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Annals of Physics

A semiclassical theory of quasienergies and floquet wave functions

Published Sep 1, 1991• 0 citations
Publisher
DOI
10.1016/0003-4916(91)90055-d

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We develop the Floquet-Bloch theory of noninteracting fermions on a periodic lattice in the presence of a constant electric field. As long as the field lies along a reciprocal-lattice vector, time periodicity of the Bloch Hamiltonian is inherited from the evolution of momentum in the Brillouin zone. The corresponding Floquet quasienergies yield the Wannier-Stark ladder with interband couplings included to all orders. These results are compared to perturbative results where the lowest-order interband correction gives the field-induced polarization shift in terms of the electric susceptibility. Additionally, we investigate electronic transport by coupling the system to a bath within the Floquet-Keldysh formalism. We then study the breakdown of the band-projected theory from the onset of interband contributions and Landau-Zener resonances in the band-resolved currents. In particular, we consider the transverse quantum-geometric response in two spatial dimensions due to the Berry curvature. In the strong-field regime, the semiclassical theory predicts a plateau of the geometric response as a function of field strength. Here, we scrutinize the conditions under which the semiclassical results continue to hold in the quantum theory.
In the framework of the Floquet formulation of time-dependent density functional theory we present several exact relations involving different parts of the quasienergy functional. These relations hold when the exact densities and exchange-correlation energy functional are employed. They can be used as useful constraints and tests when searching for the approximate forms of the time-dependent exchange-correlation functionals. The general results are illustrated on an exactly soluble model, Hooke's atom in a linearly polarized monochromatic laser field.