The realization of nanophotonic optical isolators with high optical isolation even at ultralow light levels and low optical losses is an open problem. Here, we employ the link between the local polarization of strongly confined light and its direction of propagation to realize low-loss nonreciprocal transmission through a silica nanofiber at the single-photon level. The direction of the resulting optical isolator is controlled by the spin state of cold atoms. We perform our experiment in two qualitatively different regimes, i.e., with an ensemble of cold atoms where each atom is weakly coupled to the waveguide and with a single atom strongly coupled to the waveguide mode. In both cases, we observe simultaneously high isolation and high forward transmission. The isolator concept constitutes a nanoscale quantum optical analog of microwave ferrite resonance isolators, can be implemented with all kinds of optical waveguides and emitters, and might enable novel integrated optical devices for fiber-based classical and quantum networks.
The realization of nanophotonic optical isolators with high optical isolation even at ultralow light levels and low optical losses is an open problem. Here, we employ the link between the local polarization of strongly confined light and its direction of propagation to realize low-loss nonreciprocal transmission through a silica nanofiber at the single-photon level. The direction of the resulting optical isolator is controlled by the spin state of cold atoms. We perform our experiment in two qualitatively different regimes, i.e., with an ensemble of cold atoms where each atom is weakly coupled to the waveguide and with a single atom strongly coupled to the waveguide mode. In both cases, we observe simultaneously high isolation and high forward transmission. The isolator concept constitutes a nanoscale quantum optical analog of microwave ferrite resonance isolators, can be implemented with all kinds of optical waveguides and emitters, and might enable novel integrated optical devices for fiber-based classical and quantum networks.
Photons are nonchiral particles: their handedness can be both left and right. However, when light is transversely confined, it can locally exhibit a transverse spin whose orientation is fixed by the propagation direction of the photons. Confined photons thus have chiral character. Here, we employ this to demonstrate nonreciprocal transmission of light at the single-photon level through a silica nanofibre in two experimental schemes. We either use an ensemble of spin-polarised atoms that is weakly coupled to the nanofibre-guided mode or a single spin-polarised atom strongly coupled to the nanofibre via a whispering-gallery-mode resonator. We simultaneously achieve high optical isolation and high forward transmission. Both are controlled by the internal atomic state. The resulting optical diode is the first example of a new class of nonreciprocal nanophotonic devices which exploit the chirality of confined photons and which are, in principle, suitable for quantum information processing and future quantum optical networks.
Nanophotonic components allow the control of the flow of light in integrated optical environments. Thereby, the light’s strong confinement leads to an inherent link between its local polarization and propagation direction which fundamentally alters the physics of light-matter interaction and gives rise to phenomena such as directional emission and direction-dependent coupling strengths [1]. I will present the underlying principles of this chiral light-matter interaction and its consequences for integrated applications [1]. In particular, I will show how we employ this effect to control the direction of spontaneous emission [2] and to realize low-loss nonreciprocal transmission at the single-photon level through a silica nanofiber [3]. We use two different approaches where either an ensemble of spin-polarized atoms is weakly coupled to a nanofiber or a single atom is strongly coupled to the nanofiber via a whispering-gallery-mode resonator. The resulting optical isolators show a strong imbalance between the transmissions in forward and reverse direction and, at the same time, a forward transmissions exceeding 70%. We extended this system to a 4-port device, where a single atom routes photons nonreciprocally from one fiber port to the next. This realizes a quantum optical circulator [4] which can even be prepared in a superposition of its operational modes. The demonstrated systems exemplify a new class of (quantum) nanophotonic devices that are ideally suited for photonic quantum information processing and quantum simulation. [1] Nature 541, 473, (2017). [2] Science 346, 67 (2014). [3] Phys. Rev. X 5, 041036 (2015). [4] Science 354, 1577 (2016).
