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Connecting few-body inelastic decay to many-body correlations: a weakly coupled impurity in a resonant Fermi gas

Sébastien Laurent, Matthieu Pierce, Marion Delehaye, Tarik Yefsah, Frédéric Chevy, Christophe Salomon

Published Dec 22, 2016• 0 citations
OpenAlex

Abstract

We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak inter-species coupling, the loss rate is proportional to Tan's contact. Second, using a 7 Li/ 6 Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional the 4/3 power of the fermionic density. Our results demonstrate that impurity-induced losses can be used as a quantitative probe of many-body correlations.

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Connecting Few-Body Inelastic Decay to Quantum Correlations in a Many-Body System: A Weakly Coupled Impurity in a Resonant Fermi Gas

Sébastien Laurent, Matthieu Pierce, Marion Delehaye +3 more

We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak interspecies coupling, the loss rate is proportional to Tan's contact. Second, using a ^{7}Li/^{6}Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional to n_{f}^{4/3}, where n_{f} is the fermionic density. This unusual exponent signals nontrivial two-body correlations in the system. Our results demonstrate that few-body losses can be used as a quantitative probe of quantum correlations in many-body ensembles.

arXiv:1612.08279•Physical Review Letters•Mar 10, 2017•47 citations

Three-Body Recombination at Vanishing Scattering Lengths in an Ultracold Bose Gas

Zav Shotan, Olga Machtey, S. J. J. M. F. Kokkelmans +1 more

We report on measurements of three-body recombination loss rates in an ultracold gas of ^{7}Li atoms in the extremely nonuniversal regime where the two-body scattering length vanishes. We show that the loss rate coefficient is well defined and can be described by two-body parameters only: the scattering length a and the effective range R_{e}. We find the rate to be energy independent, and, by connecting our results with previously reported measurements in the universal limit, we cover the behavior of the three-body recombination rate in the whole range from weak to strong two-body interactions. We identify a nontrivial magnetic field value in the nonuniversal regime where the rate should be suppressed.

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Three body contact in the unitary Fermi gas

Carl Heintze

The aim of this thesis was to measure the three-body contact in the unitary Fermi gas for the first time. The three-body contact is a physical observable that quantifies the three-body short-range correlations. Our probe, sensitive to three fermions with spins ↑↑↓ or ↓↓↑ at short distances, is three-body loss from the optical trap, caused by recombination into a deeply bound molecule and a free atom. In our system, the two spins signify two different hyperfine states of 6Li. We calibrate that recombination process by measuring three-body loss in the motional ground state of three fermions in an optical tweezer at unitarity. The numerically determined three-body contact C_3 (3) 3 of the three fermion system and the experimentally obtained loss rate allow us to extract Im[a_3], which quantifies the coupling to the deeply bound molecular state. Depending on the initial spin configuration ↑↑↓ or ↓↓↑, we find two different values, differing by almost a factor of two. This difference can only be explained by microscopic details of the interatomic coupling. In the many-body unitary Fermi gas, we use the coupling parameter Im[a_3] to extract the zero-temperature dimensionless three-body contact density $\zeta_3$ from three-body loss measurements. We obtain a value of $\zeta_3$ = 0.22(4) and observe that the loss rate scales with a characteristic three-body constant s = 1.77, which stems from an underlying SO(2,1) symmetry. We heat the gas and determine $\zeta_3$ in the thermal regime, observing agreement with the theoretical prediction based on the virial expansion. The extracted value of $\zeta_3$ > 0, which eludes theory, indicates three-body correlations. At the same time, the experimentally confirmed constant s proves the existence of irreducible three-body correlations that cannot be explained by two-body correlations alone.

•Jan 1, 2026•0 citations

Suppression of Unitary Three-Body Loss in a Degenerate Bose-Fermi Mixture

Xing-Yan Chen, Marcel Duda, Andreas Schindewolf +3 more

We study three-body loss in an ultracold mixture of a thermal Bose gas and a degenerate Fermi gas. We find that at unitarity, where the interspecies scattering length diverges, the usual inverse-square temperature scaling of the three-body loss found in nondegenerate systems is strongly modified and reduced with the increasing degeneracy of the Fermi gas. While the reduction of loss is qualitatively explained within the few-body scattering framework, a remaining suppression provides evidence for the long-range Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions mediated by fermions between bosons. Our model based on RKKY interactions quantitatively reproduces the data without free parameters, and predicts one order of magnitude reduction of the three-body loss coefficient in the deeply Fermi-degenerate regime.

