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Optical orientation of atoms and nuclei

Vladilen S Letokhov

Published Feb 15, 2007• 1 citation
Publisher

Abstract

Abstract A century ago Einstein introduced the notion of the linear momentum of a photon, h k, and analyzed its transfer to an atom (and back) in the establishment of thermodynamic equilibrium between black-body radiation and matter. In addition to a linear momentum, the photon also possesses an angular momentum, ħ, directed parallel (or antiparallel) to its propagation direction (the OZ axis in Fig. 4.1), depending on its polarization direction (left- or right-handed). This angular momentum is due to the spin of the photon, equal to 1. Half a century later, Kastler (1950) considered the use of the transfer of the angular momentum of a polarized photon to the angular momentum of an atom as a method of optical orientation of atoms. In essence, this was the first method to control atomic motion by means of low-intensity light, developed even before the advent of the laser; it which found widespread application in investigating and then using spin polarization effects in atomic physics. But even after lasers had made their appearance, the method of optical orientation of atoms (or pumping of certain magnetic sublevels in atoms) proved very important, specifically in the laser cooling of atoms (Chapter 5).

DOI
10.1093/oso/9780198528166.003.0004

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Abstract A century ago Einstein introduced the notion of the linear momentum of a photon, h k, and analyzed its transfer to an atom (and back) in the establishment of thermodynamic equilibrium between black-body radiation and matter. In addition to a linear momentum, the photon also possesses an angular momentum, ħ, directed parallel (or antiparallel) to its propagation direction (the OZ axis in Fig. 4.1), depending on its polarization direction (left- or right-handed). This angular momentum is due to the spin of the photon, equal to 1. Half a century later, Kastler (1950) considered the use of the transfer of the angular momentum of a polarized photon to the angular momentum of an atom as a method of optical orientation of atoms. In essence, this was the first method to control atomic motion by means of low-intensity light, developed even before the advent of the laser; it which found widespread application in investigating and then using spin polarization effects in atomic physics. But even after lasers had made their appearance, the method of optical orientation of atoms (or pumping of certain magnetic sublevels in atoms) proved very important, specifically in the laser cooling of atoms (Chapter 5).
More than a century ago, pioneeringworks carried out by Poynting (1909) and other physicists have provided the evidence of the validity of Marxwell equations for an electromagnetic field, showing how a beam of light carries energy and momentum, both in the linear and angular components. In particular the angular momentum of light, related to the generator of rotations in quantum mechanics, has been typically associated with its polarization, and more specifically with its circular polarization components. An optical beam traveling in the positive direction of the z axis that is circularly polarized, carries a z-component angular momentum content σ = ±h per photon, which is positive if the circular polarization is left-handed and negative if it is right-handed. This angular momentum content is not just a formal property, but a very concrete one that can have significant mechanical effects as for example an observable induced rotation by absorption to amaterial particle Beth (1936); Friese et al. (1998)
When an atom or a molecule interacts with a light beam, the light emitted or absorbed carries valuable information about the atomic or molecular structure. This phenomenon underlies the whole field of spectroscopy. But the interaction of a photon with an atom can be used to manipulate the atom as well as to probe its structure. For example, in an approach called optical pumping, invented by Alfred Kastler, one can use the resonant exchange of angular momentum between atoms and polarized photons to align or orient the spins of atoms or to put them in nonequilibrium situations. In his original 1950 paper Kastler also proposed using optical pumping to cool and to heat the internal degrees of freedom, calling the phenomena the “effet luminofrigorique” and the “effet luminocalorique.” Another famous example of the use of photon-atom interaction to control atoms is laser cooling. This technique relies on resonant exchange of linear momentum between photons and atoms to control their external degrees of freedom and thus to reduce their kinetic energy. Laser cooling was suggested independently by Theodor Hänsch and Arthur Schawlow for neutral atoms and by David Wineland and Hans Dehmelt for trapped ions. In an article written three years ago for PHYSICS TODAY (June 1987, page 34), Wineland and Wayne Itano presented the principle of laser cooling and the potential applications of cold atoms to fields of physics such as ultrahigh resolution spectroscopy, atomic clocks, collisions, surface physics and collective quantum effects. At that time laser cooling had brought temperatures down to a few hundred microkelvin, but unexpected improvements during the last three years have dramatically lowered those temperatures to only a few microkelvin. We now feel we understand the new physical mechanisms responsible for these very low temperatures.
