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Optics Letters

Magnetometry based on the effect of laser-induced plasmas in a sodium-containing environment

Ning Ding, Guoguo Kang, Xiaoxu Zhang, Yixin Guo, Zong-Yu Guo, Luo Zhao, Weiqi Jin, Huiqi Zheng, Qiongying Ren, Hua Zhao

Published Aug 15, 2022• 1 citation
Publisher

Abstract

The magneto-optical resonance response of sodium atoms generated by a high-energy solid-state pulse Nd:YAG laser is studied in different external magnetic fields. We investigate the resonance fluorescence signal of sodium atoms in a simulated sea fog environment based on the laser-induced plasma (LIP) effect. By ionizing an NaCl solution spray to generate sodium atoms in an atmospheric environment, we build a Bell–Bloom magneto-optical resonance system under laboratory conditions. With the help of laser-induced breakdown spectroscopy (LIBS) and extinction spectrum, we obtain sodium atoms with a lifetime of 250 µs. A narrowband tunable continuous wave (CW) 589-nm laser tuned at the D 2 line with a modulation frequency around the Larmor frequency is used as the pump beam to polarize sodium atoms in the test magnetic field. We find that the magneto-optical resonance signals vary with different external magnetic fields and the positions of the resonance signal are consistent with the theoretical values. An intrinsic magnetometric sensitivity of 620.4 pT in a 1-Hz bandwidth is achieved.

DOI
10.1364/ol.468358

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The magneto-optical resonance response of sodium atoms generated by a high-energy solid-state pulse Nd:YAG laser is studied in different external magnetic fields. We investigate the resonance fluorescence signal of sodium atoms in a simulated sea fog environment based on the laser-induced plasma (LIP) effect. By ionizing an NaCl solution spray to generate sodium atoms in an atmospheric environment, we build a Bell–Bloom magneto-optical resonance system under laboratory conditions. With the help of laser-induced breakdown spectroscopy (LIBS) and extinction spectrum, we obtain sodium atoms with a lifetime of 250 µs. A narrowband tunable continuous wave (CW) 589-nm laser tuned at the D 2 line with a modulation frequency around the Larmor frequency is used as the pump beam to polarize sodium atoms in the test magnetic field. We find that the magneto-optical resonance signals vary with different external magnetic fields and the positions of the resonance signal are consistent with the theoretical values. An intrinsic magnetometric sensitivity of 620.4 pT in a 1-Hz bandwidth is achieved.
Magnetic resonance of sodium fluorescence is studied with varying laser intensity, duty cycle, and field strength. A magnetometer based on a sodium vapor cell filled with He buffer gas is demonstrated, using a single amplitude-modulated laser beam. With a 589 nm laser tuned at the D1 or D2 line, the magnetic field is inferred from the variation of fluorescence. A magnetic field sensitivity of 150 pT/Hz is achieved at the D1 line. The work is an important step toward sensitive remote magnetometry with mesospheric sodium.
Measurement and monitoring of geomagnetic field in the mesosphere has many potential applications such as detection of oceanic currents, mapping of large-scale magnetic structures, and study of electric-current fluctuations in the ionosphere. Remote measurement of the geomagnetic field can be performed by optical pumping of sodium atoms in the mesosphere with an amplitude modulated (AM) light at the Larmor precession frequency, and observing the magnetic resonance in fluorescence at a ground station. In this context, we have conducted an experiment in the laboratory to demonstrate remote magnetic field measurement using fluorescence signal from a sodium cell. Sodium atoms in the cell are interrogated with AM light produced by an acousto-optic modulator (AOM), introduced in the beam path of a frequency-doubled amplified sodium laser made in our laboratory. Magnetic resonance observed in sodium cell fluorescence is studied as a function of varying magnetic field intensity. Characteristics of the magnetic resonance such as linewidth and contrast (or SNR), and their dependence on optical power density, AM duty cycle, B-field orientation and intensity are studied. Theoretical modeling and experimental measurements are also carried out to determine the sensitivity of the magnetometer for realizing remote magnetometry with mesospheric sodium atoms.
We report on magneto-optical resonances observed in sodium fluorescence from D2 manifold with an intensity-modulated light. Fluorescence resonances are measured in the perpendicular (90°) and backward (180°) directions to the light propagation in laboratory experiments using a sodium cell containing neon buffer gas. Properties of these resonances are studied by varying the magnetic field at fixed-light modulation frequency, and vice-versa. Modulation with low-duty cycle shows higher-harmonic resonances of the modulation frequency and sub-harmonic resonances of the Larmor frequency. A dark resonance with maximum amplitude for laser wavelength closer to the crossover peak is observed. The origin of this dark resonance observed in Na D2 line is discussed using a theoretical model. Present study is aimed towards improving the understanding of magneto-optical resonances for remote magnetometry applications with mesospheric sodium.
In order to availably solve the crosstalk of the traditionally optically pumped magnetometer,in which an oscillating magnetic field drives transitions between Zeeman magnetic sublevels,an all-optical cesium(Cs)atomic magnetometer based on Bell-Bloom structure has been investigated and demonstrated experimentally in this paper.When there is an external magnetic field,by analyzing the Larmor precession spectrum of the polarized ground state atoms induced by a modulated pump laser,the atomic magnetometer with high sensitivity is achieved.First,we present the operating principle of the magnetometer with amplitude modulation and set up the experimental system by means of a three-layer magnetic shield.Then in the case of 100 nT field by optimizing the experimental parameters,i.e.,the frequency and intensity of the pump laser,we have obtained the atomic precession spectrum with line width(full width at half maximum)of 22 Hz and signal noise ratio(SNR)of 3.2×104 per unit hertz band width,and then have evaluated the magnetometer with an intrinsic sensitivity of 100fT/Hz1/2 and spatial resolution smaller than 1.2cm,while the experimentally closed loop test shows that the cesium atomic magnetometer would have the sensitivity of 120fT/Hz1/2 and response time of 300 ms.
We have demonstrated a technique for remote magnetometry using fluorescence measurements in a sodium cell. This technique utilizes two-photon resonance instead of single-photon resonance to generate magnetic resonances with synchronous modulation of two laser fields. A strong magnetic resonance with its dip matching the Larmor frequency, ΩL, is produced when a magnetic field perpendicular to the laser propagation direction is applied. A magnetic field sensitivity of 45 pT/√Hz is measured at a 35% modulation duty cycle where ΩL resonance has a maximum amplitude. We have discussed ways to further improve the sensitivity closer to the shot-noise limit by making changes to our existing setup. An additional magnetic resonance at 3ΩL is also formed due to two-photon resonance, which can be utilized in determining the magnetic field orientation. We have developed a theoretical model based on density matrix equations to study the magnetic resonances under different conditions and also for validating our experimental observations.
A cesium atomic magnetometer based on laser-pumped rf resonance has been investigated and demonstrated experimentally. Atoms are polarized and pumped to dark states by circularly polarized light. When there exists a magnetic field, the corresponding magnetization will be precessing around the magnetic field at Larmor frequency. By means of adding a resonant rf magnetic field, the atoms will be depolarized and absorb photons again. By detecting the spectrum of the transmitted light, one can obtain the information about the external magnetic field. We build an 894nm external cavity diode laser with a frequency stabilization device, and a low noise magnetic field measurement environment. After the optimization of the magnetometer parameter and closed-loop measurement, an ultimate sensitivity of 19 fT/Hz1/2 and an intrinsic sensitivity of 1.8 pT/Hz1/2 have been achieved with the spatial resolution smaller than 2 cm.