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Journal of Applied Physics

Time response of spin-polarized rubidium thermal gas with radio-frequency pulse driving

Yanhua Wang, Zhihua Kang, Yang Li, Qiang Ma, Yu Wang, Yabin Dong, Junmin Wang

Published Apr 4, 2022• 1 citation
Publisher

Abstract

The time evolution of the polarization of a rubidium atom spin ensemble driven by a resonant radio-frequency (RF) magnetic field is analyzed based on the rate equation. A simple optical pumping experimental system is constructed and the time response of the rubidium atomic ensemble is demonstrated by recording the transmitted intensity of pumping light. In the steady-state response, the polarization difference between the optical pumping steady state and the magnetic resonance steady state depends on the optical pumping power and RF magnetic intensity. We can obtain the optimal power value corresponding to the maximum polarization difference. In terms of transient response, where the intensity of RF magnetic field is too weak to observe Rabi oscillations, two decay processes between magnetic resonance and optical pumping steady states are monitored. The decay time from magnetic resonance steady state to optical pumping steady state depends on the optical pumping rate and the spin relaxation rate. The decay time from optical pumping steady state to magnetic resonance steady state depends on the optical pumping rate, the RF driving rate, and the spin relaxation rate. The scale factor of pumping rate to pumping power is obtained, in addition to that of RF driving rate to the RF magnetic field. It can provide an intuitive understanding of the spin dynamic evolution of the polarized atomic ensemble.

