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Quantum optics with surface plasmons and plasmonic resonators (Orale)

Jean‐Jacques Greffet

Published Oct 30, 2017• 0 citations
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Revisiting quantum optics with surface plasmons (Orale)

François Marquier, Marie-Christine Dheur, Benjamin Vest +3 more

Surface plasmon polaritons (SPPs) result from collective oscillations of free electrons coupled to an electromagnetic field at a plane interface between a metal and a dielectric medium. As photons, SPPs can be considered either as waves or as bosonic particles [1] and they can experience striking quantum interferences such as Hong-Ou-Mandel (HOM) effect [2]. We use in this paper a plasmonic platform (Fig.1) that can convert photons into plasmons, and separate or recombine them on a plasmonic beamsplitter [3]. Single SPPs are excited using single photons created by parametric down conversion into a periodically-poled KTP crystal. The platform is placed in a Mach-Zehnder interferometer in order to vary the path difference between SPPs before impinging on the beamsplitter. The setup allows us to revisit quantum optics experiments using SPP as carriers of the quantum of energy. Using the same device, we can test the wave-particle duality, two-particle (HOM) interference and non-local control of single plasmon interference using the entanglement between a photon and a SPP [4]. In the case of the HOM experiment, we demonstrate that the losses can be used as a new degree of freedom [5]. Playing with the dephasing between transmission and reflection coefficient of the beamsplitter, we can observe a peak instead of the usually expected dip in the HOM interference (Fig.2), i.e. an anti-coalescence effect of SPP. In this talk, we will introduce the plasmonic device main features as well as the different quantum plasmonics experiments that have been performed thanks to the SPP beamsplitter. These results are essential to understand the SPP quantum behavior or to develop hybrid plasmon-photon systems for potential future applications in quantum communication mediated by SPP. [1] JM Elson and R.H. Ritchie, Phys. Rev. B 4, 4129 (1971) [2] J.S. Fakonas et al., Nat. Phot. 8, 317 (2014) [3] M.C. Dheur et al. , Sc. Advances 2, e151574 (2016) [4] M.C. Dheur et al. ArXiv 1610.07493, B. Vest et al. ArXiv 1610.07479 [5] S. Barnett et al., Phys. Rev. A 57, 2134 (1998) Fig.1: Plasmonic platform used for the quantum optics experiment (B). It consists in two SPP launchers (A), a plasmonic beamsplitter, and two slits to convert SPP to photons in the glass substrate. The plasmonic interference can thus be probed using single photon counting modules. Fig2: HOM experiment on a lossy plasmonic beamsplitter, whose complex amplitude reflection and transmission factors are denoted r and t respectively. The usual HOM dip is observed when r = it (left), a peak in the coincidence rate is shown when r = t.

•Jan 8, 2017•0 citations

Electromagnetically-induced-transparency plasmonics: Quantum-interference-assisted tunable surface-plasmon-polariton resonance and excitation

Jian Qi Shen

An experimentally feasible configuration of a prism coupler with an electromagnetically-induced-transparency (EIT) medium layer, e.g., a semiconductor-quantum-dot (SQD) medium, deposited upon its prism base is suggested for generating tunable surface-plasmon-polariton resonance. Such surface-plasmon-polariton resonance and optical excitation of a surface plasmon wave can be manipulated by switchable quantum interference among SQD multilevel transitions driven by two external control fields. When an incident probe field is coupled into a surface plasmon wave excitation mode, the surface-plasmon-polariton (SPP) resonance at the interface between the SQD medium layer and the substrate will arise, and the quantum-coherently controllable reflection spectrum of the probe field on the prism base can be achieved. In this process, destructive and constructive quantum interference (determined by the intensity ratio of the two external control fields) in the SQD multilevel system plays a key role for achieving the tunable reflection spectrum. The EIT-based surface-plasmon-polariton resonance presented here will have three characteristics (some of them would be attractive): (i) switchable quantum interference exhibited by surface plasmon wave excitation, (ii) quantum-coherently controllable surface plasmon polaritons by external optical fields, (iii) surface wave sensitive to dispersion of the SQD quantum coherent medium. Such an effect of controllable optical response based on the quantum-interference switchable surface-plasmon-polariton resonance in the EIT-prism coupler may find some potential applications in design of new photonic and quantum optical devices.

