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Annales de Physique

Lumino-réfrigération

P. E. Toschek

Published Jan 1, 1985• 11 citations
Publisher

Abstract

In a paper of 1950, Alfred Kastler proposed cooling of vapours by resonant light via optical pumping of the orientational levels of angular momentum, and successive collisions. Optical pumping of the degrees of freedom of the translational momentum is also feasible. This phenomenon has been demonstrated with ions, even with a single ion, in an electrodynamic or electromagnetic trap. Optical cooling by Raman-like two-photon transitions seems to be capable of generating ultra-low temperature levels.

DOI
10.1051/anphys:01985001006076100

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In a paper of 1950, Alfred Kastler proposed cooling of vapours by resonant light via optical pumping of the orientational levels of angular momentum, and successive collisions. Optical pumping of the degrees of freedom of the translational momentum is also feasible. This phenomenon has been demonstrated with ions, even with a single ion, in an electrodynamic or electromagnetic trap. Optical cooling by Raman-like two-photon transitions seems to be capable of generating ultra-low temperature levels.
When an atom or a molecule interacts with a light beam, the light emitted or absorbed carries valuable information about the atomic or molecular structure. This phenomenon underlies the whole field of spectroscopy. But the interaction of a photon with an atom can be used to manipulate the atom as well as to probe its structure. For example, in an approach called optical pumping, invented by Alfred Kastler, one can use the resonant exchange of angular momentum between atoms and polarized photons to align or orient the spins of atoms or to put them in nonequilibrium situations. In his original 1950 paper Kastler also proposed using optical pumping to cool and to heat the internal degrees of freedom, calling the phenomena the “effet luminofrigorique” and the “effet luminocalorique.” Another famous example of the use of photon-atom interaction to control atoms is laser cooling. This technique relies on resonant exchange of linear momentum between photons and atoms to control their external degrees of freedom and thus to reduce their kinetic energy. Laser cooling was suggested independently by Theodor Hänsch and Arthur Schawlow for neutral atoms and by David Wineland and Hans Dehmelt for trapped ions. In an article written three years ago for PHYSICS TODAY (June 1987, page 34), Wineland and Wayne Itano presented the principle of laser cooling and the potential applications of cold atoms to fields of physics such as ultrahigh resolution spectroscopy, atomic clocks, collisions, surface physics and collective quantum effects. At that time laser cooling had brought temperatures down to a few hundred microkelvin, but unexpected improvements during the last three years have dramatically lowered those temperatures to only a few microkelvin. We now feel we understand the new physical mechanisms responsible for these very low temperatures.
Optical pumping experiments on atomic ions which are stored in electromagnetic « traps » are discussed. Weak relaxation and extremely small energy shifts of the stored ions lead to very high resolution and accuracy in optical pumping-double resonance experiments. In the same spirit of Kastler's proposal for « lumino refrigeration » (1950), the kinetic energy levels of stored ions can be optically pumped. This technique, which has been called laser cooling, significantly reduces Doppler frequency shifts in the spectra.
Abstract A century ago Einstein introduced the notion of the linear momentum of a photon, h k, and analyzed its transfer to an atom (and back) in the establishment of thermodynamic equilibrium between black-body radiation and matter. In addition to a linear momentum, the photon also possesses an angular momentum, ħ, directed parallel (or antiparallel) to its propagation direction (the OZ axis in Fig. 4.1), depending on its polarization direction (left- or right-handed). This angular momentum is due to the spin of the photon, equal to 1. Half a century later, Kastler (1950) considered the use of the transfer of the angular momentum of a polarized photon to the angular momentum of an atom as a method of optical orientation of atoms. In essence, this was the first method to control atomic motion by means of low-intensity light, developed even before the advent of the laser; it which found widespread application in investigating and then using spin polarization effects in atomic physics. But even after lasers had made their appearance, the method of optical orientation of atoms (or pumping of certain magnetic sublevels in atoms) proved very important, specifically in the laser cooling of atoms (Chapter 5).