The control and manipulation of the atomic translational and internal degrees of freedom via atom-laser interaction is an essential tool in modern quantum optical experiments which allows for a large variety of applications. The present work is concerned with theoretical investigations which may shed some light on certain experiments in this field.In the first part of this work, cooperative effects in the fluorescence of dipole-dipole interacting atoms in a trap are studied. The famous macroscopic quantum jumps can occur for a single atom with a metastable state when illuminated by light. Then periods of fluorescence of fixed intensity alternate stochastically with dark periods. If one has two or three such atoms in a trap, there are dark periods and periods of single and multiple intensity, from overlap. The statistics of these periods is influenced by the dipole-dipole interaction between the atoms in a sensitive manner. This work is concerned with a theoretical description of these effects, including a discussion of the seemingly contradictory experimental results which have been obtained in this context. The main result indicates that the huge rate of double and triple jumps reported for three trapped Ba+ ions can in fact not be attributed to the dipole-dipole interaction.In the second part, the possible use of an evanescent wave atomic mirror as a measuring device for the properties of an atomic wave packet is investigated. The idea is taken from an experiment, in which such a mirror was used for the temporal diffraction of a cloud of laser cooled atoms dropping out of a magneto-optical trap. A model for the investigation of the atomic wave function with such a mirror is given, and the outcomes of different set-ups are investigated. The main result shows that with such a mirror one can sample the mod-squared of a spread-out wave function, and this opens the way for a realistic possibility for measuring this otherwise not easily accessible quantity.
The control and manipulation of the atomic translational and internal degrees of freedom via atom-laser interaction is an essential tool in modern quantum optical experiments which allows for a large variety of applications. The present work is concerned with theoretical investigations which may shed some light on certain experiments in this field.In the first part of this work, cooperative effects in the fluorescence of dipole-dipole interacting atoms in a trap are studied. The famous macroscopic quantum jumps can occur for a single atom with a metastable state when illuminated by light. Then periods of fluorescence of fixed intensity alternate stochastically with dark periods. If one has two or three such atoms in a trap, there are dark periods and periods of single and multiple intensity, from overlap. The statistics of these periods is influenced by the dipole-dipole interaction between the atoms in a sensitive manner. This work is concerned with a theoretical description of these effects, including a discussion of the seemingly contradictory experimental results which have been obtained in this context. The main result indicates that the huge rate of double and triple jumps reported for three trapped Ba+ ions can in fact not be attributed to the dipole-dipole interaction.In the second part, the possible use of an evanescent wave atomic mirror as a measuring device for the properties of an atomic wave packet is investigated. The idea is taken from an experiment, in which such a mirror was used for the temporal diffraction of a cloud of laser cooled atoms dropping out of a magneto-optical trap. A model for the investigation of the atomic wave function with such a mirror is given, and the outcomes of different set-ups are investigated. The main result shows that with such a mirror one can sample the mod-squared of a spread-out wave function, and this opens the way for a realistic possibility for measuring this otherwise not easily accessible quantity.
A simplified scheme for the investigation of cooperative effects in the quantum jump statistics of small numbers of fluorescing atoms and ions in a trap is presented. It allows the analytic treatment of three dipole-dipole interacting four-level systems which model the relevant level scheme of Ba+ ions. For the latter, a huge rate of double and triple jumps was reported in a former experiment and the huge rate was attributed to the dipole-dipole interaction. Our theoretical results show that the effect of the dipole-dipole interaction on these rates is at most 5% and that for the parameter values of the experiment there is practically no effect. Consequently it seems that the dipole-dipole interaction can be ruled out as a possible explanation for the huge rates reported in the experiment.
The mutual dipole-dipole interaction of atoms in a trap can affect their fluorescence. Extremely large effects were reported for double jumps between different intensity periods in experiments with two and three Ba+ ions for distances in the range of about ten wave lengths of the strong transition while no effects were observed for Hg+ at 15 wavelengths. In this theoretical paper we study this question for configurations with three and four levels, which model those of Hg+ and Ba+, respectively. For two systems in the Hg+ configuration we find cooperative effects of up to 30% for distances around one or two wavelengths, about 5% around ten wavelengths, and, for larger distances in agreement with experiments, practically none. This is similar for two V systems. However, for two four-level configurations, which model two Ba+ ions, cooperative effects are practically absent, and this latter result is at odds with the experimental findings for Ba+.
The recent development of laser cooling and trapping techniques has made possible the controlled realization of dense and cold atomic samples, thus opening the way for spectroscopic investigations in the low and ultra-low temperature regimes not accessible with conventional techniques. In our lab, an apparatus for laser cooling and Bose-Einstein condensation of rubidium atoms is in operation, producing a sample large enough to perform reliable investigations by absorption or emission techniques. Moving from previous photoionization experiments of laser-cooled atoms in a magneto-optical trap irradiated by cw-laser radiation [1] and stimulated by the interest grown recently on ultra-cold plasma [2], we have started a series of experiments aimed at investigating the interaction of intense laser pulses with the ultra-cold neutral sample, boty aboeand below the condensation temperature. Radiation from an excimer-pumped dye laser was used at a wavelength close to 594 nm, corresponding to the ionization threshold of rubidium for two photon non-resonant absorption from the ground state, with intensities in the tens of MW/cm^2 range and a pulse duration of 16 ns. Preliminary results, attained through the dynamical analysis (atom number, temperature) of the cold atom sample after the arrival of the laser pulse, suggest the occurrence of different processes, initiated by multi-photon ionization, involving collisions between cold electrons and ultra-cold neutrals, recombination at low temperatures and collective processes in the weak and cold plasma. Interpretation of those results demonstrates that this class of experiments, based on a variety of topics typical of atomic, plasma and statistical physics, can open the way for novel and intriguing investigations of laser-matter interaction. Further experimental developments will include duplication of the laser pulse frequency and one photon ionization of ground state rubidium laser-cooled atoms. [1] O. Maragò et al., Phys. Rev. A 57 R4110 (1998); E., Arimondo et al., Appl. Surf. Sci. 154-155 527 (2000); F. Fuso et al., Opt. Commun. 173 223 (2000). [2] T.C. Killian et al., Phys. Rev. Lett. 83 4776 (1999); S. Kulin et al., Phys. Rev. Lett. 85 318 (2000).
