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Soviet Physics Uspekhi

New phenomena in quantum optics: photon antibunching, sub-Poisson photon statistics, and squeezed states

D F Smirnov, A. S. Troshin

Published Oct 31, 1987• 55 citations
Publisher

Abstract

The concepts listed in the title are introduced and clarified. The relations among them are pointed out. It is shown that the corresponding optical phenomena are definitely of a quantum nature. The basic quantities which are measured in correlation optical experiments are discussed. Manifestations of photon antibunching and of sub-Poisson photon statistics in the recording of delayed coincidences, in the distribution of photon counts, and in intensity fluctuation spectra are analyzed. (More precisely, what is involved is the spectrum of fluctuations in the photocurrent; all the results of the theoretical analysis in this review are expressed in terms of directly measurable quantities.) A diagram technique for calculating the correlation characteristics of the radiation from a polyatomic system is outlined. Photon correlations in nonlinear resonance fluorescence are analyzed. There is a discussion of approaches to the development of macroscopic sources of radiation with sub-Poisson photon statistics: the production of a squeezed state of a field in phase-sensitive parametric effects in nonlinear optics and the introduction of repulsive statistics in luminescence excitation events and in the pumping of a laser. Experiments in these directions which had been reported through April 1986 are discussed. The practical importance of reducing the quantum noise in radiation for extremely precise measurements and for optical data transmission is pointed out.

