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Bulletin of the American Physical Society

Quantum Optics With Integrated Plasmonic/Optical Systems

Brendan Shields, Alexey Akimov, Frank H. L. Koppens, Chun Wei Yu, Parag B. Deotare, Darrick E. Chang, Philip Hemmer, Alexander S. Zibrov, Marko Lončar, Hongkun Park, Mikhail D. Lukin

Published May 20, 2009• 0 citations
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In this work, we experimentally observe for the first time nanoscale plasmonic enhanced Electromagnetically Induced Transparency (EIT) and Velocity Selective Optical Pumping (VSOP) effects in miniaturized Integrated Quantum Plasmonic Device (IQPD) for D 2 transitions in rubidium (Rb). Our device consists of a vapor cell integrated on top of a prism coated with a thin layer of metal. This configuration is known to allow efficient excitation of Surface Plasmon Resonance (SPR). The evanescent field of the surface plasmon mode interacts with the atomic media in close vicinity to the metal. In spite of the limited interaction length between SPR and Rb atoms, the signature of EIT along with VSOP signals could be clearly observed in our miniaturized IQPD under proper conditions of pump and probe intensities. A gradual decrease in the contrast of the plasmonic enhanced EIT and VSOP signals was observed as the excitation was detuned from the SPR critical angle, due to reduction in electromagnetic field enhancement, leading to a reduced interaction of the evanescent field with the atomic vapor media. Following the demonstration of these effects, we also present a detailed model revealing the mechanisms and the origin of plasmonic enhanced EIT and VSOP effects in our system. The model, which is based on the Bloch equations, is in good agreement with the observed experimental results. The obtained results are regarded as an important step in the quest for the realization of nanoscale quantum plasmonic effects and devices.
Plasmonic superradiance originates from the plasmon mediated strong correlation that builds up between dipolar emitters coupled to a metal nanoparticle. This leads to a fast burst of emission so that plasmonic superradiance constitutes ultrafast and extremely bright optical nanosources of strong interest for integrated quantum nano-optics platforms. We elucidate the superradiance effect by establishing the dynamics of the system, including all features such as the orientation of the dipoles, their distance to the particle, and the number of active plasmon modes. We determine an optimal configuration for Purcell enhanced superradiance. We also show superradiance blockade at small distances.