Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Conference on Lasers and Electro-Optics

Statistics of multiphoton photoemission under coherent and non-classical illumination

Jonas Heimerl, Alexander Mikhaylov, Stefan Meier, Henrick Höllerer, Ido E. Kaminer, Maria V. Chekhova, Peter Hommelhoff

Published Jan 1, 2022• 2 citations
Publisher

Abstract

We investigate experimentally how the photon statistics of light gets imprinted on multiphoton electron emission from needle tips. Coherent and bright squeezed vacuum light lead to entirely different electron statistics, matching with a quantum-optical analysis.
DOI
10.1364/cleo_qels.2022.fm5d.6

Related papers

Strong Field Electron Emission Driven by a Bright Squeezed Vacuum

Andrei Rasputnyi, Jonas Heimerl, Jonathan Pölloth +4 more

The extreme light-matter interaction has brought unique tools for the subfemtosecond control of electron dynamics [1] and ultra-fast spectroscopy [2]. Until recently, the strong-field regime was accessible only with coherent states of light, which can be well described by classical electric fields when many photons are present (Fig. 1a). With the use of intense states of non-classical light, this situation has changed. New opportunities emerge with bright squeezed vacuum (BSV), which can be generated from optical parametric amplification of quantum vacuum fluctuations. Unlike classical light, BSV is a quantum superposition of coherent states with an amplitudes spanning a range from zero to very high values, up to ~1 TW/cm2[3]. BSV has a zero mean electric field and the variance of the electric field oscillates at the double carrier frequency (Fig. 1a). How such a non-classical electric field can affect the dynamics of photoemitted electrons was theoretically demonstrated recently [4]. Furthermore, the photon-number distribution of BSV has a very long tail in contrast to coherent light. These photon-number distributions can be imprinted onto the photon statistics of optical harmonics [3] and the statistics of electrons [5].

Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•Jun 23, 2025•0 citations

Electron Dynamics Under an Effective Photon-Statistics Force

Matan Even Tzur, Michael Birk, Alexey A. Gorlach +3 more

We predict and demonstrate a novel effective force exerted on matter when illuminated by light with non-classical photon-statistics. For squeezed-vacuum irradiation, the photon-statistics force stretches and squeezes matter wavefunctions, leading to emission of squeezed-vacuum harmonics.

•Jan 1, 2023•0 citations

Multiphoton effects with bright squeezed vacuum

Д. А. Копылов, Kirill Yu. Spasibko, Paula Cutipa +2 more

Light generated through strongly pumped parametric down-conversion has extremely strong photon-number fluctuations and is therefore highly efficient for multiphoton effects. In addition, its spectral and spatial properties can be tailored to allow two-dimensional multiphoton spectroscopy.

Conference on Lasers and Electro-Optics•Jan 1, 2020•0 citations

Quantum light drives electrons strongly at metal needle tips

Jonas Heimerl, Andrei Rasputnyi, Jonathan Pölloth +3 more

Attosecond science relies on driving photoemitted electrons with the strong optical field of a laser pulse, which represents an intense classical coherent state of light. Bright squeezed vacuum is a quantum state of light that is also intense enough to drive strong-field physics. However, its mean optical electric field is zero, suggesting that, in a semi-classical view, electrons should not experience strong driving. The question arises if and how this quantum state of light can generate signatures of attosecond dynamics in strong-field photoemission. Here we show that the key signatures of strong-field physics-the high energy plateau and subsequent cut-off-also appear under driving of a needle tip by bright squeezed vacuum, but only when we post-select electron energy spectra on the individual photon number of each pulse. When averaging over many shots, we observe broad energy spectra without a plateau. This suggests that electrons driven by bright squeezed vacuum behave as if driven by an ensemble of coherent states of light. Our findings bridge strong-field physics and quantum optics, offering insights into bright squeezed vacuum and other quantum light states, and suggest the use of strongly driven electrons as quantum light sensors.

