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Chinese Optics Letters

Fabrication, testing, and assembly of high-finesse optical fiber microcavity for molecule cavity QED experiment

Yuhao Pan, Li Li, Xiaolong Zhou, Dongyu Huang, Ze-Min Shen, Jian Wang, Chuan‐Feng Li, Guang‐Can Guo

Published Jan 1, 2022• 9 citations
Publisher

Abstract

The ultracold molecule is a promising candidate for versatile quantum tasks due to its long-range interaction and rich internal rovibrational states.With the help of the cavity quantum electrodynamics (QED) effects, an optical cavity can be employed to increase the efficiency of the formation of the photoassociated molecules and offers a non-demolition detection of the internal states of molecules.Here, we demonstrate the production of the high-finesse optical fiber microcavity for the Rb 2 molecule cavity QED experiment, which includes the fabrication of fiber-based cavity mirrors, testing, and the assembly of ultra-high vacuum-compatible optical fiber microcavity.The optical fiber microcavity offers high cooperativity between cavity mode and ultracold molecule and paves the way for the study of molecule cavity QED experimental research.

DOI
10.3788/col202220.122702

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•Aug 3, 2016•0 citations
The ultracold molecule is a promising candidate for versatile quantum tasks due to its long-range interaction and rich internal rovibrational states.With the help of the cavity quantum electrodynamics (QED) effects, an optical cavity can be employed to increase the efficiency of the formation of the photoassociated molecules and offers a non-demolition detection of the internal states of molecules.Here, we demonstrate the production of the high-finesse optical fiber microcavity for the Rb 2 molecule cavity QED experiment, which includes the fabrication of fiber-based cavity mirrors, testing, and the assembly of ultra-high vacuum-compatible optical fiber microcavity.The optical fiber microcavity offers high cooperativity between cavity mode and ultracold molecule and paves the way for the study of molecule cavity QED experimental research.
The cavity quantum electrodynamics (QED) system is a promising platform for quantum optics and quantum information experiments.Its core is the strong coupling between atoms and optical cavity, which causes difficulty in the overlap between the atoms and the antinode of optical cavity mode.Here, we use a programmable movable optical dipole trap to load a cold atomic ensemble into an optical fiber microcavity and realize the strong coupling between the atoms and the optical cavity in which the coupling strength can be improved by polarization gradient cooling and adiabatic loading.By the measurement of vacuum Rabi splitting, the coupling strength can be as high as g N = 2π × 400 MHz, which means the effective atom number is N eff = 16 and the collective cooperativity is C N = 1466.These results show that this experimental system can be used for cold atomic ensemble and cold molecule based cavity QED research.
Ultracold ground-state molecules can be formed from ultracold atoms via photoassociation followed by a spontaneous emission process. Typically, the molecular products are distributed over a range of final states. Here, we propose to use an optical cavity with high cooperativity to selectively enhance the population of a pre-determined final state by controlling the spontaneous emission. During this process, a photon will be emitted into the cavity mode. Detection of this photon heralds a single reaction. We discuss the efficiency and the dynamics of cavity-assisted molecule formation in the frame of realistic parameters that can be achieved in current ultracold-atom setups. In particular, we consider the production of Rb 2 molecules in the a 3 Σ u triplet ground state. Moreover, when working with more than two atoms in the cavity, collective enhancement effects in chemistry should be observable.
We report the fabrication of a 1.2 cm long cavity directly on a nanofiber using femtosecond laser ablation. The cavity modes with finesse values in the range of 200-400 can enable the "strong-coupling" regime of cavity QED, with high cooperativity of 10-20, for a single atom trapped 200 nm away from the fiber surface [Phys. Rev. A80, 053826 (2009)PLRAAN1050-294710.1103/PhysRevA.80.053826]. Such cavity modes can still maintain the transmission between 40%-60%, suggesting a one-pass intracavity transmission of 99.53%. Other cavity modes, which can enable cooperativity in the range of 3-10, show transmission over 60%-85% and are suitable for fiber-based single-photon sources and quantum nonlinear optics in the "Purcell" regime.
We have realized a fiber-based Fabry–Perot cavity with CO 2 laser-machined mirrors. It combines very small size, high finesse , small waist and mode volume, and good mode matching between the fiber and cavity modes. This combination of features is a major advance for cavity quantum electrodynamics (CQED), as shown in recent CQED experiments with Bose–Einstein condensates enabled by this cavity (Colombe Y et al 2007 Nature 450 272). It will also be suitable for a wide range of other applications, including coupling to solid-state emitters, gas detection at the single-particle level, fiber-coupled single-photon sources and high-resolution optical filters with large stopband.
Open Fabry-Perot microcavities represent a promising route for achieving a quantum electrodynamics (cavity-QED) platform with diamond-based emitters. In particular, they offer the opportunity to introduce high-purity, minimally fabricated material into a tunable, high quality factor optical resonator. Here, we demonstrate a fiber-based microcavity incorporating a thick ($>10\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\text{m}$) diamond membrane with a finesse of 17 000, corresponding to a quality factor $Q\ensuremath{\sim}{10}^{6}$. Such minimally fabricated thick samples can contain optically stable emitters similar to those found in bulk diamond. We observe modified microcavity spectra in the presence of the membrane, and we develop analytic and numerical models to describe the effect of the membrane on cavity modes, including loss and coupling to higher-order transverse modes. We estimate that a Purcell enhancement of approximately 20 should be possible for emitters within the diamond in this device, and we provide evidence that better diamond surface treatments and mirror coatings could increase this value to 200 in a realistic system.
Fiber Fabry-Perot cavities, formed by micro-machined mirrors on the end-facets of optical fibers, are used in an increasing number of technical and scientific applications. Some of the most promising areas of application of these optical micro-resonators with high finesse and small mode volume are in the field of quantum communication and information. The resonator-enhanced light-matter interaction, for instance, provide basis for the realization of efficient optical interfaces between stationary matter-based quantum nodes and flying single-photon qubits. To date fiber Fabry-Perot cavities have been successfully applied in experiments interfacing single photons with a wide range of quantum systems, including cold atoms, ions and solid state emitters as well as quantum optomechanical experiments. Here we address some important practical questions that arise during the experimental implementation of high finesse fiber Fabry-Perot cavities: How can optimal fiber cavity alignment be achieved and how can the efficiency of coupling light from the optical fibers to the cavity mode and vice versa be characterized? How should optical fiber cavities be constructed and stabilized to fulfill their potential for miniaturization and integration into robust scientific and technological devices that can operate outside of dedicated laboratory environments in the future? The first two questions we answer with an analytic mode matching calculation that relates the alignment dependent fiber-to-cavity mode-matching efficiency to the easily measurable dip in the reflected light power at the cavity resonance. Our general analysis provides a simple recipe for the optimal alignment of fiber Fabry-Perot cavities and moreover for the first time explains the asymmetry in their reflective line shapes. The latter question we explore by investigating a novel, intrinsically rigid fiber cavity design that makes use of the high passive stability of a monolithic cavity spacer and employs thermal self-locking and external temperature tuning. The performance of this novel approach is compared to a more traditional, piezomechanically-actuated resonator that is feedback stabilized to a reference laser based on the Pound-Drever-Hall locking technique. Finally, with the application of single photon interfacing in mind we discuss the issue of fiber-generated background photons in Fiber Fabry-Perot cavities. We believe that, due to their simplicity, compactness and robustness, rigid fiber cavities could be a promising solution for miniaturized, integratable and scalable cavity quantum electrodynamic devices and further applications of FFPC with similar requirements.