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Progress of Theoretical Physics Supplement

Non-Monotonic Temperature Dependence of Local Dynamics and Local Energy upon Cooling toward the Ising Spin Glass Transition

Sharon C. Glotzer, Peter H. Poole, Antonio Coniglio A, Naeem Jan

Published May 16, 2013• 0 citations
Publisher

Abstract

We have performed a detailed analysis of the local dynamics and local energies of the equilibrium, paramagnetic phase of the d = 2 and d = 3 ±J Ising spin glass model. Here we discuss our recently reported observations1) that while the average flip rate and average energy decrease monotonically with decreasing temperature, both the flip rate and energy of an increasing fraction of spins increase as the glass transition is approached on cooling. These findings are consistent with recent experimental results for the frequency-dependent magnetic susceptibility of an insulating spin glass, which showed that the approach to the glass transition could be detected from the high frequency behavior.

DOI
10.1143/ptp.126.383

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We have performed a detailed analysis of the local dynamics and local energies of the equilibrium, paramagnetic phase of the d = 2 and d = 3 ±J Ising spin glass model. Here we discuss our recently reported observations1) that while the average flip rate and average energy decrease monotonically with decreasing temperature, both the flip rate and energy of an increasing fraction of spins increase as the glass transition is approached on cooling. These findings are consistent with recent experimental results for the frequency-dependent magnetic susceptibility of an insulating spin glass, which showed that the approach to the glass transition could be detected from the high frequency behavior.
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By using frustration-preserving hard-spin mean-field theory, we investigated the phase-transition dynamics in the three-dimensional field-free ± J Ising spin-glass model. As the temperature T is decreased from paramagnetic phase at high temperatures, with a rate ω=-dT/dt in time t, the critical temperature depends on the cooling rate through a clear power law ω^{a}. With increasing antiferromagnetic bond fraction p, the exponent a increases for the transition into the ferromagnetic case for p<p_{c} and decreases for the transition into the spin-glass phase for p>p_{c}, signaling the ferromagnetic - spin-glass phase transition at p_{c}≈0.22. The relaxation time is also investigated in the adiabatic case ω=0 and the dynamic exponent zν is found to increase with increasing p.
Slow cooling dynamics of the Ising ppp-spin interaction spin-glass model
We have studied dynamical behaviour of the infinite-range Ising spin glass model with ppp-spin interaction above and below the transition into the non-ergodic phase. The transition is continuous at sufficiently high external magnetic field. The dynamic critical exponent of the power-law decay of the autocorrelation function at the transition point is shown to decrease smoothly to zero as the field approaches the ``tricritical'' point from above; at lower fields the transition is discontinuous. The {\it slow cooling} approach is used to study the nonergodic behavior below the transition at zero external field. It is shown that the anomalous response function Δ(t,t′)Δ(t,t')Δ(t,t′) contains δδδ-function as well as regular contributions at {\it any} temperature below the phase transition. No evidence of the second phase transition (known to exist within the static replica solution of the same model) is found. At lower enough temperatures the {\it slow cooling} solution approaches the one known for the standard SK model.
I present an analysis of the dynamic behavior of short-range Ising spin glasses observed in stochastic simulations. The time dependence of the order parameter q(t)=〈Sx{S}_{x}Sx​(0)Sx{S}_{x}Sx​(t)〉\ifmmode\bar\else\textasciimacron\fi{}---which is the same as that of the structure factor---and the time dependence of the related dynamic correlation functions have been recorded with good statistics and very long observation times. The spin-glass model with a symmetric distribution of discrete nearest-neighbor \ifmmode\pm\else\textpm\fi{}J interactions on a simple-cubic lattice was used. Simulations were performed with a special fast computer, allowing for the first-time investigation of the equilibrium dynamics for a wide range of temperatures (0.7\ensuremath{\le}kT/J\ensuremath{\le}5.0) and lattice sizes (83{8}^{3}83, 163{16}^{3}163, 323{32}^{3}323, and 643{64}^{3}643). I have found that the empirical formula q(t)=${\mathrm{ct}}^{\mathrm{\ensuremath{-}}x}$exp(-\ensuremath{\omega}${t}^{\ensuremath{\beta}}$) with temperature-dependent exponents x(T) and \ensuremath{\beta}(T) describes the decay very well at all temperatures above the spin-glass transition. In the spin-glass phase, only the algebraic decay q(t)=${\mathrm{ct}}^{\mathrm{\ensuremath{-}}x}$ could be observed, with different temperature dependences of the exponent x(T). The dynamic scaling hypothesis and finite-size scaling explain well the observed temperature and size dependence of the data, and the functional form of the correlation functions is com- patible with the scaling form if corrections to scaling are taken into account. The scaling behavior and the dynamic and static critical exponents found in my simulations are in reasonable agreement with recent experiments performed on insulating spin glasses, showing that despite its simplicity the discrete model of spin glasses analyzed in this work displays behavior similar to that seen in nature.
Closed non-linear equations are derived through mode-coupling approximations for the correlation functions and susceptibilities for the Edwards-Anderson model of a classical Heisenberg system with nearest-neighbour random exchange couplings. These equations, which exhibit full dynamical stability, lead to a self-consistent treatment of spin-density propagation and spin-current relaxation. They are found to describe a transition from a paramagnetic to a spin glass phase, which is viewed as one where the dynamics changes from ergodic to a non-ergodic behaviour. Near the critical temperature T c the low-frequency correlation functions are obtained as dynamical scaling laws governed by a critical frequency omega c , which slows down proportionally to epsilon 2 , with epsilon =(T-T c )/T c . Approaching the critical point from the paramagnetic side the diffusivity vanishes linearly with epsilon . The susceptibility exhibits a symmetric cusp. The drastic changes of the spin dynamics at the transition point show up most clearly for the spin-current spectra. The numerical solution of the equations is discussed.
We examine the phase transition of Ising spin glass models in two dimensions (2D), calculating complementary two quantities, i.e., the interface free energy ΔF(T)‾\overline{\Delta F(T)}ΔF(T)​ and the Binder parameter g L , on finite L × L ( L ≤24) lattices at very low temperatures T . We find that these quantities exhibit quite different features depending on the distribution of bonds. For the ± J distribution, ΔF(T)‾\overline{\Delta F(T)}ΔF(T)​ at very low temperatures slightly increases with L and g L intersect at T ∼0.25 J . These results suggest a non-zero temperature phase transition, T c ≠0. On the other hand, for the Gaussian distribution, ΔF(T)‾\overline{\Delta F(T)}ΔF(T)​ decreases as L increases even at T = 0 and g L for different L converges to unity at T = 0. These results confirm the assumption of the zero temperature phase transition, T c = 0. Finite-size scaling analyses support those results. Thus we suggest that, in 2D, the existence of a finite-temperature phase transition depends on the distribution of bonds and it exists when the bond distribution is ± J .