arXiv:2503.22464•Nature Physics•Nov 7, 2025•17 citations

Nonlinear atomic tunnelling boosted by bright squeezed vacuum

Zhejun Jiang, Shengzhe Pan, Jianqi Chen +12 more

Nonlinear optical processes, mediated by multiphoton interactions rather than single-photon response, are routinely exploited to enable a range of light-based functionalities in devices and applications. Nonlinear effects are enhanced through higher intensity fields, which is a limiting strategy owing to potential radiation damage. An alternative strategy relies on the fluctuation redistribution typical of quantum light, but experimental demonstrations at the most fundamental level have been limited. Here we report experimental nonlinear tunnelling ionization of isolated atoms, a pivotal nonlinear process that drives high-harmonic generation and forms the basis of attosecond science, boosted by quantum light -- bright squeezed vacuum (BSV). A BSV light with an average pulse energy of 300 nJ achieves an effective intensity equivalent to that of a coherent light with 7.1 {\textmu}J, demonstrating a more than 20-fold quantum boost in nonlinear effect from BSV light. This boost is revealed by matching the peaks of the photoelectron momentum spectra produced by the BSV and coherent light using angular streaking. Furthermore, we demonstrate control of the effective intensity of the BSV by tuning the correlation function at fixed average pulse energy, establishing a robust method to tailor nonlinear processes via quantum statistics rather than classical intensity scaling. These findings may facilitate the development of quantum-controlled strong-field dynamics using tailored quantum light sources.

quant-pharXiv:2604.05783•Nature•Apr 8, 2026•7 citations

Tunneling driven by quantum light described via field Bohmian trajectories

Kim, Sangwon, Seongjin Ahn, Denis V. Seletskiy +1 more

Recent realization of an intense quantum light, namely bright squeezed vacuum, opened a new perspective on quantum light-matter interaction. Several theoretical works have appeared based on coherent state expansions of quantum state of light to investigate non-classical driving of high-harmonic generation in atomic gases and solids, or free-electron dynamics, but their predictions surprisingly coincide with what one could expect from essentially classical interpretations of the light statistics. A deeper theoretical insight into the underlying physics is necessary for understanding of observed experimental findings and predicting emerging effects relying on this new configuration. Here we present a theoretical framework to describe tunneling driven by quantum light, where the properties of such light are captured by a statistical ensemble of classical fields via a hydrodynamic, also referred to as Bohmian, formulation. Generalizing the quasiclassical theory of non-adiabatic tunneling driven by classical light, a single tunneling event is described by a bundle of tunneling solutions, each driven by a classical field corresponding to one realization in the ensemble. Quantum statistics of light are thus imprinted on the measured current. Fully quantum description of light via the Bohmian trajectories of its field provides a perfect fit to the description of the electron (under-) above-barrier dynamics in terms of (complex quasiclassical) real classical trajectories, resulting in a consistent and elegant theoretical approach. To illustrate this, we consider BSV-induced electron transport from the tip to the surface in the tunneling microscope configuration demonstrating the transition from the multiphoton to the direct tunneling regime.