DOI
10.1063/5.0082535

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•Aug 21, 1961•0 citations
The time evolution of the polarization of a rubidium atom spin ensemble driven by a resonant radio-frequency (RF) magnetic field is analyzed based on the rate equation. A simple optical pumping experimental system is constructed and the time response of the rubidium atomic ensemble is demonstrated by recording the transmitted intensity of pumping light. In the steady-state response, the polarization difference between the optical pumping steady state and the magnetic resonance steady state depends on the optical pumping power and RF magnetic intensity. We can obtain the optimal power value corresponding to the maximum polarization difference. In terms of transient response, where the intensity of RF magnetic field is too weak to observe Rabi oscillations, two decay processes between magnetic resonance and optical pumping steady states are monitored. The decay time from magnetic resonance steady state to optical pumping steady state depends on the optical pumping rate and the spin relaxation rate. The decay time from optical pumping steady state to magnetic resonance steady state depends on the optical pumping rate, the RF driving rate, and the spin relaxation rate. The scale factor of pumping rate to pumping power is obtained, in addition to that of RF driving rate to the RF magnetic field. It can provide an intuitive understanding of the spin dynamic evolution of the polarized atomic ensemble.
We observe the transient evolution of the laser pumped magnetic resonance in a paraffin-coated rubidium vapor cell and analyze the phenomena numerically by using the four-level density matrix. With the increased radio frequency (RF) sweep rate, the traditional Lorentz signal turns to an asymmetric shape at low sweep rate and starts to oscillate at a high sweep rate. The transient oscillation's features, including frequency and the decay time, are studied by suddenly turning on the RF field to the resonance Larmor precession frequency under the different RF field and light field parameters. The experimental result reveals the transient signals' strong dependence on the RF field power and light power. Especially, the transient oscillation frequency primarily depends on the RF field's power and whatever power the laser light is. When the laser power is lower, the transient oscillation frequency is proportional to the RF field's amplitude. These transient evolution signals are also confirmed with the numerical calculations based on the density-matrix equation of motion.
Results of a fairly straightforward experiment on resonant magneto-optical rotation by rubidium-87 atoms revealed strong time-dependence of the polarization plane of light emerging from atomic vapors following a sudden irradiation with a laser beam. The rotation of the plane appears as a not direct consequence of the influence of the magnetic field on atoms. Reported measurements conducted using a vapor cell without any buffer gas or an anti-relaxation wall coating show that transmitted light has initially the same (linear) polarization as the incident one. Rotation of the polarization plane caused by an axial magnetic field develops in time scales similar to the pace of establishing the optical pumping/relaxation equilibrium in the atomic ensemble. The traditional passive Faraday rotation picture providing working description for the resonant magneto-optical effects in steady-state conditions does not explain the observed sequence of evolution of the polarization. The picture has to be augmented with analysis of time dependence in the spatial distribution of relevant quantum states within the atomic ensemble as well as longitudinal and transversal intensity profiles of the light beam. Isolation of external effects caused by the optical pumping and relaxation processes from consequences of internal atomic coherences should uncover more details of mechanisms of the latter in the presence of magnetic field. Plentitude of data available from time-dependent polarization measurements provides strong incentives for further development and tests of comprehensive models of coherent interactions of atomic ensembles with radiation and possibly a base for additional advance in understanding and applications of these phenomena.
The transient dynamics of atomic spins under oscillating and static magnetic fields have been studied in the spin-exchange relaxation-free (SERF) regime with a dual-beam configuration. The spin-relaxation rate can be accurately measured by detecting the transient response signal of the free induction decay (FID) process within several milliseconds. Leveraging this convenient method for measuring a large relaxation rate in a small cell volume, the dependence of the spin-relaxation rate on the probe intensity and ambient magnetic field was studied in the limit of low spin polarization. Moreover, by theoretical analysis of the dynamic evolution of the Rabi oscillation generated by a consecutive oscillating field and a small static magnetic field, we experimentally demonstrate that the amplitude of the Rabi oscillation is affected by the amplitude of the oscillating field in the SERF regime. According to the retrieved frequency of the FID signal and amplitude of relevant Rabi oscillation, the coil constants were 75.55 ± 0.78~nT/mA, 151.5 ± 0.9~nT/mA, and 116.6 ± 0.3~nT/mA along the x-, y-, and z-axes, respectively.
In this paper, we experimentally study the saturation effect of rubidium atomic magnetic resonance. A pump beam is applied to create atomic spin polarization, a radio frequency (RF) magnetic field is used to drive the spin precession about a static magnetic field, and an off-resonant linearly polarized probe beam is applied to detect the spin dynamics based on the Faraday-rotation effect. When the RF magnetic field intensity becomes strong, a saturation effect is observed. We measure the resonant peak under strong RF magnetic field driving and obtain a saturation dip as an indication of the saturation effect. Furthermore, we show that the line-width of the saturation dip is much smaller than that of magnetic resonance. Accordingly, the sensitivity of the precision measurement based on the saturation dip can be significantly improved. The relations between the saturation dip in the resonant peak and the driving RF magnetic field intensity, as well as pumping intensity, are also studied in our experiment.
A free-induction-decay (FID) type optically-pumped rubidium atomic magnetometer driven by a radio-frequency (RF) magnetic field is presented in this paper. Influences of parameters, such as the temperature of rubidium vapor cell, the power of pump beam, and the strength of RF magnetic field and static magnetic field on the amplitude and the full width at half maximum (FWHM) of the FID signal, have been investigated in the time domain and frequency domain. At the same time, the sensitivities of the magnetometer for the single-pass and the triple-pass probe beam cases have been compared by changing the optical path of the interaction between probe beam and atomic ensemble. Compared with the sensitivity of ∼21.2 pT/Hz1/2 in the case of the single-pass probe beam, the amplitude of FID signal in the case of the triple-pass probe beam has been significantly enhanced, and the sensitivity has been improved to ∼13.4 pT/Hz1/2. The research in this paper provids a reference for the subsequent study of influence of different buffer gas pressure on the FWHM and also a foundation for further improving the sensitivity of FID rubidium atomic magnetometer by employing a polarization-squeezed light as probe beam, to achieve a sensitivity beyond the photo-shot-noise level.
Abstract : A method for the optical observation of nutational resonance in optically pumped rubidium vapor has been studied both experimentally and theoretically. The method consists of pulsemodulating an rf magnetic field a one of the Zeeman resonance frequencies of the vapor and observing the resulting damped transient modulation in the transmitted light intensity. Of particular interest is the application of this method to a study of the spin relaxation of vapor atoms as influenced by the physical parameters of the system, in the case where the applied steady magnetic field is intense enough to cause individual Zeeman intervals to become noticeably unequal. Both single and double quantum resonances at a wide spectrum of Zeeman transitions of Rb-85 vapor diffusing through neon and helium buffer gases have been observed and identified, and the damping of the transient nutations in light intensity has been recorded under a variety of conditions. (Author)