arXiv:2110.01290•Physical Review Letters•Apr 14, 2022•24 citations

The Road to the Unitary Bose Gas

Benno S. Rem

Ultracold gases have become versatile systems to study quantum many-body effects. Their high degree of control and the tunability of the atomic interactions led to important advances in the understanding of strongly correlated matter. In the regime of strong interactions, unlike fermions, the study of bosons is hampered by three-particle recombination that leads to atom losses and keeps the system from reaching a real equilibrium state. In this thesis, we have performed the first quantitative comparison between theory and experiment on the three-particle loss coefficient L_3(a,T), for arbitrary scattering length a and temperature T. For unitary two-particle scattering (|a| → ∞), we show that the three-particle loss coefficient follows the law L_3(∞, T ) = λ_3/T^2, that we have tested using a trapped non-degenerate ^{7}Li gas maintained at constant temperature. The measured value of λ_3 = 2.5(3)_{stat}(6)_{cyst} × 10^{−20}(μK)^2cm^6s^{−1} is, within the error bars in good agreement with the theory prediction λ_3^{th} = 1.52 × 10^{−20}(μK)^2cm^6s^{−1}. We have extended our measurements to arbitrary values of the scattering length a. For a < 0, the theory predicts a smooth connection between the previously derived zero-temperature model for L_3(a, 0) and the unitarity limited loss coefficient L_3(∞, T ). We also show that a second Efimov resonance in 7Li should be observable near a = − 500 a0 for a temperature of 1 μK. Finally, we compare our theoretical prediction with measurements performed at Innsbruck with ^{133}Cs and at Cambridge with ^{39}K. The theory also shows remarkable quantitative agreement with these measurements.

•Jan 1, 2013•1 citation

Universal three-body recombination and Efimov resonances in an ultracold Li-Cs mixture

Juris Ulmanis, S. Häfner, R. Pires +4 more

We study Efimov resonances via three-body loss in an ultracold two-component gas of fermionic $^{6}\mathrm{Li}$ and bosonic $^{133}\mathrm{Cs}$ atoms close to a Feshbach resonance at 843 G, extending results reported previously [Pires et al., Phys. Rev. Lett. 112, 250404 (2014)] to temperatures around 120 nK. The experimental scheme for reaching lower temperatures is based upon compensating the gravity-induced spatial separation of the mass-imbalanced gases with bichromatic optical dipole traps. We observe the first and second excited Li-Cs-Cs Efimov resonance in the magnetic field dependence of the three-body event rate constant, in good agreement with the universal zero-range theory at finite temperature [Petrov and Werner, Phys. Rev. A 92, 022704 (2015)]. Deviations are found for the Efimov ground state, and the inelasticity parameter $\ensuremath{\eta}$ is found to be significantly larger than those for single-species systems.