Physical Review A•Aug 11, 2014•17 citations
Surface plasmon polaritons (SPPs) result from collective oscillations of free electrons coupled to an electromagnetic field at a plane interface between a metal and a dielectric medium. As photons, SPPs can be considered either as waves or as bosonic particles [1] and they can experience striking quantum interferences such as Hong-Ou-Mandel (HOM) effect [2]. We use in this paper a plasmonic platform (Fig.1) that can convert photons into plasmons, and separate or recombine them on a plasmonic beamsplitter [3]. Single SPPs are excited using single photons created by parametric down conversion into a periodically-poled KTP crystal. The platform is placed in a Mach-Zehnder interferometer in order to vary the path difference between SPPs before impinging on the beamsplitter. The setup allows us to revisit quantum optics experiments using SPP as carriers of the quantum of energy. Using the same device, we can test the wave-particle duality, two-particle (HOM) interference and non-local control of single plasmon interference using the entanglement between a photon and a SPP [4]. In the case of the HOM experiment, we demonstrate that the losses can be used as a new degree of freedom [5]. Playing with the dephasing between transmission and reflection coefficient of the beamsplitter, we can observe a peak instead of the usually expected dip in the HOM interference (Fig.2), i.e. an anti-coalescence effect of SPP. In this talk, we will introduce the plasmonic device main features as well as the different quantum plasmonics experiments that have been performed thanks to the SPP beamsplitter. These results are essential to understand the SPP quantum behavior or to develop hybrid plasmon-photon systems for potential future applications in quantum communication mediated by SPP. [1] JM Elson and R.H. Ritchie, Phys. Rev. B 4, 4129 (1971) [2] J.S. Fakonas et al., Nat. Phot. 8, 317 (2014) [3] M.C. Dheur et al. , Sc. Advances 2, e151574 (2016) [4] M.C. Dheur et al. ArXiv 1610.07493, B. Vest et al. ArXiv 1610.07479 [5] S. Barnett et al., Phys. Rev. A 57, 2134 (1998) Fig.1: Plasmonic platform used for the quantum optics experiment (B). It consists in two SPP launchers (A), a plasmonic beamsplitter, and two slits to convert SPP to photons in the glass substrate. The plasmonic interference can thus be probed using single photon counting modules. Fig2: HOM experiment on a lossy plasmonic beamsplitter, whose complex amplitude reflection and transmission factors are denoted r and t respectively. The usual HOM dip is observed when r = it (left), a peak in the coincidence rate is shown when r = t.
An experimentally feasible configuration of a prism coupler with an electromagnetically-induced-transparency (EIT) medium layer, e.g., a semiconductor-quantum-dot (SQD) medium, deposited upon its prism base is suggested for generating tunable surface-plasmon-polariton resonance. Such surface-plasmon-polariton resonance and optical excitation of a surface plasmon wave can be manipulated by switchable quantum interference among SQD multilevel transitions driven by two external control fields. When an incident probe field is coupled into a surface plasmon wave excitation mode, the surface-plasmon-polariton (SPP) resonance at the interface between the SQD medium layer and the substrate will arise, and the quantum-coherently controllable reflection spectrum of the probe field on the prism base can be achieved. In this process, destructive and constructive quantum interference (determined by the intensity ratio of the two external control fields) in the SQD multilevel system plays a key role for achieving the tunable reflection spectrum. The EIT-based surface-plasmon-polariton resonance presented here will have three characteristics (some of them would be attractive): (i) switchable quantum interference exhibited by surface plasmon wave excitation, (ii) quantum-coherently controllable surface plasmon polaritons by external optical fields, (iii) surface wave sensitive to dispersion of the SQD quantum coherent medium. Such an effect of controllable optical response based on the quantum-interference switchable surface-plasmon-polariton resonance in the EIT-prism coupler may find some potential applications in design of new photonic and quantum optical devices.