranging with quantum frequency combs in order to derive the associated precision bounds for distance estimation. The problem needs addressing of the pulse shape and its quantum properties at once. The analysis reveals that quantum solutions may be appealing mostly for short-distance applications.
Optical frequency combs combine ultrashort pulse duration and phase stability, making them powerful resources for high-precision ranging even when affected by atmospheric dispersion. It has been established that by classical modal engineering and mdoe-sensitive detection sensitivity to distance at the standard limit can be achieved, however attaining improved uncertainties by the use of squeezing has not been explored. Here, we apply an effective Hamiltonian framework to the problem of ranging with quantum frequency combs in order to derive the associated precision bounds for distance estimation. We analyse the role of intensity anti-squeezing and temporal beam shaping, and find that quantum solutions may be appealing mostly for short-distance applications.
Optical frequency combs have emerged as a cornerstone for a wide range of areas, including spectroscopy, ranging, optical clocks, time and frequency transfer, waveform synthesis, and communications. However, quantum-mechanical fluctuations of the optical carrier impose fundamental performance limits on the precision of classical optical frequency combs, particularly in their use for interferometry and spectroscopy. Entanglement, as a quintessential quantum resource, allows for surpassing the fundamental limits of classical systems. Here, we introduce entanglement into the realm of optical frequency combs, formulating entangled dual-comb spectroscopy (EDCS) that surmounts the fundamental limits of classical DCS. EDCS capitalizes on tailored entangled structures across the frequency comb, enabling simultaneous detection of all comb lines below the standard quantum limit of classical DCS. Applying EDCS in gas detection, we achieve a 2.6-dB enhancement in signal-to-noise ratio and a 1.7-fold reduction in integration time over classical DCS, rendering EDCS particularly suited for dynamic chemical and biological sensing, where fast, precise measurements subject to power constraints are required. EDCS opens a new avenue for exploiting quantum frequency combs, underscoring their prospects in a plethora of applications in precision metrology, spectroscopy, and timekeeping.