arXiv:1509.05585•Physical Review A•Feb 16, 2016•36 citations
We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak inter-species coupling, the loss rate is proportional to Tan's contact. Second, using a 7 Li/ 6 Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional the 4/3 power of the fermionic density. Our results demonstrate that impurity-induced losses can be used as a quantitative probe of many-body correlations.
We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak interspecies coupling, the loss rate is proportional to Tan's contact. Second, using a ^{7}Li/^{6}Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional to n_{f}^{4/3}, where n_{f} is the fermionic density. This unusual exponent signals nontrivial two-body correlations in the system. Our results demonstrate that few-body losses can be used as a quantitative probe of quantum correlations in many-body ensembles.
We report on measurements of three-body recombination loss rates in an ultracold gas of ^{7}Li atoms in the extremely nonuniversal regime where the two-body scattering length vanishes. We show that the loss rate coefficient is well defined and can be described by two-body parameters only: the scattering length a and the effective range R_{e}. We find the rate to be energy independent, and, by connecting our results with previously reported measurements in the universal limit, we cover the behavior of the three-body recombination rate in the whole range from weak to strong two-body interactions. We identify a nontrivial magnetic field value in the nonuniversal regime where the rate should be suppressed.
The aim of this thesis was to measure the three-body contact in the unitary Fermi gas for the first time. The three-body contact is a physical observable that quantifies the three-body short-range correlations. Our probe, sensitive to three fermions with spins ↑↑↓ or ↓↓↑ at short distances, is three-body loss from the optical trap, caused by recombination into a deeply bound molecule and a free atom. In our system, the two spins signify two different hyperfine states of 6Li. We calibrate that recombination process by measuring three-body loss in the motional ground state of three fermions in an optical tweezer at unitarity. The numerically determined three-body contact C_3 (3) 3 of the three fermion system and the experimentally obtained loss rate allow us to extract Im[a_3], which quantifies the coupling to the deeply bound molecular state. Depending on the initial spin configuration ↑↑↓ or ↓↓↑, we find two different values, differing by almost a factor of two. This difference can only be explained by microscopic details of the interatomic coupling. In the many-body unitary Fermi gas, we use the coupling parameter Im[a_3] to extract the zero-temperature dimensionless three-body contact density ζ3\zeta_3ζ3​ from three-body loss measurements. We obtain a value of ζ3\zeta_3ζ3​ = 0.22(4) and observe that the loss rate scales with a characteristic three-body constant s = 1.77, which stems from an underlying SO(2,1) symmetry. We heat the gas and determine ζ3\zeta_3ζ3​ in the thermal regime, observing agreement with the theoretical prediction based on the virial expansion. The extracted value of ζ3\zeta_3ζ3​ > 0, which eludes theory, indicates three-body correlations. At the same time, the experimentally confirmed constant s proves the existence of irreducible three-body correlations that cannot be explained by two-body correlations alone.
We study three-body loss in an ultracold mixture of a thermal Bose gas and a degenerate Fermi gas. We find that at unitarity, where the interspecies scattering length diverges, the usual inverse-square temperature scaling of the three-body loss found in nondegenerate systems is strongly modified and reduced with the increasing degeneracy of the Fermi gas. While the reduction of loss is qualitatively explained within the few-body scattering framework, a remaining suppression provides evidence for the long-range Ruderman-Kittel-Kasuya-Yosida (RKKY) interactions mediated by fermions between bosons. Our model based on RKKY interactions quantitatively reproduces the data without free parameters, and predicts one order of magnitude reduction of the three-body loss coefficient in the deeply Fermi-degenerate regime.
Ultracold gases have become versatile systems to study quantum many-body effects. Their high degree of control and the tunability of the atomic interactions led to important advances in the understanding of strongly correlated matter. In the regime of strong interactions, unlike fermions, the study of bosons is hampered by three-particle recombination that leads to atom losses and keeps the system from reaching a real equilibrium state. In this thesis, we have performed the first quantitative comparison between theory and experiment on the three-particle loss coefficient L_3(a,T), for arbitrary scattering length a and temperature T. For unitary two-particle scattering (|a| → ∞), we show that the three-particle loss coefficient follows the law L_3(∞, T ) = λ_3/T^2, that we have tested using a trapped non-degenerate ^{7}Li gas maintained at constant temperature. The measured value of λ_3 = 2.5(3)_{stat}(6)_{cyst} × 10^{−20}(μK)^2cm^6s^{−1} is, within the error bars in good agreement with the theory prediction λ_3^{th} = 1.52 × 10^{−20}(μK)^2cm^6s^{−1}. We have extended our measurements to arbitrary values of the scattering length a. For a < 0, the theory predicts a smooth connection between the previously derived zero-temperature model for L_3(a, 0) and the unitarity limited loss coefficient L_3(∞, T ). We also show that a second Efimov resonance in 7Li should be observable near a = − 500 a0 for a temperature of 1 μK. Finally, we compare our theoretical prediction with measurements performed at Innsbruck with ^{133}Cs and at Cambridge with ^{39}K. The theory also shows remarkable quantitative agreement with these measurements.
We study Efimov resonances via three-body loss in an ultracold two-component gas of fermionic 6Li^{6}\mathrm{Li}6Li and bosonic 133Cs^{133}\mathrm{Cs}133Cs atoms close to a Feshbach resonance at 843 G, extending results reported previously [Pires et al., Phys. Rev. Lett. 112, 250404 (2014)] to temperatures around 120 nK. The experimental scheme for reaching lower temperatures is based upon compensating the gravity-induced spatial separation of the mass-imbalanced gases with bichromatic optical dipole traps. We observe the first and second excited Li-Cs-Cs Efimov resonance in the magnetic field dependence of the three-body event rate constant, in good agreement with the universal zero-range theory at finite temperature [Petrov and Werner, Phys. Rev. A 92, 022704 (2015)]. Deviations are found for the Efimov ground state, and the inelasticity parameter $\ensuremath{\eta}$ is found to be significantly larger than those for single-species systems.