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Reviews of Modern Physics

Photon antibunching

Henryk Paul

Published Oct 1, 1982• 328 citations

Abstract

A review is given of recent theoretical studies devoted to the problem of generating radiation fields that exhibit the opposite of the well-known bunching of photons observed in light from thermal sources, the so-called antibunching effect. It is made clear that this phenomenon reflects the corpuscular nature of light and, hence, cannot be interpreted in terms of classical electrodynamics, needing, instead, the quantum-mechanical formalism for its description. It is shown in some detail that nonlinear interaction mechanisms like multiphoton absorption and parametric three-wave interaction are suited to change the photon statistical properties of incident (in most cases coherent) light such that the output field will be endowed with antibunching properties. Special emphasis is given to the problem of correctly specifying the dimensions of the mode volume occurring in the usual single-mode treatment of the field, which is, in fact, of great practical interest, since the magnitude of the antibunching effect is determined by the inverse average number of photons contained in that volume. In a later section it is pointed out that destructive interference with a coherent reference beam provides a means of (a) effectively enhancing photon antibunching that is already present in a high-intensity field, through reduction of the intensity, and (b) transforming phase fluctuations produced in a Kerr medium into antibunching-type intensity fluctuations. On the other hand, there exists a way of directly generating light with antibunching properties, the physical mechanism being resonance fluorescence from a single atom. The main features of this technique, both theoretical and experimental, are outlined, including a discussion of the first experimental results obtained a few years ago.

DOI: 10.1103/revmodphys.54.1061

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A review is given of recent theoretical studies devoted to the problem of generating radiation fields that exhibit the opposite of the well-known bunching of photons observed in light from thermal sources, the so-called antibunching effect. It is made clear that this phenomenon reflects the corpuscular nature of light and, hence, cannot be interpreted in terms of classical electrodynamics, needing, instead, the quantum-mechanical formalism for its description. It is shown in some detail that nonlinear interaction mechanisms like multiphoton absorption and parametric three-wave interaction are suited to change the photon statistical properties of incident (in most cases coherent) light such that the output field will be endowed with antibunching properties. Special emphasis is given to the problem of correctly specifying the dimensions of the mode volume occurring in the usual single-mode treatment of the field, which is, in fact, of great practical interest, since the magnitude of the antibunching effect is determined by the inverse average number of photons contained in that volume. In a later section it is pointed out that destructive interference with a coherent reference beam provides a means of (a) effectively enhancing photon antibunching that is already present in a high-intensity field, through reduction of the intensity, and (b) transforming phase fluctuations produced in a Kerr medium into antibunching-type intensity fluctuations. On the other hand, there exists a way of directly generating light with antibunching properties, the physical mechanism being resonance fluorescence from a single atom. The main features of this technique, both theoretical and experimental, are outlined, including a discussion of the first experimental results obtained a few years ago.

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We analyze the most popular approaches to photon antibunching as exemplified in a sim-ple model of second-harmonic generation. We find the exact evolution of the fundamental and harmonic fields for initial Fock states with small photon numbers. We show explicitly that definitions of photon antibunching based on the unnormalized, G(2)(t, t′), and normal-ized, g(2)(t, t′), two-time correlation functions describe distinct phenomena for nonstationary fields. For completeness, we also compare antibunching effects defined by the two-time and single-time correlations. 1 Photon antibunching Photon antibunching and sub-Poisson photon statistics (also called antibunching) reveal the quan-tum nature of light and therefore have received a great deal of attention during the last decades. The first detection of antibunched light by Kimble, Dagenais and Mandel [1] and first detection of sub-Poisson light by Short and Mandel [2] are regarded as milestones in the progress in quantum optics. In spite of many experimental and theoretical achievements, a deeper analysis of these effects seems to be necessary, particularly in the case of nonstationary fields. We shall clarify some of these aspects by referring to an example of second-harmonic generation. There are several commonly used definitions of photon antibunching for a single-mode radiation field (e.g., Refs. [1]–[9]): Definition I: The photon antibunching (see, e.g., Ref. [3]) occurs if the two-time light intensity correlation function G(2)(t, t+ τ) increases from its initial value at τ = 0,

The concepts listed in the title are introduced and clarified. The relations among them are pointed out. It is shown that the corresponding optical phenomena are definitely of a quantum nature. The basic quantities which are measured in correlation optical experiments are discussed. Manifestations of photon antibunching and of sub-Poisson photon statistics in the recording of delayed coincidences, in the distribution of photon counts, and in intensity fluctuation spectra are analyzed. (More precisely, what is involved is the spectrum of fluctuations in the photocurrent; all the results of the theoretical analysis in this review are expressed in terms of directly measurable quantities.) A diagram technique for calculating the correlation characteristics of the radiation from a polyatomic system is outlined. Photon correlations in nonlinear resonance fluorescence are analyzed. There is a discussion of approaches to the development of macroscopic sources of radiation with sub-Poisson photon statistics: the production of a squeezed state of a field in phase-sensitive parametric effects in nonlinear optics and the introduction of repulsive statistics in luminescence excitation events and in the pumping of a laser. Experiments in these directions which had been reported through April 1986 are discussed. The practical importance of reducing the quantum noise in radiation for extremely precise measurements and for optical data transmission is pointed out.

A comprehensive review is given of investigations, both theoretical and experimental, that demonstrate interference to take place even when the fields involved are produced by independent sources. The physical situation is rather different for coherent and incoherent fields. In the first case, where the sources are lasers, a conventional interference pattern can be observed which is adequately described by the classical theory. In the present paper, special attention is paid to the question of whether this interference persists when the two laser beams become strongly attenuated. In the second case, the sources are individual atoms excited by a pumping mechanism, that emit spontaneously and, hence, independently from each other. In those circumstances, no interference pattern can show up. However, it becomes evident from both the classical and the quantum-mechanical theory that interference effects can still be established by observing intensity correlations rather than the intensity itself. This point is discussed in greater detail. The pioneering experiments of Forrester, Gudmundson and Johnson, and Brown and Twiss are reviewed in this context. Especially interesting from the theoretical point of view is the case of two emitting atoms, since then the classical and the quantum-mechanical description differ significantly, the quantum theory predicting the intensity correlations to be distinctly stronger than those following from classical considerations. This specific quantum-mechanical feature is shown to be intimately connected with the corpuscular aspect of light.

The statistical properties of fluorescent light from a single two-level atom driven by nonclassical light beams that exhibit antibunching and squeezing are discussed in the weak-field limit. The fields produced in intracavity second-harmonic generation and those produced by superposing the light from a degenerate parametric oscillator with a coherent field are considered to be the models of nonclassical light beams. These fields can be described in terms of real Gaussian random processes with nonzero mean coherent components. Analytical expressions for the fluorescent light intensity, the second-order intensity correlation function, and the variance of the photon number in the steady state are obtained. The effects of driving-field correlations, detuning, and other parameters characterizing the atom-field interaction on the statistics of scattered light are investigated. It is found that for a certain range of parameters the second-order intensity correlation function may vanish at nonzero times. Under certain other circumstances the antibunching of the fluorescent photons is enhanced. These and other interesting features that appear in the scattered light are discussed.

The quantum statistical properties of a single mode of the radiation field, prepared in the coherent state, interacting with a nonlinear medium of inversion symmetry are studied with the help of the usual two photon correlation function for zero time delay. We report the photon antibunching and sub-Poissonian photon statistics in addition to the usual photon bunching and the super-Poissonian photon statistics for an input vacuum field. The manipulation of the phase of input coherent light gives rise to the well known self induced transparency. The possible physical explanations for these events are presented.