Four-Photon Coherent Interaction

M. M. T. Loy

J.-C. Diels, Nandini Mukherjee, Arindum Mukherjee

Multiphoton coherent interaction effects are investigated in atoms and molecules. It is demonstrated theoretically as well as experimentally that, in the presence of a two photon resonance, maximum conversion efficiency can be achieved using energy preserving pulse sequences, in condition of coherent interaction. However, highest conversion efficiencies are obtained with weak two photon resonances. A study of four photon resonant coherent interaction in mercury points to a peculiar quenching of the interaction by the generated third harmonic. Four photon resonant coherent interaction is also investigated in molecules, where it is shown that an input signal can be found that results in selective excitation of the upper levels.

E. Gaižauskas, G. Gedvilas

Chen Mei-Feng

A scheme is presented for generating a four-photon coherent state via the degenerate Raman interaction. The scheme does not need classical fields to manipulate the atoms. Its another advantage is that the atomic spontaneous emission can be neglected. Therefore, the coherence of the system may be better maintained. The scheme can be generalized to generate superposition of 2 n coherent states and superposition of 2 n two-mode coherent states. The coherent states in each mode are on a circle symmetrically.

Holger Friedrich Hofmann, Kunihiro Kojima, Shigeki Takeuchi +1 more

We investigate the nonlinear interaction between two photons in a single-input pulse at an atomic two-level nonlinearity. A one-dimensional model for the propagation of light to and from the atom is used to describe the precise spatiotemporal coherence of the two-photon state. It is shown that the interaction generates spatiotemporal entanglement in the output state similar to the entanglement observed in parametric down-conversion. A method of generating photon pairs from coherent pump light using this quantum-mechanical four-wave mixing process is proposed.

M. M. T. Loy