Techniques to controllably interface atoms with quantum optical fields form the basis for many applications in quantum information science. For example, photons are convenient to relay information over large quantum networks, while atoms naturally are physical systems that can process and store this information. Thus far, the available techniques to efficiently couple single photons with atomic media fall into one of the following, mostly independent, categories: i) cavity quantum electrodynamics (QED), where atomic interactions with light are enhanced via a high-finesse cavity, ii) coherent coupling with atomic ensembles exhibiting large optical depths, and iii) the use of fields tightly focused to dimensions smaller than or approaching the scattering cross-section of a single atom. Although remarkable achievements have been made with all of these approaches, a robust, scalable technique remains elusive. Recently, several groups have successfully demonstrated that cold atoms can be trapped near and interfaced with nanophotonic systems, such as hollow-core photonic crystal fibers [1] and tapered nanofibers [2–4]. The traps are well-characterized [2, 3, 5], and the nearly diffraction-limited transverse confinement of optical fields enables ∼ 10% coupling efficiency of a single atom to the fiber [2, 3]. This has already led to remarkable observations of strong light-matter interactions using relatively few atoms and low powers [1]. It has also been proposed that such techniques can be extended to highly configurable photonic crystal waveguides [6]. Together, these efforts raise the intriguing possibility for future nanophotonic systems with tremendous figures of merit, wherein atom-light interactions can be tailored nearly at will. Here, we discuss recent efforts to develop novel techniques to realize strong, controllable atom-photon and photon-photon interactions, which take full advantage of the parameter space afforded by nanophotonic interfaces and are not based upon the extension of existing techniques. As a specific example, we discuss a protocol to achieve “all-atomic” cavity QED [7], as briefly described below. First, we show that although the single-atom coupling to guided modes of a nanophotonic waveguide might be relatively weak, there exist collective modes of a trapped atomic ensemble whose coupling to light is enhanced by the square root of the atom number, √ NA. While collective effects are generally well-known, special consequences emerge in the nanofiber system when the atoms are trapped in a lattice. In particular, collective effects cause such a lattice to act as a near-perfect mirror for an incident field close to resonance. In analogy to cavity QED, we then demonstrate that two sets of atomic mirrors can form an effective cavity, which can greatly enhance the coupling of a single, specially chosen “impurity” atom (or a few impurity atoms) positioned inside. We introduce a novel quantum spin model to describe the atom-light coupling, which allows one to exactly map the atom-nanofiber interface onto the simple and elegant Jaynes-Cummings model of cavity QED [8]. A unique feature of our atomic mirrors compared to conventional cavities is that they have long relaxation times and are highly dispersive. Remarkably, even with very low mirror finesse (F ∼ 10 2 ), this property allows one to attain the “strong coupling” regime of cavity QED, where vacuum Rabi oscillations [9–12] occur between an excited impurity atom and a single “photon” stored in the cavity (or more precisely, in the atomic mirrors). Furthermore, as quantum mechanical objects, these atom mirrors can be used to store quantum information and transfer this information into propagating waveguide modes. These various features can be combined to realize all of the building blocks for scalable quantum information processing.
Optical waveguides in the form of glass fibers are the backbone of global telecommunication networks. In such optical fibers, the light is guided over long distances by continuous total internal reflection which occurs at the interface between the fiber core with a higher refractive index and the lower index cladding. Although this mechanism ensures that no light escapes from the waveguide, it gives rise to an evanescent field in the cladding. While this field is protected from interacting with the environment in standard optical fibers, it is routinely employed in air- or vacuum-clad fibers in order to efficiently couple light fields to optical components or emitters using, e.g., tapered optical fiber couplers. Remarkably, the strong confinement imposed by the latter can lead to significant coupling of the light's spin and orbital angular momentum. Taking advantage of this effect, we demonstrate the controlled directional spontaneous emission of light by quantum emitters into a sub-wavelength-diameter waveguide. The effect is investigated in a paradigmatic setting, comprising cesium atoms which are located in the vicinity of a vacuum-clad silica nanofiber. We experimentally observe an asymmetry higher than 10:1 in the emission rates into the counterpropagating fundamental guided modes of the nanofiber. Moreover, we demonstrate that this asymmetry can be tailored by state preparation and suitable excitation of the quantum emitters. We expect our results to have important implications for research in nanophotonics and quantum optics and for implementations of integrated optical signal processing in the classical as well as in the quantum regime.
Summary form only given. Controlling the interaction of light and matter is the basis for diverse applications ranging from light technology to quantum information processing. Nowadays, many of these applications are based on nanophotonic structures. It turns out that the confinement of light in such nanostructures imposes an inherent link between its local polarization and its propagation direction, also referred to as spin-momentum locking of light [1]. Remarkably, this leads to chiral, i.e., propagation direction-dependent effects in the emission and absorption of light, and elementary processes of light-matter interaction are fundamentally altered. For example, when coupling plasmonic particles or atoms to evanescent fields, the intrinsic mirror symmetry of the particles' emission can be broken. In our group, we observed this effect in the interaction between single rubidium atoms and the evanescent part of a light field that is confined by continuous total internal reflection in a whispering-gallery-mode microresonator [2]. In the following, this allowed us to realize chiral nanophotonic interfaces in which the emission direction of light into the structure is controlled by the polarization of the excitation light [3] or by the internal quantum state of the emitter [4], respectively. Moreover, we employed this chiral interaction to demonstrate an integrated optical isolator [5] as well as an integrated optical circulator [6] which operate at the single-photon level and which exhibit low loss. The latter are the first two examples of a new class of nonreciprocal nanophotonic devices which exploit the chiral interaction between single quantum emitters and transversally confined photons.
Complete control of light-matter interactions at a single quantum level is critical for quantum science applications such as precision measurements and information processing. Nanophotonic devices, developed with recent advancements in nanofabrication techniques, can be used to tailor the interactions between single photons and atoms. One example of such a device is the optical nanofibre, which provides an excellent platform due to the strongly confined transverse light fields, long interaction length, low loss, and diverse optical modes. This facilitates a strong interaction between atoms and guided light, revealing chiral atom-light processes and the prospect of waveguide quantum electrodynamics. This work highlights recent advances on optical nanofiber mediated excitation of cold rubidium Rydberg atoms for the creation of a 1D Rydberg array.