The problem of the interaction of N atoms with a laser beam and vacuum modes can give rise to many interesting phenomena concerning the spontaneous emission of light and its propagation in the medium. The cooperative effects, for example, such as superadiance and subradiance, are effects related to the coherence created between the atoms when a photon is emitted spontaneously by a single excited atom. Superradiance can be defined as the enhancement of the spontaneous emission due to constructive interference of the scattered light. Its counterpart, subradiance, is the trapping of some remaining light due to destructive interference. In cold atoms, some previous theoretical works predict and characterize these two cooperative effects in a large and diluted atomic cloud, in the regime of low intensities and large detunings of the incident laser. The theoretical model is a coupled-dipole model for two-level atoms driven by a low-intensity field and in the scalar approach. The experiment consists in measuring the super- and subradiant decay rates from the temporal emitted intensity after the switch off of the incident laser in the steady state. Our experimental setup consists in a magneto-optical trap of rubidium 87 atoms at large resonant optical thicknesses. A probe beam excites the atoms close to the D2 line. The intensity emitted is detected by a single photon detector with no afterpulsing and a calibration procedure allows us to determine the resonant optical thickness of the cloud and its temperature. In this work, we report the experimental observation of super- and subradiance in a large cloud of cold atoms. For subradiance, the main result is the linear evolution of the characteristic time with the resonant optical thickness of the cloud and its independence of the detuning. For superradiance, we observe superradiance out of the forward direction. We verify the validity of our interpretations with the predictions of the coupled-dipole model. Finally, we discuss the interplay of subradiance and radiation trapping, as well as theoretical predictions for: a setup of a phased cloud, to control the subradiant amplitude emission; and temperature effects, where subradiance is shown to be robust in a large range of temperatures.
Light and atoms couple together via the electromagnetic interaction. The simplest form of this interaction is the electric dipole interaction, and in its quantised form it provides a useful starting point for the investigation of quantum effects in optics. Two examples of quantum noise manipulation of the light field due to interaction with atoms will be presented, as well as an analysis of a simple model for laser cooling of trapped atoms. The first example of quantum noise manipulation is the investigation of a quantum non-demolition measurement scheme based on a three-level atomic system in the ladder configuration. An effective two-level model of the atomic system is used, which enables the inclusion of spontaneous emission noise from the upper atomic level. The system is found to perform well, when detuned far from resonance. The second example is the treatment of squeezing in the intensity difference between two modes coupled by a three-level atomic system in the ladder configuration. The noise correlations are similar to those occurring in the optical parametric oscillator, and give rise to good squeezing when the system is well detuned from the intermediate level. The simple model of laser cooling consists of a single two-level atom with quantised centre-of-mass motion constrained to move in a one-dimensional harmonic potential while interacting with a single-mode classical travelling light field. It is shown that there is an analogy between this model and the Jaynes-Cummings model. This gives rise to interesting coherent effects including quantum collapses and revivals in the atomic inversion. Sideband cooling occurs for this model when the light field is tuned to the atom's first lower vibrational sideband. The strong sideband and Lamb-Dicke perturbation regimes are defined. Analytic results have previously been obtained for the latter regime, but we carry out a numerical investigation of the steady state and time evolution behaviour in the former regime. Differences in the behaviour in the two regimes are discussed. Finally the possibility of observing quantum jumps between trap levels is discussed.
This thesis presents experiments concerning the preparation and manipulation of single neutral atoms in optical traps. The experimental setup as well as the properties of the optical dipole trap are described. The examination and control of all trapping parameters and heating effects is a prerequisite for the future realization of quantum gates. A magneto-optical trap captures and cools down a few cesium atoms. By efficiently detecting their fluorescence, we are able to determine their exact number. They are then transferred without loss into a standing-wave optical dipole trap. The temperature of the atoms in this trap is measured using two methods which are devised to work with small numbers of atoms: By adiabatically lowering the trap depth, an energy-selective loss of atoms is obtained, which yields the energy distribution of the atoms in the trap. Alternatively, the temperature is inferred from the size of the cloud and from the oscillation frequencies of the atoms in the dipole trap. The oscillation frequencies are determined using resonant and parametric excitation. Various intrinsic as well as technical heating mechanisms in the dipole trap are examined experimentally and theoretically. Finally, the setup of a miniature ultra-high finesse optical resonator is presented, which will be used to couple two trapped atoms via the exchange of a photon. The optical resonance frequency of the resonator is successfully stabilized to the atomic transition by an electronic servo loop.