The Wigner representation of angular-momentum orientation in the classical limit on $J\ensuremath{\gg}1$ has been used to derive an equation of angular-momentum motion in the case of a closed two-level system interacting with an arbitrary polarized radiation. This equation enables us to carry out a theoretical analysis of angular-momentum motion and consider final states of the quantum system for all types of dipole transitions. We have found that in the case of a zero magnetic field in the final state of the system with $\stackrel{\ensuremath{\rightarrow}}{J}J$ or $\stackrel{\ensuremath{\rightarrow}}{J}J+1$ optical transition, the angular momentum is directed along or opposite to the wave vector of the radiation depending on the sign of the polarization ellipsity, while for a linear polarization the angular momentum is isotropically distributed on the plane orthogonal to the polarization vector. For the $\stackrel{\ensuremath{\rightarrow}}{J}J\ensuremath{-}1$ transition two directions of angular momentum are possible in the final state. These directions are determined by the ellipsity of polarization. The spatial size of the final distribution of the angular momentum has been defined by the quantum uncertainty, 1/J,1/\sqrt{J},1/J​, of the angular-momentum orientation. In the case of the $\stackrel{\ensuremath{\rightarrow}}{J}J\ensuremath{-}1$ or $\stackrel{\ensuremath{\rightarrow}}{J}J,$ transition particles come into ``dark'' states while for the $\stackrel{\ensuremath{\rightarrow}}{J}J+1$ transition they occupy the ``brightest'' state. In the presence of a nonzero magnetic field, particles with $\stackrel{\ensuremath{\rightarrow}}{J}J$ transition have in the final state only one angular-momentum orientation, i.e., along or opposite to the direction of the magnetic field depending on the polarization ellipsity sign. For the $\stackrel{\ensuremath{\rightarrow}}{J}J+1$ transition both directions are possible, i.e., along and opposite to the magnetic field. In the case of the $\stackrel{\ensuremath{\rightarrow}}{J}J\ensuremath{-}1$ transition the directions of the angular momentum form a cone around the magnetic field.
In the preceding chapters, we discussed the manipulation and observation of atomic variables associated with the internal degrees of freedom. A complete separation between internal and external degrees of freedom, like position and momentum, is not always possible, however. It therefore appears appropriate to include a discussion of the mechanical effects of light, which have received increasing attention in recent years. The transfer of momentum between photons and atoms, first observed more than sixty years ago, had to wait for the wide availability of lasers to become a useful experimental tool. In particular the cooling of atoms and atomic ions to very low temperatures has found numerous applications. Light-induced forces That light exerts mechanical forces on massive particles like atoms may appear surprising. To motivate the existence of such an effect two different approaches are possible. The first approach considers the light as a collection of photons that carry, apart from energy and angular momentum, linear momentum as well. Photons interacting with atoms can therefore change the momentum of the atoms. The second approach considers light as a wave, i.e., an inhomogeneous electromagnetic field interacting with the atomic dipole moment. Both approaches provide a possible description for the numerous phenomena that can occur in this context, but in many situations, one of them turns out to be more intuitive or more useful for calculations than the other.
Anisotropy of angular momenta: ideas and methods The fundamental idea forming the basis of early quantum theory was the quantization of the angular momentum of the atom, which, at a later stage, assumed the form of the Bohr–Sommerfeld quantization rule [360], namely ∲ pdq = n ℏ where p and q are the generalized momentum and coordinate. This concept has retained its physical meaning in modern-day quantum mechanics [371, 372]. In the course of the further development of quantum mechanical concepts it became increasingly clear that in the theory of atoms and molecules the angular momentum is a ‘dominant’ notion, the fundamental significance of which is in no small degree connected with its dimension of action, which coincides with that of Planck's constant ℏ. In the interaction between particles and a directed beam of photons the angular momentum of the system is conserved, thus forming the basis for the optical method of producing spatial anisotropy of the distribution of the angular momenta of the ensemble of particles, i.e. its optical polarization . In terms of quantum concepts, spatial anisotropy means that in an ensemble of particles a non-equilibrium population of magnetic sublevels m j of angular momenta is created. We make a distinction between the alignment of momenta, for instance in the absorption of linear polarized light, when there is no difference between the population of ± m j -sublevels, and orientation , when such a difference exists. Anisotropic distribution of angular momenta in an excited state, as produced in absorption, manifests itself directly in the polarization of fluorescence. It is rather likely that understanding of the anisotropic distribution of the angular momenta of atoms was enhanced by Hanle's [184] discovery in 1924.
Abstract Optical pumping is an efficient method for initializing and maintaining atomic spin ensembles in a well-defined quantum spin state. Standard optical pumping methods orient the spins by transferring photonic angular momentum to spin polarization. Generally the spins are oriented along the propagation direction of the light due to selection rules of the dipole interaction. Here we present and experimentally demonstrate that by modulating the light polarization, angular momentum perpendicular to the optical axis can be transferred efficiently to cesium vapor. The transverse pumping scheme employs transversely oriented dark states, allowing for control of the trajectory of the spins on the Bloch sphere. This new mechanism is suitable and potentially beneficial for diverse applications, particularly in quantum metrology.