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Quantum 2.0 Conference and Exhibition

Non-Reciprocal Amplification of Light Using Cold Atoms Coupled to a Nanophotonic Waveguide

Christian Liedl, Sebastian Pucher, Shu‐Wei Jin, Arno Rauschenbeutel, Philipp Schneeweiß

Published Jan 1, 2022• 0 citations
Publisher

Abstract

We experimentally demonstrate non-reciprocal Raman amplification of light using atoms coupled to a nanofiber by employing the spin-momentum locking inherent to this system. Furthermore, we can set the amplification direction by the spin state in which the atoms are prepared.
DOI
10.1364/quantum.2022.qth4c.2

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Optical nanofibers realized as the waist of tapered silica fibers can be used to trap and optically interface laser-cooled atoms. Building on this system, we experimentally show a novel scheme for the nonreciprocal Raman amplification of light. While typically either the magneto-optical effect, a temporal modulation or an optical nonlinearity is employed to break reciprocity, in our approach, this results from the spin of the atoms forming the gain medium. By taking advantage of the inherent spin-momentum locking present in optical nanofibers, we perform an experiment in which we set the amplification direction by a suitable preparation of the atomic spin state. Our approach is general and, suitable quantum emitters provided, could also be implemented beyond the optical domain of the electromagnetic spectrum.
The realization of nanophotonic optical isolators with high optical isolation even at ultralow light levels and low optical losses is an open problem. Here, we employ the link between the local polarization of strongly confined light and its direction of propagation to realize low-loss nonreciprocal transmission through a silica nanofiber at the single-photon level. The direction of the resulting optical isolator is controlled by the spin state of cold atoms. We perform our experiment in two qualitatively different regimes, i.e., with an ensemble of cold atoms where each atom is weakly coupled to the waveguide and with a single atom strongly coupled to the waveguide mode. In both cases, we observe simultaneously high isolation and high forward transmission. The isolator concept constitutes a nanoscale quantum optical analog of microwave ferrite resonance isolators, can be implemented with all kinds of optical waveguides and emitters, and might enable novel integrated optical devices for fiber-based classical and quantum networks.
We experimentally and theoretically investigate collective radiative effects in an ensemble of cold atoms coupled to a single-mode optical nanofiber. Our analysis unveils the microscopic dynamics of the system, showing that collective interactions between the atoms and a single guided photon gradually build up along the atomic array in the direction of propagation of light. These results are supported by time-resolved measurements of the light transmitted and reflected by the ensemble after excitation via nanofiber-guided laser pulses, whose rise and fall times are shorter than the atomic lifetime. Superradiant decays more than 1 order of magnitude faster than the single-atom free-space decay rate are observed for emission in the forward-propagating guided mode, while at the same time, no speed-up of the decay rate is measured in the backward direction. In addition, position-resolved measurements of the light that is transmitted past the atoms are performed by inserting the nanofiber-coupled atomic array in a 45-m-long fiber ring resonator, which allow us to experimentally reveal the progressive growth of the collective response of the atomic ensemble. Our results highlight the unique opportunities offered by nanophotonic cold atom systems for the experimental investigation of collective light-matter interaction.
Techniques to controllably interface atoms with quantum optical fields form the basis for many applications in quantum information science. For example, photons are convenient to relay information over large quantum networks, while atoms naturally are physical systems that can process and store this information. Thus far, the available techniques to efficiently couple single photons with atomic media fall into one of the following, mostly independent, categories: i) cavity quantum electrodynamics (QED), where atomic interactions with light are enhanced via a high-finesse cavity, ii) coherent coupling with atomic ensembles exhibiting large optical depths, and iii) the use of fields tightly focused to dimensions smaller than or approaching the scattering cross-section of a single atom. Although remarkable achievements have been made with all of these approaches, a robust, scalable technique remains elusive. Recently, several groups have successfully demonstrated that cold atoms can be trapped near and interfaced with nanophotonic systems, such as hollow-core photonic crystal fibers [1] and tapered nanofibers [2–4]. The traps are well-characterized [2, 3, 5], and the nearly diffraction-limited transverse confinement of optical fields enables ∼ 10% coupling efficiency of a single atom to the fiber [2, 3]. This has already led to remarkable observations of strong light-matter interactions using relatively few atoms and low powers [1]. It has also been proposed that such techniques can be extended to highly configurable photonic crystal waveguides [6]. Together, these efforts raise the intriguing possibility for future nanophotonic systems with tremendous figures of merit, wherein atom-light interactions can be tailored nearly at will. Here, we discuss recent efforts to develop novel techniques to realize strong, controllable atom-photon and photon-photon interactions, which take full advantage of the parameter space afforded by nanophotonic interfaces and are not based upon the extension of existing techniques. As a specific example, we discuss a protocol to achieve “all-atomic” cavity QED [7], as briefly described below. First, we show that although the single-atom coupling to guided modes of a nanophotonic waveguide might be relatively weak, there exist collective modes of a trapped atomic ensemble whose coupling to light is enhanced by the square root of the atom number, √ NA. While collective effects are generally well-known, special consequences emerge in the nanofiber system when the atoms are trapped in a lattice. In particular, collective effects cause such a lattice to act as a near-perfect mirror for an incident field close to resonance. In analogy to cavity QED, we then demonstrate that two sets of atomic mirrors can form an effective cavity, which can greatly enhance the coupling of a single, specially chosen “impurity” atom (or a few impurity atoms) positioned inside. We introduce a novel quantum spin model to describe the atom-light coupling, which allows one to exactly map the atom-nanofiber interface onto the simple and elegant Jaynes-Cummings model of cavity QED [8]. A unique feature of our atomic mirrors compared to conventional cavities is that they have long relaxation times and are highly dispersive. Remarkably, even with very low mirror finesse (F ∼ 10 2 ), this property allows one to attain the “strong coupling” regime of cavity QED, where vacuum Rabi oscillations [9–12] occur between an excited impurity atom and a single “photon” stored in the cavity (or more precisely, in the atomic mirrors). Furthermore, as quantum mechanical objects, these atom mirrors can be used to store quantum information and transfer this information into propagating waveguide modes. These various features can be combined to realize all of the building blocks for scalable quantum information processing.
Reaching a regime of strong coupling between light and atoms is a long-sought goal in quantum optics, as it will enable non-linear optics at the photon level. Interfacing atoms with guided light in nanophotonic waveguides is a promising route to achieve such regimes. Experimental platforms include nanofibers [1] and photonic crystal waveguides (PCWs), owing to the large transverse confinement of their guided modes. With PCWs, tuning the dispersion relation gives rise to the additional benefit of a very low group velocity of the guided light [2] , allowing for strong coupling even in single pass. Moreover these systems can help explore waveguide-QED and probe exciting novel bandgap physics [3] . While encouraging values of couplings have been observed with first corrugated devices [4] , a photonic platform with trapped atoms via guided modes in the vicinity of a waveguide and lying deep in the strong coupling regime has yet to be demonstrated.