DOI
10.1070/pu1987v030n10abeh002966

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•Jul 1, 1988•4 citations
The concepts listed in the title are introduced and clarified. The relations among them are pointed out. It is shown that the corresponding optical phenomena are definitely of a quantum nature. The basic quantities which are measured in correlation optical experiments are discussed. Manifestations of photon antibunching and of sub-Poisson photon statistics in the recording of delayed coincidences, in the distribution of photon counts, and in intensity fluctuation spectra are analyzed. (More precisely, what is involved is the spectrum of fluctuations in the photocurrent; all the results of the theoretical analysis in this review are expressed in terms of directly measurable quantities.) A diagram technique for calculating the correlation characteristics of the radiation from a polyatomic system is outlined. Photon correlations in nonlinear resonance fluorescence are analyzed. There is a discussion of approaches to the development of macroscopic sources of radiation with sub-Poisson photon statistics: the production of a squeezed state of a field in phase-sensitive parametric effects in nonlinear optics and the introduction of repulsive statistics in luminescence excitation events and in the pumping of a laser. Experiments in these directions which had been reported through April 1986 are discussed. The practical importance of reducing the quantum noise in radiation for extremely precise measurements and for optical data transmission is pointed out.
The statistical fluctuations of light can, under certain circumstances, exhibit a number of interesting nonclassical features. These include photon antibunching, sub-Poissonian statistics, and squeezing, all of which exist only in a quantum field. The three effects are distinct, and do not necessarily go together, although the first two are sometimes mistakenly treated as interchangeable. Both photon antibunching and sub-Poissonian statistics have been observed in experiments on resonance fluorescence from single atoms, which is described. Squeezing has not yet been seen experimentally, although many nonlinear processes are expected to give rise to it. The squeezed state can be recognized in heterodyne or homodyne experiments, where the squeezing becomes manifest as sub-Poissonian photon fluctuations.
A review is given of recent theoretical studies devoted to the problem of generating radiation fields that exhibit the opposite of the well-known bunching of photons observed in light from thermal sources, the so-called antibunching effect. It is made clear that this phenomenon reflects the corpuscular nature of light and, hence, cannot be interpreted in terms of classical electrodynamics, needing, instead, the quantum-mechanical formalism for its description. It is shown in some detail that nonlinear interaction mechanisms like multiphoton absorption and parametric three-wave interaction are suited to change the photon statistical properties of incident (in most cases coherent) light such that the output field will be endowed with antibunching properties. Special emphasis is given to the problem of correctly specifying the dimensions of the mode volume occurring in the usual single-mode treatment of the field, which is, in fact, of great practical interest, since the magnitude of the antibunching effect is determined by the inverse average number of photons contained in that volume. In a later section it is pointed out that destructive interference with a coherent reference beam provides a means of (a) effectively enhancing photon antibunching that is already present in a high-intensity field, through reduction of the intensity, and (b) transforming phase fluctuations produced in a Kerr medium into antibunching-type intensity fluctuations. On the other hand, there exists a way of directly generating light with antibunching properties, the physical mechanism being resonance fluorescence from a single atom. The main features of this technique, both theoretical and experimental, are outlined, including a discussion of the first experimental results obtained a few years ago.
We analyze the most popular approaches to photon antibunching as exemplified in a sim-ple model of second-harmonic generation. We find the exact evolution of the fundamental and harmonic fields for initial Fock states with small photon numbers. We show explicitly that definitions of photon antibunching based on the unnormalized, G(2)(t, t′), and normal-ized, g(2)(t, t′), two-time correlation functions describe distinct phenomena for nonstationary fields. For completeness, we also compare antibunching effects defined by the two-time and single-time correlations. 1 Photon antibunching Photon antibunching and sub-Poisson photon statistics (also called antibunching) reveal the quan-tum nature of light and therefore have received a great deal of attention during the last decades. The first detection of antibunched light by Kimble, Dagenais and Mandel [1] and first detection of sub-Poisson light by Short and Mandel [2] are regarded as milestones in the progress in quantum optics. In spite of many experimental and theoretical achievements, a deeper analysis of these effects seems to be necessary, particularly in the case of nonstationary fields. We shall clarify some of these aspects by referring to an example of second-harmonic generation. There are several commonly used definitions of photon antibunching for a single-mode radiation field (e.g., Refs. [1]–[9]): Definition I: The photon antibunching (see, e.g., Ref. [3]) occurs if the two-time light intensity correlation function G(2)(t, t+ τ) increases from its initial value at τ = 0,
Two manifestations of the quantum nature of coherent, resonant light scattering from atoms are photon antibunching and sub-Poissonian statistics. The existence of both effects has been demonstrated previously; in the present work, using individual barium atoms, measurements of the dependence of the latter effect on the frequency of the radiation field are presented. The distinction between the two phenomena is demonstrated by data that exhibit antibunching, yet have a photon counting distribution with variance equal to the Poisson value.
Nonclassical effects such as squeezing, antibunching, and sub-Poissonian statistics of photons have been attracting attention in quantum optics over the last decade. Up to now most theoretical and experimental investigations have been carried out exclusively in the time domain while neglecting the spatial aspects by considering only one spatial mode of the electromagnetic field. In many situations such an approximation is well justified. There are, however, problems that do not allow in principle a single-mode consideration. This is the case when one wants to investigate the quantum fluctuations of light at different spatial points in the plane perpendicular to the direction of propagation of the light beam. Such an investigation requires a complete description of quantum fluctuations of light in both time and space and cannot be done within a single-mode theory. This space-time description brings about a natural generalization into the spatial domain of such notions as the standard quantum limit, squeezing, antibunching, etc. It predicts, for example, the possibility of generating a light beam with sub-Poissonian statistics of photons not only in time but also in the beam's transverse plane. Of particular relevance to the applications is a situation in which the cross section of the light beam contains several nonoverlapping areas with sub-Poissonian statistics of photons in each. Photodetection of such a beam produces several sub-shot-noise photocurrents depending on the number of independent areas with sub-Poissonian statistics. This is in marked contrast to the case of a single-mode sub-Poissonian light beam in which any attempt to collect light from only a part of the beam deteriorates the degree of shot-noise reduction. This property of multimode squeezed light opens a range of interesting new applications in optical imaging, optical parallel processing of information, parallel computing, and many other areas in which it is desirable to have a light beam with regular photon statistics across its transverse area. The aim of this review is to describe the recent development in this branch of quantum optics.
A review is made of some quantum effects that have no classical analogs: antibunching and sub-Poisson statistics of photons, violation of the classical Cauchy-Schwarz inequality, and squeezed states of light. Nonclassical effects in the generation of harmonics and collective resonance fluorescence are investigated. Various schemes for generating squeezed states of light are proposed, and conditions for obtaining highly squeezed states are indicated. Possible applications of quantum light are also discussed.