arXiv:2507.15972•Jul 21, 2025•0 citations
The extreme light-matter interaction has brought unique tools for the subfemtosecond control of electron dynamics [1] and ultra-fast spectroscopy [2]. Until recently, the strong-field regime was accessible only with coherent states of light, which can be well described by classical electric fields when many photons are present (Fig. 1a). With the use of intense states of non-classical light, this situation has changed. New opportunities emerge with bright squeezed vacuum (BSV), which can be generated from optical parametric amplification of quantum vacuum fluctuations. Unlike classical light, BSV is a quantum superposition of coherent states with an amplitudes spanning a range from zero to very high values, up to ~1 TW/cm2[3]. BSV has a zero mean electric field and the variance of the electric field oscillates at the double carrier frequency (Fig. 1a). How such a non-classical electric field can affect the dynamics of photoemitted electrons was theoretically demonstrated recently [4]. Furthermore, the photon-number distribution of BSV has a very long tail in contrast to coherent light. These photon-number distributions can be imprinted onto the photon statistics of optical harmonics [3] and the statistics of electrons [5].
Attosecond science relies on driving photoemitted electrons with the strong optical field of a laser pulse, which represents an intense classical coherent state of light. Bright squeezed vacuum is a quantum state of light that is also intense enough to drive strong-field physics. However, its mean optical electric field is zero, suggesting that, in a semi-classical view, electrons should not experience strong driving. The question arises if and how this quantum state of light can generate signatures of attosecond dynamics in strong-field photoemission. Here we show that the key signatures of strong-field physics-the high energy plateau and subsequent cut-off-also appear under driving of a needle tip by bright squeezed vacuum, but only when we post-select electron energy spectra on the individual photon number of each pulse. When averaging over many shots, we observe broad energy spectra without a plateau. This suggests that electrons driven by bright squeezed vacuum behave as if driven by an ensemble of coherent states of light. Our findings bridge strong-field physics and quantum optics, offering insights into bright squeezed vacuum and other quantum light states, and suggest the use of strongly driven electrons as quantum light sensors.
Nonlinear optical processes, mediated by multiphoton interactions rather than single-photon response, are routinely exploited to enable a range of light-based functionalities in devices and applications. Nonlinear effects are enhanced through higher intensity fields, which is a limiting strategy owing to potential radiation damage. An alternative strategy relies on the fluctuation redistribution typical of quantum light, but experimental demonstrations at the most fundamental level have been limited. Here we report experimental nonlinear tunnelling ionization of isolated atoms, a pivotal nonlinear process that drives high-harmonic generation and forms the basis of attosecond science, boosted by quantum light -- bright squeezed vacuum (BSV). A BSV light with an average pulse energy of 300 nJ achieves an effective intensity equivalent to that of a coherent light with 7.1 {\textmu}J, demonstrating a more than 20-fold quantum boost in nonlinear effect from BSV light. This boost is revealed by matching the peaks of the photoelectron momentum spectra produced by the BSV and coherent light using angular streaking. Furthermore, we demonstrate control of the effective intensity of the BSV by tuning the correlation function at fixed average pulse energy, establishing a robust method to tailor nonlinear processes via quantum statistics rather than classical intensity scaling. These findings may facilitate the development of quantum-controlled strong-field dynamics using tailored quantum light sources.
Recent realization of an intense quantum light, namely bright squeezed vacuum, opened a new perspective on quantum light-matter interaction. Several theoretical works have appeared based on coherent state expansions of quantum state of light to investigate non-classical driving of high-harmonic generation in atomic gases and solids, or free-electron dynamics, but their predictions surprisingly coincide with what one could expect from essentially classical interpretations of the light statistics. A deeper theoretical insight into the underlying physics is necessary for understanding of observed experimental findings and predicting emerging effects relying on this new configuration. Here we present a theoretical framework to describe tunneling driven by quantum light, where the properties of such light are captured by a statistical ensemble of classical fields via a hydrodynamic, also referred to as Bohmian, formulation. Generalizing the quasiclassical theory of non-adiabatic tunneling driven by classical light, a single tunneling event is described by a bundle of tunneling solutions, each driven by a classical field corresponding to one realization in the ensemble. Quantum statistics of light are thus imprinted on the measured current. Fully quantum description of light via the Bohmian trajectories of its field provides a perfect fit to the description of the electron (under-) above-barrier dynamics in terms of (complex quasiclassical) real classical trajectories, resulting in a consistent and elegant theoretical approach. To illustrate this, we consider BSV-induced electron transport from the tip to the surface in the tunneling microscope configuration demonstrating the transition from the multiphoton to the direct tunneling regime.